The ability to slow down light at the single-photon level has applications in quantum information processing and other quantum technologies. We demonstrate two methods, both using just a single artificial atom, enabling dynamic control over microwave light velocities in waveguide quantum electrodynamics (QED). Our methods are based on two distinct mechanisms harnessing the balance between radiative decay and nonradiative decoherence rates of a superconducting artificial atom in front of a mirror. In the first method, we tune the radiative decay of the atom using interference effects due to the mirror; in the second method, we pump the atom to effectively control its nonradiative decoherence. When the half of the radiative decay rate exceeds the nonradiative decoherence rate, we observe positive group delay; conversely, dominance of the nonradiative decoherence results in negative group delay. Our results advance signal-processing capabilities in waveguide QED.
The ability to slow down light at the single-photon level has applications in quantum information processing and other quantum technologies. We demonstrate two methods, both using just a single artificial atom, enabling dynamic control over microwave light velocities in waveguide quantum electrodynamics (QED). Our methods are based on two distinct mechanisms harnessing the balance between radiative decay and nonradiative decoherence rates of a superconducting artificial atom in front of a mirror. In the first method, we tune the radiative decay of the atom using interference effects due to the mirror; in the second method, we pump the atom to effectively control its nonradiative decoherence. When the half of the radiative decay rate exceeds the nonradiative decoherence rate, we observe positive group delay; conversely, dominance of the nonradiative decoherence results in negative group delay. Our results advance signal-processing capabilities in waveguide QED.
The interaction between superconducting qubits and one-dimensional microwave transmission lines has been studied experimentally and theoretically in the past two decades. In this work, we investigate the spontaneous emission of an initially excited artificial atom which is capacitively coupled to a semi-infinite transmission line, shorted at one end. This configuration can be viewed as an atom in front of a mirror. The distance between the atom and the mirror introduces a time delay in the system, which we take into account fully. When the delay time equals an integer number of atom oscillation periods, the atom converges into a dark state after an initial decay period. The dark state is an effect of destructive interference between the reflected part of the field and the part directly emitted by the atom. Based on circuit quantization, we derive linearized equations of motion for the system and use these for a semiclassical analysis of the transient dynamics. We also make a rigorous connection to the quantum optics system-reservoir approach and compare these two methods to describe the dynamics. We find that both approaches are equivalent for transmission lines with a low characteristic impedance, while they differ when this impedance is higher than the typical impedance of the superconducting artificial atom.
We study the collective effects that emerge in waveguide quantum electrodynamics where several (artificial) atoms are coupled to a one-dimensional superconducting transmission line. Since single microwave photons can travel without loss for a long distance along the line, real and virtual photons emitted by one atom can be reabsorbed or scattered by a second atom. Depending on the distance between the atoms, this collective effect can lead to super- and subradiance or to a coherent exchange-type interaction between the atoms. Changing the artificial atoms transition frequencies, something which can be easily done with superconducting qubits (two levels artificial atoms), is equivalent to changing the atom-atom separation and thereby opens the possibility to study the characteristics of these collective effects. To study this waveguide quantum electrodynamics system, we extend previous work and present an effective master equation valid for an ensemble of inhomogeneous atoms driven by a coherent state. Using input-output theory, we compute analytically and numerically the elastic and inelastic scattering and show how these quantities reveal information about collective effects. These theoretical results are compatible with recent experimental results using transmon qubits coupled to a superconducting one-dimensional transmission line [van Loo et al. (unpublished)].
Waveguide quantum electrodynamics studies photon-mediated interactions of quantum emitters in a one-dimensional radiation channel. Although signatures of such interactions have been observed previously in a variety of physical systems, observation of coherent cooperative dynamics has been obscured by radiative decay of atoms into the waveguide. Employing transmon qubits as artificial atoms coupled to a microwave coplanar waveguide, here we observe dynamical oscillations in an open system where a designated probe qubit interacts with an entangled dark state of an array of qubits which effectively traps radiation as an atomic cavity. The qubit-cavity system is shown to achieve a large cooperativity of C=172 due to collective enhancement of photon-mediated interactions, entering the strong coupling regime. The quantum coherence of the dark state cavity is also explored through its nonlinear response at the single-excitation level. With realistic refinements, this system is suitable for studying the many-body dynamics of large (N>10) quantum spin chains, synthesizing highly non-classical radiation fields on demand, and implementing universal quantum logic operations with high fidelity on information encoded within decoherence-free subspaces.
Experiments utilizing quantum optics have progressed rapidly in last few decades, particularly in the context of quantum computation, simulation, and communication. Early work in this field focused on implementations of cavity quantum electrodynamics (QED), where atoms, either natural or artificial, are strongly coupled to the confined photonic modes of cavities. However, in recent years, achieving strong coupling between atoms and itinerant photons has also gained significant interest for its applications in quantum networking. To this end, many atomic platforms are attempting to realize the waveguide QED architecture: atoms that interact with the continua of propagating photonic modes within a waveguide. In this thesis, we realize the strong-coupling regime of a waveguide QED architecture by coupling superconducting artificial atoms, typically operated as qubits, to one-dimensional transmission lines. We first demonstrate that superconducting qubits in a waveguide QED system can be used as high-quality quantum emitters. We then leverage the quantum interference between the simultaneous emission from multiple qubits in order to generate non-classical, spatially entangled, and directional itinerant microwave photons. These types of photons are particularly useful for remote entanglement and quantum communication protocols. Finally, we demonstrate that superconducting qubits can be engineered to enter novel regimes of light-matter interactions that are difficult, or even impossible, to achieve in other atomic platforms. In particular, we realize the giant-atom regime of waveguide QED, where the atom can no longer be treated as a point-like object. We use our giant atoms to implement tunable atom-waveguide couplings, as well as decoherence-free waveguide-mediated interactions between multiple atoms.
Waveguide circuit quantum electrodynamics (waveguide circuit QED) studies light-matter interaction with superconducting circuits in one dimension. In circuit QED, natural atoms are replaced by superconducting qubits consisting of a non-linear Josephson junction, resulting in an anharmonic energy spectrum just like real atoms. With superconducting qubits, it is possible to study quantum optical phenomena and reach new regimes hard to achieve with real atoms due to weak coupling to the electromagnetic field. The reduction to one dimension in waveguide QED increases the electromagnetic field's directionality, which results in reduced losses. In this thesis, we first introduce circuit quantisation, giving the basis for the next part, where we investigate a transmon, a charge-insensitive artificial atom, coupled to a semi-infinite transmission line. An atom coupled to a semi-infinite waveguide is referred to as an atom in front of a mirror and is the subject of all appended papers. We proceed by summarising Paper I and III's main results: in Paper I, we investigate the spontaneous emission of a transmon coupled to a semi-infinite transmission line, where we take time-delay effects into account. We find that the system dynamics strongly depend on the coupling strength to the transmission line and the atom's position with respect to the electromagnetic field, leading to the Purcell effect or the convergence to a dark state with finite excitation probability. In the high-impedance regime, which we investigate in Paper III, the properties of the transmon coupled to the high-impedance transmission line change drastically. It becomes highly reflective and creates its own cavity with the mirror, resulting in the emergence of cavity modes and vacuum Rabi oscillations in the spontaneous emission dynamics. In the next chapter of the thesis, we demonstrate how to quantise an electromagnetic field and derive a light-matter interaction Hamiltonian within dipole approximation. We then give an introduction to open quantum systems and derive the quantum-optical master equation in Lindblad form. Furthermore, we introduce the dressed state picture, where the interaction of light and matter is so strong that the individual energy levels of light and matter are no longer separable. Both the quantum optical master equation and the dressed state picture are relevant in Paper II and IV. In Paper II, an experimental collaboration, we perform several experiments to characterise and discriminate different decay rates of a superconducting qubit coupled to the end of a transmission line. One experiment measured the atomic fluorescence spectral density, which shows an asymmetry for off-resonant driving, resulting from pure dephasing: an effect that we explain in more detail in this thesis and Paper II. In Paper IV, we theoretically investigate amplification mechanisms realised by different set-ups of an atom coupled to a semi-infinite waveguide. In the considered systems, the amplification of a probe field happens either due to population inversion between the pure states or dressed states or multi-photon processes. We find that compared to an open waveguide, we can achieve a higher gain in the amplification with a semi-infinite waveguide.
Waveguide quantum electrodynamics studies photon-mediated interactions of quantum emitters in a one-dimensional radiation channel. Although signatures of such interactions have been observed previously in a variety of physical systems, observation of coherent cooperative dynamics has been obscured by radiative decay of atoms into the waveguide. Employing transmon qubits as artificial atoms coupled to a microwave coplanar waveguide, here we observe dynamical oscillations in an open system where a designated probe qubit interacts with an entangled dark state of an array of qubits which effectively traps radiation as an atomic cavity. The qubit-cavity system is shown to achieve a large cooperativity of C=172 due to collective enhancement of photon-mediated interactions, entering the strong coupling regime. The quantum coherence of the dark state cavity is also explored through its nonlinear response at the single-excitation level. With realistic refinements, this system is suitable for studying the many-body dynamics of large (N>10) quantum spin chains, synthesizing highly non-classical radiation fields on demand, and implementing universal quantum logic operations with high fidelity on information encoded within decoherence-free subspaces.