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arXiv:2409.09139 · Physical Review Letters

Conservation of Angular Momentum on a Single-Photon Level

Lea Kopf, Rafael F. Barros, Shashi Prabhakar, Enno Giese, Robert Fickler

Published May 20, 2025• 13 citations
arXivHTMLPDF

Abstract

Identifying conservation laws is central to every subfield of physics, as they illuminate the underlying symmetries and fundamental principles. A prime example can be found in quantum optics: the conservation of orbital angular momentum (OAM) during spontaneous parametric down-conversion (SPDC) enables the generation of a photon pair with entangled OAM. In this Letter, we report on the observation of OAM conservation in SPDC pumped on the single-photon level by a preceding SPDC process. We implement this cascaded down-conversion scheme in free space, without waveguide confinement, and thereby set the stage for experiments on the direct generation of multiphoton high-dimensional entanglement using all degrees of freedom of light.

DOI
10.1103/physrevlett.134.203601

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Conservation laws are at the heart of our natural scientific understanding, as they dictate why certain phenomena do or do not exist in nature. In the realm of nonlinear optics — where light-matter interactions enable the generation of photon pairs — these principles are also essential. In the common interpretation of spontaneous parametric down-conversion (SPDC), the conservation of momenta is attributed to the transfer of the well-defined linear or orbital angular momenta (OAM) of the single pump photon to the generated photon pair [1], [2]. However, due to the low conversion efficiencies, this conservation rule has only been tested with a strong coherent laser pumping the process. Here, we show for the first time that the OAM of a single pump photon is indeed conserved and that an OAM quanta of up to 2 is transferred to the generated photon pair.

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Identifying conservation laws is central to every subfield of physics, as they illuminate the underlying symmetries and fundamental principles. A prime example can be found in quantum optics: the conservation of orbital angular momentum (OAM) during spontaneous parametric down-conversion (SPDC) enables the generation of a photon pair with entangled OAM. In this Letter, we report on the observation of OAM conservation in SPDC pumped on the single-photon level by a preceding SPDC process. We implement this cascaded down-conversion scheme in free space, without waveguide confinement, and thereby set the stage for experiments on the direct generation of multiphoton high-dimensional entanglement using all degrees of freedom of light.
Conservation laws are at the heart of our natural scientific understanding, as they dictate why certain phenomena do or do not exist in nature. In the realm of nonlinear optics — where light-matter interactions enable the generation of photon pairs — these principles are also essential. In the common interpretation of spontaneous parametric down-conversion (SPDC), the conservation of momenta is attributed to the transfer of the well-defined linear or orbital angular momenta (OAM) of the single pump photon to the generated photon pair [1], [2]. However, due to the low conversion efficiencies, this conservation rule has only been tested with a strong coherent laser pumping the process. Here, we show for the first time that the OAM of a single pump photon is indeed conserved and that an OAM quanta of up to 2 is transferred to the generated photon pair.
Orbital angular momentum (OAM)-entangled states produced by spontaneous parametric down-conversion (SPDC) are considered ideal for realizing high-dimensional entangled states, which have several advantages for quantum technologies. However, the limited sensitivity of current two-photon OAM detectors is a major roadblock not only for realizing such technologies but also for resolving foundational questions, such as OAM conservation in SPDC. The current theoretical understanding is that OAM is not conserved in Type-II SPDC but is conserved in Type-I. Experimentally, although non-conservation in TypeII has not been demonstrated, conservation in Type-I has been reported frequently and has become an underlying assumption for techniques generating high-dimensional OAM entangled states. In this work, we experimentally demonstrate a high-sensitivity two-photon OAM detector, using which, contrary to the current understanding, we report non-conservation of OAM in Type-I SPDC. We attribute this to a spatial walk-off effect and prove it using a framework free of standard phase-matching approximations.
The generation of paired photons entangled in the spatial degree of freedom, i.e., in orbital angular momentum, offers a convenient physical resource to investigate the nature of entanglement in a multidimensional Hilbert space with controllable dimensionality. The two main physical processes that generate pairs of photons which show correlations in orbital angular momentum are (a) spontaneous parametric down-conversion (SPDC), and (b) Raman transitions induced in atomic ensembles. One question naturally arises: what kinds of correlations exist between the orbital angular momentum of the generated photons? The answer might be different if we consider the whole quantum state of the generated photons, i.e., all possible directions where the pairs of photons can be emitted, or if we consider only a small section of the full set of directions.
States of light that are simultaneously eigenstates of orbital, intrinsic, and total angular momentum are found and eigenstates describing pairs of photons from spontaneous parametric down-conversion reveal classes of photon conversion with angular momentum conservation and cases where the initial angular momentum from the pump laser beam is shared between the converted photons and the generating medium. These angular momentum conservation laws open up a wide range of applications to be explored.
The bandwidth of any communication system, classical or quantum, is limited by the number of orthogonal states in which the information can be encoded. Quantum key distribution systems available commercially rely on the two-dimensional polarisation state of photons. Quantum computation has also been largely designed on the basis of qubits. However, a photon is endowed with other degrees of freedom, such as orbital angular momentum (OAM). OAM is an attractive basis to be used for quantum information because it is discrete and theoretically infinite-dimensional. This promises a higher information capacity per photon which can lead to more complex quantum computation protocols and more security and robustness for quantum cryptography. Entanglement of OAM naturally arises from spontaneous parametric down-conversion (SPDC). However, any practical experiment utilising the innately high-dimensional entanglement of the orbital angular momentum (OAM) state space of photons is subject to the modal capacity of the detection system. Only a finite subset of this space is accessible experimentally. Given such a constraint, we show that the number of measured, entangled OAM modes in photon pairs generated by SPDC can be increased by tuning the phase-matching conditions in the SPDC process. We achieve this by tuning the orientation angle of the nonlinear crystal generating the entangled photons.
Stimulated parametric down-conversion (StimPDC) produces an idler beam that exhibits a phase conjugate of the spatial structure of the classical seed beam. Extending this effect to the single-photon regime can, in principle, enable the control of the orbital angular momentum of single photons. However, its experimental implementation remains challenging due to the lower photon flux of realistic single-photon sources compared to a classical pump beam, which causes the StimPDC process to occur less frequently compared to its spontaneous counterpart. To overcome this, we propose a cascaded parametric down-conversion scheme, in which the signal photon from a spontaneously down-converted pair seeds the StimPDC process, while the idler photon heralds the seed's presence. This configuration uses coincidence detection to effectively post-select for stimulated events among the background of spontaneous contributions. We show that phase conjugation at the single-photon level manifests as a bias towards equal orbital angular momentum between the heralding idler and the stimulated idler. Our results offer a practical route to manipulate single-photon correlations in the orbital angular momentum degree of freedom and could have implications for applications such as free-space quantum communication and quantum-enhanced sensing.