The dressed atom approach provides a tool to investigate the dynamics of an atom-laser system by fully retaining the quantum nature of the coherent mode. In its standard derivation, the internal atom-laser evolution is described within the rotating-wave approximation, which determines a doublet structure of the spectrum and the peculiar fluorescence triplet in the steady state. However, the rotating wave approximation may fail to apply to atomic systems subject to femtosecond light pulses, light-matter systems in the strong-coupling regime or sustaining permanent dipole moments. This work aims to demonstrate how the general features of the steady-state radiative cascade are affected by the interaction of the dressed atom with propagating radiation modes. Rather than focusing on a specific model, we analyze how these features depend on the parameters characterizing the dressed eigenstates in arbitrary atom-laser dynamics, given that a set of general hypotheses is satisfied. Our findings clarify the general conditions in which a description of the radiative cascade in terms of transition between dressed states is self-consistent. We provide a guideline to determine the properties of photon emission for any atom-laser interaction model, which can be particularly relevant when the model should be tailored to enhance a specific line. We apply the general results to the case in which a permanent dipole moment is a source of low-energy emission, whose frequency is of the order of the Rabi coupling.
The dressed atom approach provides a tool to investigate the dynamics of an atom-laser system by fully retaining the quantum nature of the coherent mode. In its standard derivation, the internal atom-laser evolution is described within the rotating-wave approximation, which determines a doublet structure of the spectrum and the peculiar fluorescence triplet in the steady state. However, the rotating wave approximation may fail to apply to atomic systems subject to femtosecond light pulses, light-matter systems in the strong-coupling regime or sustaining permanent dipole moments. This work aims to demonstrate how the general features of the steady-state radiative cascade are affected by the interaction of the dressed atom with propagating radiation modes. Rather than focusing on a specific model, we analyze how these features depend on the parameters characterizing the dressed eigenstates in arbitrary atom-laser dynamics, given that a set of general hypotheses is satisfied. Our findings clarify the general conditions in which a description of the radiative cascade in terms of transition between dressed states is self-consistent. We provide a guideline to determine the properties of photon emission for any atom-laser interaction model, which can be particularly relevant when the model should be tailored to enhance a specific line. We apply the general results to the case in which a permanent dipole moment is a source of low-energy emission, whose frequency is of the order of the Rabi coupling.
The Rabi Hamiltonian, describing the interaction between a two-level atomic system and a single-cavity mode of the electromagnetic field, is one of the fundamental models in quantum optics. The model becomes exactly solvable by considering an atom without permanent dipole moments, whose excitation energy is quasiresonant with the cavity photon energy, and by neglecting the nonresonant (counter-rotating) terms. In this case, after including the decay of either the atom or the cavity mode to a continuum, one can derive the well-known phenomenology of quasiresonant transitions, including the fluorescence triplets. In this work we consider the most general Rabi model, incorporating the effects of permanent atomic electric dipole moments. Based on a perturbative analysis, we compare the intensities of emission lines induced by rotating terms, counter-rotating terms, and parity-symmetry-breaking terms in order to identify the parameter regimes in which these different contributions play a significant role. The analysis reveals that the emission strength related to the existence of permanent dipoles may surpass the one due to the counter-rotating interaction terms but is usually much weaker than the emission due to the main, resonant coupling. This ratio can be modified in systems with a reduced dimensionality or by engineering the energy spectral density of the continuum.
A dressed-state perturbation theory beyond the rotating wave approximation(RWA) is presented to investigate the interaction between a two-level electronic transition of polar molecules and a quantized cavity field. Analytical expressions can be explicitly derived for both the ground- and excited-state-energy spectrums and wave functions of the system, where the contribution of permanent dipole moments(PDM) and the counter-rotating wave term(CRT) can be shown separately.The validity of these explicit results is discussed by comparison with the direct numerical simulation. Compared to the CRT coupling, PDM results in the coupling of more dressed states and the energy shift is proportional to the square of the normalized permanent dipole difference, and a greater Bloch–Siegert shift can be produced in the giant dipole molecule cavity QED. In addition, our method can also be extended to the solution of the two-level atom Rabi model Hamiltonian beyond the RWA.更多还原
In this chapter,we shall analyze the particular case of an atom interacting with a laser pulse whose duration is sufficiently long, so that the evolution of the atom in the laser field is adiabatic. When this condition is fulfilled, the atom can be considered to interact with a monochromatic laser field. As a consequence, the Hamiltonian of the system is periodic in time, and the Floquet theory [1] can be used to solve the time-dependent Schrödinger equation (TDSE) non-perturbatively. We begin in Section 4.1 by considering the Hermitian Floquet theory. We first derive the Floquet theorem for a monochromatic, spatially homogeneous laser field and show that the solutions of the TDSE correspond to dressed states having real quasi-energies , which can be obtained by solving an infinite system of time-independent coupled equations. We then generalize the Floquet theory to multicolor laser fields and to “non-dipole” laser fields which are not spatially homogeneous. In Section 4.2, the Floquet theory is applied to study the dynamics of a model atom having M discrete levels interacting with a monochromatic laser field. In this case, the coupling between the bound and continuum atomic states is neglected.We analyze the relationship between the Floquet theory and the rotating wave approximation, and examine the perturbative limit of the Floquet theory. We also consider the population transfer between Floquet dressed states.
We study the dynamics of a system consisting of a two-level atom and a quantum oscillator coupled by the vacuum radiation field. The oscillator and the atom are assumed to have the same resonance frequency. In contrast to the two-atom or two-oscillator case, the atom-oscillator system leads to an unclosed hierarchy of equations for the operators that determine the radiation pattern emitted by the atom-oscillator system. Instead of using the operator equations, we formulate the problem in terms of density-matrix equations which can be solved once the initial conditions are specified. As an example, we looked at the radiation pattern, the decay dynamics, and the spectrum for an initial condition in which the oscillator is in its n=1 state and the atom is in its excited state. Dressed states (dressed by the static interaction between the atom and oscillator) prove to be especially useful for interpreting the results and comparing them with the two-atom and two-oscillator systems. All calculations are carried out using the resonance or rotating-wave approximation. The relationship of our work to damped Jaynes-Cummings models is noted.
Recent developments on intense laser sources is opening a new field of optical sciences. An intense coherent light beam strongly interacting with the matter causes a coherent motion of a particle, forming a strongly dressed excited particle. A photon emission from this dressed excited particle is a strong nonlinear process causing high-harmonic generation (HHG), where the perturbation analysis is broken down. In this work, we study a coherent photon emission from a strongly dressed excited atom in terms of complex spectral analysis in the extended Floquet-Hilbert-space. We have obtained the eigenstates of the total Hamiltonian with use of Feshbach-Brilloiun-Wigner projection method. In this extended space, the eigenstates of the total Hamiltonian consisting of the radiation field and the atom system have complex eigenvalues whose imaginary part represents the decay rate. Time evolution of the system is represented by the complex eigenvector expansion so that the correlation dynamics between the photon and the atom is fully taken into account. The HHG is interpreted as the irreversible spontaneous photon emission due to the resonance singularity in terms of the multiple Floquet states that are generated by periodic external field. We have found that the interference between the emitted photons over the different Floquet states causes spatial pulse emission correlated with the decay process of the excited atom.
Recalling that the rotating wave approximation (RWA) is only valid in the weak coupling regimes, the purpose of this paper is to study the Hamiltonian dynamics describing the full quantum mechanical approach of the interaction between various configurations of three-level atoms Lambda, V and ladder distinctly with a two-mode radiation field, while the RWA is not considered; the counter-rotating terms (CRTs) are taken into account. Generally, the presence of CRTs in the Hamiltonian prevents one to achieve an analytical solution. Moreover, as we will show in the present work, using the perturbation theory, analytical solvable Hamiltonians can be successfully obtained. According to our calculations, the contribution of CRTs within the ordinary Hamiltonian is equivalent to the replacement of the constant detuning with a specific intensity dependent detuning in the first order, and the constant atom field coupling with a particular intensity dependent (f deformed) coupling in the second order of the associated perturbation parameter. Moreover, noticing that according to the initial expression of the Hamiltonian, each mode of the field interacts only with a specific pair of the allowed transitions of each type of the three-level atom, it is surprisingly observed that via applying the mentioned approach, the obtained intensity dependent coupling functions depend on both modes of the field, f(na,nb). In this way, it is seen that the CRTs are removed with the price of arriving at some intermixed intensity dependent atom field coupling functions of the two modes of the field. In this way, the obtained final Hamiltonians are analytically solvable. At last, by determining the time evolution of the atom field wave function, we study the effects of CRTs on a few nonclassical properties of the state of the system, including the atomic population inversion and photon statistics.