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arXiv:2409.19683 · npj Quantum Information

True decoherence-free-subspace derived from a semiconductor double quantum dot Heisenberg spin-trimer

Wonjin Jang, Jehyun Kim, Jaemin Park, Min-Kyun Cho, Hyeongyu Jang, Sangwoo Sim, Hwanchul Jung, V. Umansky, Dohun Kim

Published Dec 18, 2025• 2 citations
arXivHTMLPDF

Abstract

Spins in solid systems can inherently serve as qubits for quantum simulation or quantum information processing. Spin qubits are usually prone to environmental magnetic field fluctuations; however, a spin qubit encoded in a decoherence-free-subspace (DFS) can be protected from certain degrees of environmental noise depending on the specific structure of the DFS. Here, we derive the “true” DFS from an antiferromagnetic Heisenberg spin-1/2 trimer, which protects the qubit states against both short- and long-wavelength magnetic field fluctuations. We define the spin trimer with three electrons confined in a gate-defined GaAs double quantum dot (DQD) where we exploit Wigner-molecularization in one of the quantum dots. We first utilize the trimer for dynamic nuclear polarization (DNP), which generates a sizable magnetic field difference, Δ B z , within the DQD. We show that large Δ B z significantly alters the eigenspectrum of the trimer and results in the “true” DFS in the DQD. Real-time Bayesian estimation of the DFS energy gap explicitly demonstrates protection of the DFS against short-wavelength magnetic field fluctuations in addition to long-wavelength ones. Our findings pave the way toward compact DFS structures for exchange-coupled quantum dot spin chains, the internal structure of which can be coherently controlled completely decoupled from environmental magnetic fields.

DOI
10.1038/s41534-025-01151-5

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Spins in solid systems can inherently serve as qubits for quantum simulation or quantum information processing. Spin qubits are usually prone to environmental magnetic field fluctuations; however, a spin qubit encoded in a decoherence-free-subspace (DFS) can be protected from certain degrees of environmental noise depending on the specific structure of the DFS. Here, we derive the “true” DFS from an antiferromagnetic Heisenberg spin-1/2 trimer, which protects the qubit states against both short- and long-wavelength magnetic field fluctuations. We define the spin trimer with three electrons confined in a gate-defined GaAs double quantum dot (DQD) where we exploit Wigner-molecularization in one of the quantum dots. We first utilize the trimer for dynamic nuclear polarization (DNP), which generates a sizable magnetic field difference, Δ B z , within the DQD. We show that large Δ B z significantly alters the eigenspectrum of the trimer and results in the “true” DFS in the DQD. Real-time Bayesian estimation of the DFS energy gap explicitly demonstrates protection of the DFS against short-wavelength magnetic field fluctuations in addition to long-wavelength ones. Our findings pave the way toward compact DFS structures for exchange-coupled quantum dot spin chains, the internal structure of which can be coherently controlled completely decoupled from environmental magnetic fields.
Quantum computing promises significant speed-up for certain types of computational problems. However, robust implementations of semiconducting qubits must overcome the effects of charge noise that currently limit coherence during gate operations. Here we describe a scheme for protecting solid-state qubits from uniform electric field fluctuations by generalizing the concept of a decoherence-free subspace for spins, and we propose a specific physical implementation: a quadrupole charge qubit formed in a triple quantum dot. The unique design of the quadrupole qubit enables a particularly simple pulse sequence for suppressing the effects of noise during gate operations. Simulations yield gate fidelities 10-1,000 times better than traditional charge qubits, depending on the magnitude of the environmental noise. Our results suggest that any qubit scheme employing Coulomb interactions (for example, encoded spin qubits or two-qubit gates) could benefit from such a quadrupolar design.
Spin degrees of freedom have been extensively explored in the context of quantum information processing. Many proposals of quantum computation architectures use spins as carriers of quantum of information. A central problem is to efficiently generate quantum entanglement between spin qubits which proves to be a crucial resource for quantum information tasks. On the other hand, uncontrollable spin degrees of freedom in the environment of spin qubits are the major causes of errors at low temperature, for example, the lattice nuclear spins hyperfine coupled to single electron spin qubit localized in semiconductor nano-structures. An outstanding problem for scalable quantum computation is to suppress the collective fluctuations from such spin baths so that the coherence time of the spin qubit can be improved. With these two motivations, the problems of suppressing collective spin fluctuations and generating entanglement in various spin ensembles are addressed in this thesis.\n\n\n\nIn the first half of the thesis, two approaches are introduced for suppressing the collective fluctuations in the nuclear spin bath so that the quantum coherence time of electron spin qubit in semiconductor quantum dots can be improved. The first approach works for a coupled double dot system. A theory for the interaction with the nuclear spins is developed when the two-electron singlet state is in resonance with one of the triplet state in moderate external magnetic field. At this resonance condition, the nuclear-electron flip-flop process caused by the hyperfine interaction can lead to a feedback mechanism, which can be used to suppress the nuclear hyperfine field. The second approach works for a single dot system. It is shown that strong pumping of the nuclear spins in dynamic nuclear polarization processes can saturate the nuclear spin bath towards the collective “dark states”. In such dark states, the transverse nuclear field fluctuation can be substantially suppressed compared to the value at thermal equilibrium. Two physical schemes are proposed to realize the nuclear dark states for suppression of the nuclear field fluctuations.\n\n\n\nIn the second half of the thesis, schemes are presented for generating large scale quantum entanglement in two types of spin qubit systems. For atomic spin qubits in optical lattices, schemes are proposed on how to prepare pure spin coherent state (SCS) with low collective spin by incoherent pumping with collective spin raising and lowering operations. Such SCS realize networks of mutually entangled spins which can be idea resources for the quantum telecloning algorithm. For donor nuclear spin qubits in silicon architecture, proposals are shown on how to deterministic prepare Dicke states which constitute an important class of multipartite entangled states. Our scheme is capable of preparing both symmetric and asymmetric Dicke states which form a complete basis set of the spin Hilbert space. The required controls are in situ to the prototype Kane’s quantum computer. The preparation is robust because each desired Dicke state is the steady state under designed pumping process. The schemes presented here also make possible the construction of decoherence free subspaces where quantum information is protected from collective noises.
We propose altermagnetic semiconductors as a platform for field-free, all-electrically controlled spin qubits in gate-defined quantum dots. The momentum-dependent spin splitting of an altermagnet produces a Zeeman-like qubit splitting whose magnitude and sign are set by the dot ellipticity, enabling local frequency tunability without external magnetic fields or micromagnets. Because the splitting is tied to a fixed altermagnetic quantization axis, electric-field noise is longitudinally suppressed at leading order, while quantization-axis fluctuations couple transversely and therefore cause relaxation rather than pure dephasing. The compensated magnetic order also avoids stray fields, making the platform naturally compatible with superconducting resonators and dispersive circuit-QED readout through the qubit's spin-dependent electric dipole. Starting from an effective quantum-dot model, supported by a microscopic lattice model, we derive the single- and two-dot Hamiltonian models. We show that electric-dipole spin resonance enables single-qubit control, while tunable exchange and electrically addressable qubit frequencies realize fSim two-qubit gates. The same double-dot architecture also supports singlet-triplet qubits with electrical control of both exchange and splitting gradients, removing the need for micromagnets or nuclear-polarization gradients. These results establish altermagnetic quantum dots as a route to field-free spin qubits with intrinsic electrical tunability and enhanced dephasing protection.
Abstract Electron spins in semiconductors are promising qubits because their long coherence times enable nearly 10 9 coherent quantum gate operations. However, developing a scalable high-fidelity two-qubit gate remains challenging. Here, we demonstrate an entangling gate between two double-quantum-dot spin qubits in GaAs by using a magnetic field gradient between the two dots in each qubit to suppress decoherence due to charge noise. When the magnetic gradient dominates the voltage-controlled exchange interaction between electrons, qubit coherence times increase by an order of magnitude. Using randomized benchmarking, we measure single-qubit gate fidelities of ~ 99%, and through self-consistent quantum measurement, state, and process tomography, we measure an entangling gate fidelity of 90%. In the future, operating double quantum dot spin qubits with large gradients in nuclear-spin-free materials, such as Si, should enable a two-qubit gate fidelity surpassing the threshold for fault-tolerant quantum information processing.
We present a scheme for implementing robust quantum gates in decoherence-free subspaces (DFSs) with double-dot spin qubits. Through the resonator-assisted interaction, the controllable interqubit couplings can be achieved only by adjusting the qubit transition frequencies. We construct a set of logic gates on the DFS-encoded qubits to eliminate the collective noise effects, and thus the gate fidelities can be enhanced remarkably. This proposal may offer a potential approach to realize the robust quantum computing with spin qubits.
We propose a quadrupolar exchange-only spin qubit that is highly robust against charge noise and nuclear spin dephasing, the dominant decoherence mechanisms in quantum dots. The qubit consists of four electrons trapped in three quantum dots, and operates in a decoherence-free subspace to mitigate dephasing due to nuclear spins. To reduce sensitivity to charge noise, the qubit can be completely operated at an extended charge noise sweet spot that is first-order insensitive to electrical fluctuations. Because of on-site exchange mediated by the Coulomb interaction, the qubit energy splitting is electrically controllable and can amount to several GHz even in the "off" configuration, making it compatible with conventional microwave cavities.