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arXiv:2409.19695 · Physica Scripta

Infinite cycles of interacting bosons

András Sütö

Published Oct 11, 2024• 0 citations
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Abstract

Abstract In the first-quantized description of bosonic systems permutation cycles formed by the particles play a fundamental role. In the ideal Bose gas Bose-Enstein condensation (BEC) is signaled by the appearance of infinite cycles. When the particles interact, the two phenomena may not be simultaneous, the existence of infinite cycles is necessary but not sufficient for BEC. We demonstrate that their appearance is always accompanied by a singularity in the thermodynamic quantities which in three and four dimensions can be as strong as a one-sided divergence of the isothermal compressibility. Arguments are presented that long-range interactions can give rise to unexpected results, such as the absence of infinite cycles in three dimensions for long-range repulsion or their presence in one and two dimensions if the pair potential has a long attractive tail.

DOI
10.1088/1402-4896/ad8602

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Abstract In the first-quantized description of bosonic systems permutation cycles formed by the particles play a fundamental role. In the ideal Bose gas Bose-Enstein condensation (BEC) is signaled by the appearance of infinite cycles. When the particles interact, the two phenomena may not be simultaneous, the existence of infinite cycles is necessary but not sufficient for BEC. We demonstrate that their appearance is always accompanied by a singularity in the thermodynamic quantities which in three and four dimensions can be as strong as a one-sided divergence of the isothermal compressibility. Arguments are presented that long-range interactions can give rise to unexpected results, such as the absence of infinite cycles in three dimensions for long-range repulsion or their presence in one and two dimensions if the pair potential has a long attractive tail.
Based on the paper "Fourier formula for quantum partition functions", arXiv:2106.10032 [math-ph], we show that in an infinite system of identical bosons interacting via a positive-type pair potential there is off-diagonal long-range order if and only if a nonzero fraction of the particles form infinite permutation cycles. In particular, there is Bose-Einstein condensation if and only if the diverging cycle lengths increase at least as fast with NNN, the number of particles, as N2/dN^{2/d}N2/d in d≥3d\geq 3d≥3 dimensions. This extends a similar result known for the ideal Bose gas.
We study the relationship between long cycles and Bose-Einstein condensation (BEC) in the case of several models. A convenient expression for the density of particles on cycles of length qqq is obtained, in terms of qqq unsymmetrised particles coupled with a boson field. Using this formulation we reproduce known results on the Ideal Bose Gas, Mean-Field and Perturbed Mean-Field Models, where the condensate density exactly equals the long cycle density. Then we consider the Infinite-Range-Hopping Bose-Hubbard model, with and without hard-cores. For the hard-core case, we find we can disregard the hopping contribution of the q unsymmetrised particles to obtain an exact expression for the density of particles on long cycles. It is shown that only the cycle of length one contributes to the cycle density. We conclude that while the existence of a non-zero long cycle density coincides with the occurrence of Bose-Einstein condensation, the respective densities are not necessarily equal. For the case of a finite on-site repulsion, we obtain an expression for the cycle density by neglecting the qqq unsymmetrised hop. Inspired by the Approximating Hamiltonian method we conjecture a simplified expression for the short cycle density as a ratio of single-site partition functions. In the absence of condensation we prove that this simplification is exact and find that in this case the long-cycle density vanishes. In the presence of condensation we justify this simplification when a gauge-symmetry breaking term is introduced in the Hamiltonian. Assuming our conjecture is correct, we compare numerically the long-cycle density with the condensate and again find that though they coexist, in general they are not equal.
We prove two equilibrium properties of a system of interacting atoms in three or higher dimensional continuous space. (i) If the particles interact via pair potentials of a nonnegative Fourier transform, their self-organization into infinite permutation cycles is simultaneous with off-diagonal long-range order. If the cycle lengths tend to infinity not slower than the square of the linear extension of the system, there is also Bose-Einstein condensation. (ii) If the pair potential is also nonnegative, cycles composed of a nonzero fraction of the total number of particles do appear if the density exceeds a temperature-dependent threshold value. The two together constitute the proof that in such a system Bose-Einstein condensation takes place at high enough densities.
The canonical partition function of a Bose gas gives rise to a probability distribution over the permutations of N particles. The author studies the probability and mean value of the cycle lengths in the cyclic permutations, their relation to physical quantities like pair correlations, and their thermodynamic limit. He shows that in the ground state of most interacting boson gases the mean cycle length diverges in the bulk limit and the particles form macroscopic cycles. In the free Bose gas Bose-Einstein condensation is accompanied by a percolation transition: the appearance of infinite cycle with nonvanishing probability.
In this third paper of a series that started with arXiv:2106.10032 [math-ph] and continued with arXiv:2108.02659 [math-ph] we show that in d≥3d\geq 3d≥3 dimensions at low temperatures or high densities bosons interacting via pair potentials that are both positive and positive type form permutation cycles whose length diverges proportionally with the number of particles. Based on the second-cited paper, this implies Bose-Einstein condensation.
We consider interacting Bose particles in an external potential. It is shown that a Bose-Einsteincondensate is possible at finite temperatures that describes a supersolid in three dimensions (3D) for a wide range of potentials in the absence of an external potential. However, for 2D, a self-organized supersolid exists for finite temperatures provided the interaction between bosons is nonlocal and of infinitely long-range. It is interesting that in the absence of the latter type of potential and in the presence of a lattice potential, there is no Bose-Einstein condensate and so in such a case, a 2D supersolid is not possible at finite temperatures. We also propose the correct Bloch form of the condensate wave function valid for finite temperatures, which may be used as the correct trial wave function.