Thermalization in quantum many-body systems typically unfolds over timescales governed by intrinsic relaxation mechanisms. Yet, its spatial aspect is less understood. We investigate this phenomenon in the nonequilibrium steady state (NESS) of a Bose-Hubbard chain subject to coherent driving and dissipation at its boundaries, a setup inspired by current designs in circuit quantum electrodynamics. The dynamical fingerprints of chaos in this NESS are probed using semiclassical out-of-time-order correlators within the truncated Wigner approximation. At intermediate drive strengths, we uncover a two-stage thermalization along the spatial dimension: phase coherence is rapidly lost near the drive, while amplitude relaxation occurs over much longer distances. This separation of scales gives rise to an extended hydrodynamic regime exhibiting anomalous temperature profiles, which we designate as a “prethermal” domain. At stronger drives, the system enters a nonthermal, non-chaotic finite-momentum condensate characterized by sub-Poissonian photon statistics and a spatially modulated phase profile, whose stability is undermined by quantum fluctuations. We explore the conditions underlying this protracted thermalization in space and argue that similar mechanisms are likely to emerge in a broad class of extended driven-dissipative systems. Thermalization in quantum many-body systems can unfold across space in surprising ways. The authors reveal nonequilibrium regimes in a driven-dissipative quantum chain, including a spatially emergent prethermal domain and a nonthermal condensate destabilized by quantum fluctuations, with broad implications for driven quantum platforms
Thermalization in quantum many-body systems typically unfolds over timescales governed by intrinsic relaxation mechanisms. Yet, its spatial aspect is less understood. We investigate this phenomenon in the nonequilibrium steady state (NESS) of a Bose-Hubbard chain subject to coherent driving and dissipation at its boundaries, a setup inspired by current designs in circuit quantum electrodynamics. The dynamical fingerprints of chaos in this NESS are probed using semiclassical out-of-time-order correlators within the truncated Wigner approximation. At intermediate drive strengths, we uncover a two-stage thermalization along the spatial dimension: phase coherence is rapidly lost near the drive, while amplitude relaxation occurs over much longer distances. This separation of scales gives rise to an extended hydrodynamic regime exhibiting anomalous temperature profiles, which we designate as a “prethermal” domain. At stronger drives, the system enters a nonthermal, non-chaotic finite-momentum condensate characterized by sub-Poissonian photon statistics and a spatially modulated phase profile, whose stability is undermined by quantum fluctuations. We explore the conditions underlying this protracted thermalization in space and argue that similar mechanisms are likely to emerge in a broad class of extended driven-dissipative systems. Thermalization in quantum many-body systems can unfold across space in surprising ways. The authors reveal nonequilibrium regimes in a driven-dissipative quantum chain, including a spatially emergent prethermal domain and a nonthermal condensate destabilized by quantum fluctuations, with broad implications for driven quantum platforms
We investigate the steady-state dynamical regimes of boundary-driven, dissipative bosonic chains subjected to n-photon drives. Using the truncated Wigner approximation, we explore how multiphoton drives shape the interplay between quantum fluctuations, nonlinear interactions, and dissipative processes in such quantum systems. We identify two main regimes: a chaotic hydrodynamic regime characterized by the restoration of a local U(1) symmetry, photon saturation due to Kerr nonlinearity, and spatial prethermalization effects and a nonchaotic resonant nonlinear wave (RNW) regime exhibiting sub-Poissonian photon statistics, persistent Zn symmetry, and quantum-driven phase decoherence. Our findings reveal the universal nature of the hydrodynamic regime and highlight the RNW regime's sensitivity to boundary driving conditions, suggesting novel routes for quantum state engineering in driven-dissipative quantum devices. These results are experimentally relevant for state-of-the-art circuit quantum electrodynamics platforms.
We investigate the non-equilibrium dynamics and steady-state properties of a driven-dissipative Bose-Hubbard chain using a self-consistent Gutzwiller mean-field (GMF) approach. By employing a robust Picard iteration scheme, we solve the non-linear master equation for the non-equilibrium steady state (NESS) in the presence of strong Kerr nonlinearity. We identify two distinct dynamical regimes governed by the interplay between coherent drive, dissipation, and interaction: a regular quasilinear regime and a chaotic regime. Linear stability analysis reveals that the transition to the chaotic regime is triggered by parametric instabilities arising from the drive-induced coherence. Furthermore, we characterize the onset of quantum chaos by calculating the out-of-time-order correlator (OTOC). Our results show that in the strong coupling regime, the OTOC exhibits rapid exponential growth and saturation, providing a clear signature of information scrambling in this open quantum system. The proposed numerical framework offers an efficient pathway to explore many-body correlations in larger photonic lattices.
We define quantum chaos and integrability in open quantum many-body systems as a dynamical property of single stochastic realizations, referred to as quantum trajectories. This definition relies on the predictions of random matrix theory applied to the subset of the Liouvillian eigenspectrum involved in each quantum trajectory. Our approach, which we name (SSQT), enables a natural distinction between transient and steady-state quantum chaos as general phenomena in open setups. We test the generality and reliability of the SSQT criterion on several dissipative systems, further showing that an open system with a chaotic structure can evolve towards either a chaotic or integrable steady state. We apply our theoretical framework to two driven-dissipative bosonic systems. First, we study the driven-dissipative Bose-Hubbard model, a paradigmatic example of a quantum simulator, clarifying the interplay of integrability, transient, and steady-state chaos across its phase diagram. Our analysis shows the existence of an emergent dissipative quantum chaotic phase, whereas the classical and semiclassical limits display an integrable behavior. In this regime, chaos arises from the quantum and classical fluctuations associated with the dissipation mechanisms. Second, we investigate dissipative quantum chaos in the dispersive readout of a transmon qubit: a measurement technique ubiquitous in superconducting-based quantum hardware. Through the SSQT, we distinguish several regimes where the performance of the measurement instrument can be connected to the integrable or chaotic nature of the underlying driven-dissipative bosonic system. Our work offers a general understanding of the integrable and chaotic dynamics of open quantum systems and paves the way for the investigation of dissipative quantum chaos and its consequences on state-of-the-art noisy intermediate-scale quantum devices.
This work investigates the emergent thermalization regimes in a chaotic Tavis-Cummings (TC) model and their implications in quantum spectroscopy. While the TC model is a cornerstone of cavity quantum electrodynamics, traditional treatments often overlook many-body effects that arise in the thermodynamic limit. We utilize the Eigenstate Thermalization Hypothesis to demonstrate that a non-integrable excitonic Hamiltonian within the material manifold drives local thermalization. By tuning the polariton splitting g, we observe two dynamical regimes: a thermalizing regime at low interactions driven by quantum chaos and ergodicity, and a non-thermalizing regime at high interactions where strong coupling suppresses ergodicity. We further show that these regimes have direct implications on output photon statistics, specifically influencing the correlation times τc of the cavity population and the second-order correlation function g(2)(t+τ). We propose that entangled-biphoton spectroscopy serves as an ideal experimental platform to probe these effects and to allow the characterization of the underlying many-body exciton-coupling disorder σ through coincidence measurements of the output. Taken together, these results exploit a naturally occurring many-body phenomenon to bridge theoretical predictions with experimental observables.
Modern experimental platforms such as superconducting circuit arrays call for the exploration of bosonic tight-binding models in unconventional situations with no counterpart in real materials. Here we investigate one such situation in which excitations are driven and damped by pairs, leading to pattern formation and exotic bosonic states emerging from a nonequilibrium quantum many-body system. Focusing on a two-dimensional driven-dissipative Bose-Hubbard model, we find that its steady states are characterized by the condensation of bosons around momenta lying on a "Bose surface," a bosonic analog of the Fermi surface in solid-state systems. The interplay between instabilities generated by the driving, the nonlinear dissipative mode coupling, and the underlying lattice effect allows the system to equilibrate into an exotic superfluid state of bosons condensed on a closed ring in momentum space instead of discrete points. Such an unconventional state with a spatially uniform density distribution goes beyond the traditional scope of pattern formation and thus has no counterpart in the classical literature. In addition, it is a state connected to several open problems in modern condensed-matter physics. Here we provide the means to stabilize it, opening the way to its experimental study. Moreover, we also provide a concrete experimental implementation of our model in currently available superconducting circuit arrays. We also investigate the relaxation spectrum around the condensate, which shows a characteristic purely diffusive behavior.
Collective quantum phenomena are fascinating, as they repeatedly challenge our comprehension of nature and its underlying mechanisms. The qualification ``quantum'' can be attributed to a generic many-body system whenever the interference effects related to the underlying wave nature of its elementary constituents can not be neglected anymore, and a naive classical description in terms of interacting billiard balls fails to catch its most essential features. This interference phenomenon called ``quantum degeneracy'' which occurs at weak temperatures, leads to spectacular collective behaviours such as the celebrated Bose-Einstein Condensation (BEC) phase transition, where a macroscopic fraction of a bosonic system of particles collapses below a critical temperature T_c on a single-particle state. Quantum coherence, when combined with inter-particle interactions, gives rise to highly non-classical frictionless hydrodynamic behaviours such as superfluidity (SF) and superconductivity (SC). \nEven more exotic quantum phases emerge in presence of important interactions as matter reaches a ``strongly correlated regime'' dominated by quantum fluctuations, where each particle is able to affect significantly the surrounding fluid: characteristic examples are the so-called Mott-Insulator (MI) quantum phase where particles are localized on a lattice due to a strong interaction-induced blockade, along with the Tonks-Girardeau (TG) gas where impenetrable bosons in one-dimension acquire effective fermionic statistics up to a unitary transformation, and the Fractional Quantum Hall (FQH) effect which occurs in presence of a gauge field, and features a special type of elementary excitation possessing a fractional charge and obeying to fractional statistics called `anyon'. \nThese quantum many-body effects were explored in a first place in systems well isolated from the external environment such as ultra-cold atomic gases or electrons in solid-state systems, within a physical context well described by ``equilibrium statistical mechanics''. Yet, over the last two decades a broad community has started investigating the possibility of stabilizing interacting quantum phases in novel nonlinear quantum optics architectures, where interacting photons have replaced their atomic and electronic counterpart. Thanks to their high level of controllability and flexibility, and the possibility of reaching the quantum degeneracy regime at exceptionally high temperatures, these platforms appear as extremely promising candidates for the ``quantum simulation'' of the most exotic many-body quantum problems: while the precursors experiments in semiconductor exciton-polariton already allow to reach the Bose-Einstein Condensation and superfluid regimes, novel platforms such as superconducting circuits, coupled cavity arrays or photons coupled to Rydberg EIT (Electromagnetically induced Transparency) atoms have entered the so-called `photon blockade' where photons behave as impenetrable particles, and open a encouraging pathway toward the future generation of strongly correlated phases with light. \nA specificity of quantum optics devices is their intrinsic ``non-equilibrium'' nature: the interplay between the practically unavoidable radiative and non-radiative losses and the external drive needed to replenish the photon gas leads the many-body system toward a steady-state presenting important non-thermal features. One one hand, an overwhelmingly large quantity of novel quantum phenomena is expected in the non-equilibrium framework, as breaking the thermal equilibrium condition releases severe constraints on the state of a quantum system and on the nature of its surrounding environment. On the other hand, we do not benefit yet of an understanding of non-equilibrium statistical mechanics comparable with its well-established equilibrium counterpart, which relies on strong historical foundations. Understanding how to tame (and possibly exploit) non-equilibrium effects in order to stabilize interesting quantum phases in a controlled manner often reveals a hard challenge. \nIn that prospect, an important conceptual issue in the non-equilibrium physics of strongly interacting photons regards the possibility of stabilizing ``incompressible quantum phases'' such as the Mott-Insulator or Fractional Quantum Hall states, and more generally to stabilize the ground-state of a given particle-number conserving Hamiltonian, in a physical context where dissipative losses can not be neglected. While being able to quantum simulate those emblematic strongly correlated quantum phases in this novel experimental context would strongly benefit to the quantum optics community, gaining such a kind of flexibility would also contribute to fill an important bridge between the equilibrium and the non-equilibrium statistical physics of open quantum systems, allowing to access in a controlled manner a whole new phenomenology at the interface between the two theories. \nIn this thesis I address those questions, which I reformulate in the following manner: \n \n-What are the conditions for the emergence of analogue equilibrium properties in open quantum systems in contact with a non-thermal environment ? \n \n-In particular, is it possible to stabilize strongly correlated quantum phases with a perfectly defined particle number in driven-dissipative photonic platforms, in spite of environment-induced losses and heating effects ? \n \nThe structure of the thesis is the following. \n \n \n[Chapter 1.] We give an overview of the physics of many-body photonic systems. As a first step we address the weakly interacting regime in the physical context of exciton-polaritons: after describing the microscopic aspects of typical experiments, we move to the discussion of non-equilibrium Bose-Einstein Condensation and the various mechanisms related to the emergence of thermal signatures at steady-state. The second part of this Chapter is dedicated to strongly interacting fluids. After drawing a quick overview of several experimental platforms presenting a good potential for the study of such physics in a near future, we discuss the relative performance of several schemes proposed in order to replenish the photonic population \n \n[Chapter 2.] We investigate the potential of a non-Markovian pump scheme with a narrow bandpass (Lorentzian shaped) emission spectrum for the generation of strongly correlated states of light in a Bose-Hubbard lattice. Our proposal can be implemented by mean of embedded inverted two-level emitters with a strong incoherent pumping toward the excited state. Our study confirms in a single cavity the possibility of stabilizing photonic Fock states in a single configuration, and strongly localized n=1 Mott-Insulator states in a lattice with n=1 density. We show that a relatively moderate hopping is responsible for a depletion of the Mott-state, which then moves toward a delocalized state reminiscent of the superfluid regime. Finally, we proceed to a mean-field analysis of the phase diagram, and unveil a Mott-to-Superfluid transition characterized by a spontaneous breaking of the U(1) symmetry and incommensurate density. The results of this Chapter are based on the following publications: \n- J. Lebreuilly, M. Wouters and I. Carusotto, ``Towards strongly correlated photons in arrays of dissipative nonlinear cavities under a frequency-dependent incoherent pumping'', C. R. Phys., 17(8), 836, 2016. \n- A. Biella, F. Storme, J. Lebreuilly, D. Rossini, R. Fazio, I. Carusotto and C. Ciuti, ``Phase diagram of incoherently driven strongly correlated photonic lattice'', Phys. Rev. A, 96, 023839, 2017. \n \n[Chapter 3.] In view of improving the performance of the scheme introduced in last chapter, and reproducing in particular the equilibrium zero temperature phenomenology in driven-dissipative photonic lattices, we develop a fully novel scheme based on the use of non-Markovian reservoirs with tailored broadband spectra which allows to mimick the effect of tunable chemical potential. Our proposal can be implemented by mean of a small number of emitters and absorbers and is accessible to current technologies. \n \nWe first analyse the case of a frequency-dependent emission with a square spectrum and confirm the possibility of stabilizing Mott insulator states with arbitrary integer density. Unlike the previous proposal the Mott state is robust against both losses and tunneling. A sharp transition toward a delocalized superfluid-like state can be induced by strong values of the tunneling or a change in the effective chemical potential. While an overall good agreement is found with the T=0 predictions, our analysis highlights small deviations from the equilibrium case in some parts of the parameters space, which are characterized by a non-vanishing entropy and the kinetic generation of doublon excitations. We finally consider an improved scheme involving additional frequency-dependent losses, and show in that case that the Hamiltonian ground-state is fully recovered for any choice of parameters. Our proposal, whose functionality relies on generic energy relaxation mechanisms and is not restricted to the Bose-Hubbard model, appears as a promising quantum simulator of zero temperature physics in photonic devices. The results of this Chapter are based on the following publication: \n- J. Lebreuilly, A. Biella, F. Storme, D. Rossini, R. Fazio, C. Ciuti and I. Carusotto, ``Stabilizing strongly correlated photon fluids with non-Markovian reservoirs'', Phys. Rev. A 96, 033828 (2017). \n \n[Chapter 4.] We adopt a broader perspective, and analyse the conditions for the emergence of analogous thermal properties in driven-dissipative quantum systems. We show that the impact of an equilibrated environment can be mimicked by several non-Markovian and non-equilibrated reservoirs. Chapter 2 already f