Full coherent control and generation of nonclassical superpositions of the quantum harmonic oscillator are not only of fundamental interest but are crucial for applications in quantum simulations, quantum-enhanced metrology, and continuous-variable quantum computation. Here, we create arbitrary superpositions of nonclassical and non-Gaussian states of a quantum harmonic oscillator using the motion of a trapped ion coupled to its internal spin states. We interleave spin-dependent nonlinear interactions with midcircuit spin measurements that herald the probabilistic preparation of superpositions of squeezed, trisqueezed, and quadsqueezed states, which have not previously been experimentally demonstrated. We achieve independent control over the complex-valued squeezing parameter and the probability amplitude of each constituent, as well as their spatial separation. We directly observe the nonclassical nature of these states in the form of Wigner negativity following a full-state reconstruction. Our methods apply to any system where a quantum harmonic oscillator is coupled to a spin.
Full coherent control and generation of nonclassical superpositions of the quantum harmonic oscillator are not only of fundamental interest but are crucial for applications in quantum simulations, quantum-enhanced metrology, and continuous-variable quantum computation. Here, we create arbitrary superpositions of nonclassical and non-Gaussian states of a quantum harmonic oscillator using the motion of a trapped ion coupled to its internal spin states. We interleave spin-dependent nonlinear interactions with midcircuit spin measurements that herald the probabilistic preparation of superpositions of squeezed, trisqueezed, and quadsqueezed states, which have not previously been experimentally demonstrated. We achieve independent control over the complex-valued squeezing parameter and the probability amplitude of each constituent, as well as their spatial separation. We directly observe the nonclassical nature of these states in the form of Wigner negativity following a full-state reconstruction. Our methods apply to any system where a quantum harmonic oscillator is coupled to a spin.
Quantum harmonic oscillators model phenomena from electromagnetic fields to molecular vibrations, with excitations represented by bosons such as photons or phonons. Linear interactions that create or annihilate single bosons generate coherent states of light or motion. Introducing higher-order nonlinear interactions produces richer quantum behaviour: second-order interactions enable squeezing, whereas higher-order interactions generate non-Gaussian states useful for continuous-variable quantum computation. However, such interactions are usually weak or require specialized hardware. Hybrid systems, where a linear interaction couples an oscillator to a spin, offer an alternative. Here we combine two spin-dependent linear bosonic interactions to implement up to fourth-order nonlinear bosonic interactions in a single trapped ion, focusing on generalized squeezing. We demonstrate and characterize squeezing, trisqueezing and quadsqueezing; reconstruct the Wigner functions of the resulting states; and achieve quadsqueezing over 100 times faster than conventional methods. The approach has no fundamental limit on the interaction order and applies to any platform supporting spin-dependent linear interactions.
Quantum harmonic oscillators model a wide variety of phenomena ranging from electromagnetic fields to vibrations of atoms in molecules. Their excitations can be represented by bosons such as photons, single particles of light, or phonons, the quanta of vibrational energy. Linear interactions that only create and annihilate single bosons can generate coherent states of light or motion. Introducing nth-order nonlinear interactions, that instead involve n bosons, leads to increasingly complex quantum behaviour. For example, second-order interactions enable squeezing, used to enhance the precision of measurements beyond classical limits, while higher-order interactions create non-Gaussian states essential for continuous-variable quantum computation. However, generating nonlinear interactions is challenging, typically requiring higher-order derivatives of the driving field or specialized hardware. Hybrid systems, where linear interactions couple an oscillator to an additional spin, offer a solution and are readily available across many platforms. Here, using the spin of a single trapped ion coupled to its motion, we employ two linear interactions to demonstrate up to fourth-order bosonic interactions; we focus on generalised squeezing interactions and demonstrate squeezing, trisqueezing, and quadsqueezing. We characterise these interactions, including their spin dependence, and reconstruct the Wigner function of the resulting states. We also discuss the scaling of the interaction strength, where we drive the quadsqueezing interaction more than 100 times faster than using conventional techniques. Our method presents no fundamental limit in the interaction order n and applies to any platform supporting spin-dependent linear interactions. Strong higher-order nonlinear interactions unlock the study of fundamental quantum optics, quantum simulation, and computation in a hitherto unexplored regime.
Quantum harmonic oscillators are a central resource in quantum technologies. Coupling this resource to a two-level system gives rise to spin-oscillator dynamics that can be used for system calibrations, enhanced sensitivity to signals, and the preparation of oscillator entangled states. Chapter 4 introduces a motional-frequency calibration protocol based on a time-reversal, state-dependent force sequence that maps the effects of motional-frequency miscalibration onto a narrow spin-response feature. The chapter also discusses how thermally occupied motional states enhance sensitivity to particular Hamiltonian terms, making them effective probe states. A two-point feedback servo with processing performed on a field-programmable gate array, or FPGA, is used to track the interaction resonance in real time, enabling sub-second updates and continuous correction of frequency drift during data acquisition. Chapter 5 realizes phase-insensitive displacement sensing by embedding spin-dependent squeezing in a time-reversal interferometry sequence. The method prepares a spin-correlated superposition of orthogonally squeezed motional states, yielding a spin-observable response used to estimate displacement amplitudes while remaining agnostic to the signal phase. Experiments with vacuum and number-state probes demonstrate enhanced sensitivity with increasing motional energy. Chapter 6 extends the spin-oscillator toolkit to multi-oscillator control. Optimized phase modulations applied to Jaynes-Cummings and anti-Jaynes-Cummings couplings between a single spin and two motional modes synthesize an effective two-mode squeezing interaction, enabling preparation of two-mode squeezed vacuum states and a non-Gaussian superposition of those states. Joint phase-space tomography reveals multi-mode correlations, and continuous-variable entanglement is certified by the Einstein-Podolsky-Rosen criterion and a Clauser-Horne-Shimony-Holt-type continuous-variable Bell test.
Abstract Coupled harmonic oscillators are ubiquitous in physics and play a prominent role in quantum science. They are a cornerstone of quantum mechanics and quantum field theory, where second quantization relies on harmonic oscillator operators to create and annihilate particles. Descriptions of quantum tunneling, beamsplitters, coupled potential wells, ``hopping terms'', decoherence, and many other phenomena rely on coupled harmonic oscillators. However, the ability to couple separate quantum harmonic oscillators directly, with coupling rates that substantially exceed decoherence rates, has remained elusive. Here, we realize high-fidelity coherent exchange of single motional quanta between harmonic oscillators -- in this case, spectrally separated harmonic modes of motion of a trapped ion crystal -- where the timing, strength, and phase of the coupling are controlled through an oscillating electric potential with suitable spatial variation. The coupling rate can be made much larger than the decoherence rates, enabling demonstrations of high-fidelity quantum state transfer, entanglement of motional modes, and Hong-Ou-Mandel-type interference. We also project a harmonic oscillator into its ground state by measurement and preserve that state during repetitions of the projective measurement, an important prerequisite for non-destructive syndrome measurement in continuous-variable quantum error correction. Controllable coupling between harmonic oscillators has potential applications in quantum information processing with continuous variables, quantum simulation, and precision measurements. It can also enable cooling and quantum logic spectroscopy involving motional modes of trapped ions that are not directly accessible.
Mesoscopic quantum superpositions, or Schrödinger cat states, are widely studied for fundamental investigations of quantum measurement and decoherence as well as applications in sensing and quantum information science. The generation and maintenance of such states relies upon a balance between efficient external coherent control of the system and sufficient isolation from the environment. Here we create a variety of cat states of a single trapped atom's motion in a harmonic oscillator using ultrafast laser pulses. These pulses produce high fidelity impulsive forces that separate the atom into widely separated positions, without restrictions that typically limit the speed of the interaction or the size and complexity of the resulting motional superposition. This allows us to quickly generate and measure cat states larger than previously achieved in a harmonic oscillator, and create complex multi-component superposition states in atoms.Generation of mesoscopic quantum superpositions requires both reliable coherent control and isolation from the environment. Here, the authors succeed in creating a variety of cat states of a single trapped atom, mapping spin superpositions into spatial superpositions using ultrafast laser pulses.
Generating multi-partite quantum entangled states amid dissipative environment is essential for advancing quantum simulation, metrology, and fundamental quantum research. Here, we use controlled dissipation as a resource and present an approach to generate programmable multimode entangled states in the vibrational modes of trapped ions, free of stringent requirements of initial state preparation. We experimentally demonstrate the generation of multimode squeezed states across two, three, and five modes out of initial thermal states by controlled couplings to dissipative internal spins. We characterize the output states by fidelity estimates and two-body correlations, confirming genuine multipartite entanglement using the van Loock-Furusawa inseparability criteria. This work outlines a generic path to create entangled nonclassical states with quantum harmonic oscillators, applicable for quantum information processing in continuous-variable quantum systems.