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arXiv:2410.04505 · Physical Review A

Efficient characterization of spatial Schmidt modes of multiphoton entangled states produced from high-gain parametric down-conversion

Mahtab Amooei, Girish S. Kulkarni, Jeremy Upham, Robert W. Boyd

Published Feb 27, 2025• 6 citations
arXivHTMLPDF

Abstract

The ability to efficiently characterize the spatial correlations of entangled states of light is critical for applications of many quantum technologies such as quantum imaging. Here, we demonstrate highly efficient theoretical and experimental characterization of the spatial Schmidt modes and the Schmidt spectrum of bright multiphoton entangled states of light produced from high-gain parametric down-conversion. In contrast to previous studies, we exploit the approximate quasihomogeneity and isotropy of the signal field and dramatically reduce the numerical computations involved in the experimental and theoretical characterization procedures. In our particular case where our experimental datasets consist of 5000 single-shot images of $256\ifmmode\times\else\texttimes\fi{}256$ pixels each, our method reduced the overall computation time by 2 orders of magnitude. This speedup would be even more dramatic for larger input sizes. Consequently, we are able to rapidly characterize the Schmidt modes and the Schmidt spectrum for a range of pump amplitudes and study their variation with increasing gain. Our results clearly reveal the broadening of the Schmidt modes and the narrowing of the Schmidt spectrum for increasing gain with agreement between theory and experiment.

DOI
10.1103/physreva.111.023714

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•Jan 1, 2026•0 citations
The ability to efficiently characterize the spatial correlations of entangled states of light is critical for applications of many quantum technologies such as quantum imaging. Here, we demonstrate highly efficient theoretical and experimental characterization of the spatial Schmidt modes and the Schmidt spectrum of bright multiphoton entangled states of light produced from high-gain parametric down-conversion. In contrast to previous studies, we exploit the approximate quasihomogeneity and isotropy of the signal field and dramatically reduce the numerical computations involved in the experimental and theoretical characterization procedures. In our particular case where our experimental datasets consist of 5000 single-shot images of 256\ifmmode×\else\texttimes\fi256256\ifmmode\times\else\texttimes\fi{}256256\ifmmode×\else\texttimes\fi256 pixels each, our method reduced the overall computation time by 2 orders of magnitude. This speedup would be even more dramatic for larger input sizes. Consequently, we are able to rapidly characterize the Schmidt modes and the Schmidt spectrum for a range of pump amplitudes and study their variation with increasing gain. Our results clearly reveal the broadening of the Schmidt modes and the narrowing of the Schmidt spectrum for increasing gain with agreement between theory and experiment.
The full Schmidt decomposition of spatiotemporally entangled states generated from spontaneous parametric down-conversion (SPDC) has not been carried out until now due to the immense computational complexity arising from the large dimensionalities of the states. In this Letter, we utilize the rotational symmetry of the states to reduce the complexity by at least four orders of magnitude and carry out the decomposition to reveal the precise forms of the spatiotemporal Schmidt modes and the Schmidt spectrum spanning over 10^4 modes. We show that the Schmidt modes have a phase profile with a transverse spatial vortex structure that endows them with orbital angular momentum at all frequencies. In the high-gain regime, these Schmidt modes broaden and the Schmidt spectrum narrows with increasing pump strength. Our work can spur novel applications at the intersection of quantum imaging and spectroscopy that utilize entangled states produced from SPDC.
High-dimensional spatially entangled two-photon state generated by spontaneous parametric down-conversion process (SPDC) has become a promising resource for several quantum information science applications. For harnessing high-dimensional entanglement advantages, detection capability in the Schmidt basis is a necessity. Spatial entanglement has been explored in several modal bases, such as pixel, azimuthal, and radial modes. Among them, pixel and azimuthal entanglement have been widely utilized due to efficient access to their Schmidt modes, while radial-mode entanglement remains underexploited. This is because for radial coordinates, there is neither a Schmidt-decomposed form for the SPDC photons nor is there a technique for measuring high-dimensional radial Schmidt modes, which is a major roadblock in harnessing radial mode advantages. In this work, we first theoretically show that the azimuthal averaging of SPDC two-photon state yields a radial Schmidt-decomposed form under typical experimental situations. We then demonstrate an innovative approach for extracting the radial Schmidt modes and their spectrum by characterizing the density matrix in the radial basis of one of the SPDC photons. Finally, we report the first-ever measurement of radial Schmidt spectrum of upto 50 radial Schmidt modes with about 98\% fidelity.
Abstract High-dimensional spatially entangled two-photon states generated by the spontaneous parametric down-conversion process (SPDC) have become a promising resource for several quantum information science applications. In order to harness high-dimensional entanglement advantages, detection capability in the Schmidt basis is a necessity. Spatial entanglement has been explored in several modal bases, such as pixel, azimuthal, and radial modes. Among them, pixel and azimuthal entanglement have been widely utilized due to efficient access to their Schmidt modes, while radial-mode entanglement remains underexploited. This is due to radial coordinates not having a Schmidt-decomposed form for the SPDC photons or a technique for measuring high-dimensional radial Schmidt modes, which is a major roadblock in harnessing radial mode advantages. In this work, we first theoretically show that azimuthal averaging of SPDC two-photon states yields a radial Schmidt-decomposed form under typical experimental situations. We then demonstrate an innovative approach for extracting the radial Schmidt modes and their spectrum by characterizing the density matrix in the radial basis of one of the SPDC photons. Finally, we report the first-ever measurement of the radial Schmidt spectrum of up to 50 radial Schmidt modes with about 98% fidelity.
Multimode quantum light has promising applications in many areas of physics, such as quantum communications and quantum computing. However, its multimode nature also makes it challenging to measure its properties. Recently [I. Barakat , ], a technique for the simultaneous measurement of squeezing of multiple broadband modes based on a phase-sensitive amplification approach was experimentally implemented using a setup that effectively corresponds to an SU(1,1) interferometer. Here, we aim to provide a complete theoretical analysis of the modal structure of (generally unbalanced) SU(1,1) interferometers and a detailed theoretical formal derivation of the framework for this technique. Utilizing the joint Schmidt decomposition of the transfer functions, we investigate the shape and phase profiles of the modes of the SU(1,1) interferometer and its components [parametric down-conversion (PDC) sections] for different parametric gain regimes. We discover a complicated interplay between the PDC modes and the modes of the entire interferometer, and analyze it by using their overlap coefficients as a similarity measure. Finally, we develop a rigorous processing method for the aforementioned multimode squeezing measurement technique and discuss necessary approximations to make this method experimentally feasible.
Spontaneous parametric down-conversion (SPDC) is the most widely-used source of high-dimensional entangled two-photon states, and the entanglement in the spatial degree of freedom is considered best suited for harnessing high-dimensional advantages. Although the Schmidt basis provides a natural choice for state characterisation of entangled two-photon states in any degree of freedom, there is currently no technique that can measure the Schmidt basis of an entangled two-photon field. The existing techniques can only reconstruct the Schmidt spectrum when the Schmidt basis is known a priori. In contrast, we present a technique that measures the complete set of spatial Schmidt modes without any prior knowledge. Using this technique, we report measurement of states with over 3000 Schmidt modes -- highest reported yet -- with up to 98%\%% fidelity. We expect our work to significantly advance the harnessing of high-dimensional advantages in SPDC-based systems.
Multimode quantum light has promising applications in many areas of physics, such as quantum communications and quantum computing. However, its multimode nature also makes it challenging to measure its properties. Recently [I. Barakat et al., Optica Quantum 3, 36 (2025)], a technique for the simultaneous measurement of squeezing of multiple broadband modes based on a phase-sensitive amplification approach was experimentally implemented using a setup that effectively corresponds to an SU(1,1) interferometer. Here, we aim to provide a complete theoretical analysis of the modal structure of (generally unbalanced) SU(1,1) interferometers and a detailed theoretical formal derivation of the framework for this technique. Utilizing the joint Schmidt decomposition of the transfer functions, we investigate the shape and phase profiles of the modes of the SU(1,1) interferometer and its components [parametric down-conversion (PDC) sections] for different parametric gain regimes. We discover a complicated interplay between the PDC modes and the modes of the entire interferometer, and analyze it by using their overlap coefficients as a similarity measure. Finally, we develop a rigorous processing method for the aforementioned multimode squeezing measurement technique and discuss necessary approximations to make this method experimentally feasible.