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arXiv:2409.12503

Progress towards efficient 4-level photon echo memories

James S. Stuart, K. Smith, Morgan P. Hedges, Rose L. Ahlefeldt, Matthew J. Sellars

Published Sep 19, 2024• 0 citations
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Abstract

Quantum memories could benefit many devices in quantum information processing. For a quantum to be useful in real-world applications, the quantum memory must have a high recall efficiency. Here we demonstrate an efficient (up to 80%) spin-storage quantum memory in Er:YSO, using the 4-level rephased amplified spontaneous emission protocol. We show non-classical correlations between the ASE and RASE fields produced by the quantum memory. Also, we demonstrate the storage of 70 temporal modes, with a write time of 150 us, and a storage time of 25 us. Finally, a clear pathway is presented to improve the efficiency, storage time, and mode capacity. Such a device would have applications in quantum networking and measurement-based quantum computing.

DOI
10.48550/arxiv.2409.12503

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Quantum memories could benefit many devices in quantum information processing. For a quantum to be useful in real-world applications, the quantum memory must have a high recall efficiency. Here we demonstrate an efficient (up to 80%) spin-storage quantum memory in Er:YSO, using the 4-level rephased amplified spontaneous emission protocol. We show non-classical correlations between the ASE and RASE fields produced by the quantum memory. Also, we demonstrate the storage of 70 temporal modes, with a write time of 150 us, and a storage time of 25 us. Finally, a clear pathway is presented to improve the efficiency, storage time, and mode capacity. Such a device would have applications in quantum networking and measurement-based quantum computing.
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We studied the recall efficiency as a function of optical depth of rephased amplified spontaneous emission (RASE), a protocol for generating entangled light. The experiments were performed on the 3 ⁣H4^{3}\! H_{4}3H4​ →\rightarrow→ 1 ⁣D2^{1}\! D_{2}1D2​ transition in the rare-earth doped crystal Pr3+^{3+}3+:Y2_{2}2​SiO5_{5}5​, using a four-level echo sequence between four hyperfine levels to rephase the emission. Rephased emission was observed for optical depths in the range of αLαLαL = 0.8 to 2.0 with a maximum rephasing efficiency of 14 % observed while incorporating spin storage. This efficiency is a significant improvement over the previously reported non-classical result but is well short of the predicted efficiency. We discuss the possible mechanisms limiting the protocol's performance, and suggest ways to overcome these limits.
In this paper we report the first demonstration of "rephased amplified spontaneous emission" (RASE) with photon-counting detection. This protocol provides an all-in-one photon-pair source and quantum-memory that has applications as a quantum repeater node. The RASE protocol is temporally multimode, and in this demonstration the photon echo was generated in a way that is spatially multimode and includes intermediate storage between two potentially long-lived spin states. A correlation between spontaneous emission and its photon echo was observed, using an ensemble of Pr(3+) ions doped into a Y2SiO5 crystal. Alterations that would allow for the measurement of nonclassical correlations are identified. These should generally apply for future experiments in rare-earth ion crystals, which are promising systems for implementing highly-multiplexed quantum repeater operations.
Abstract Photon echo is a fundamental tool for the manipulation of electromagnetic fields. Unavoidable spontaneous emission noise is generated in this process due to the strong rephasing pulse, which limits the achievable signal-to-noise ratio and represents a fundamental obstacle towards their applications in the quantum regime. Here we propose a noiseless photon-echo protocol based on a four-level atomic system. We implement this protocol in a Eu3+:Y2SiO5 crystal to serve as an optical quantum memory. A storage fidelity of 0.952 ± 0.018 is obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity achievable using the classical measure-and-prepare strategy. In this work, the demonstrated noiseless photon-echo quantum memory features spin-wave storage, easy operation and high storage fidelity, which should be easily extended to other physical systems.
Abstract Photon echo is a fundamental tool for the manipulation of electromagnetic fields. Unavoidable spontaneous emission noise is generated in this process due to the strong rephasing pulse, which limits the achievable signal-to-noise ratio and represents a fundamental obstacle towards their applications in the quantum regime. Here we propose a noiseless photon-echo protocol based on a four-level atomic system. We implement this protocol in a Eu3+:Y2SiO5 crystal to serve as an optical quantum memory. A storage fidelity of 0.952 ± 0.018 is obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity achievable using the classical measure-and-prepare strategy. In this work, the demonstrated noiseless photon-echo quantum memory features spin-wave storage, easy operation and high storage fidelity, which should be easily extended to other physical systems.
Here, we demonstrate generating and storing entanglement in a solid-state spin-wave quantum memory with on-demand readout using the process of rephased amplified spontaneous emission (RASE). Amplified spontaneous emission (ASE), resulting from an inverted ensemble of Pr^{3+} ions doped into a Y_{2}SiO_{5} crystal, generates entanglement between collective states of the praseodymium ensemble and the output light. The ensemble is then rephased using a four-level photon echo technique. Entanglement between the ASE and its echo is confirmed and the inseparability violation preserved when the RASE is stored as a spin wave for up to 5 μs. RASE is shown to be temporally multimode with almost perfect distinguishability between two temporal modes demonstrated. These results pave the way for the use of multimode solid-state quantum memories in scalable quantum networks.