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arXiv:2409.01381 · Physical review. B./Physical review. B

Correlations in interacting electron liquids: Many-body statistics and hyperuniformity

Haina Wang, Rhine Samajdar, Salvatore Torquato A

Published Sep 3, 2024• 5 citations
arXivHTMLPDF

Abstract

Disordered hyperuniform many-body systems are exotic states of matter with novel optical, transport, and mechanical properties. These systems are characterized by an anomalous suppression of large-scale density fluctuations compared to ordinary liquids. The structure factor of disordered hyperuniform systems often obeys the scaling relation $S(k)\ensuremath{\sim}\mathcal{B}{k}^{\ensuremath{\alpha}}$ with $\mathcal{B},\ensuremath{\alpha}>0$ in the limit $k\phantom{\rule{0.16em}{0ex}}\ensuremath{\rightarrow}\phantom{\rule{0.16em}{0ex}}0$. Ground states of $d$-dimensional free fermionic gases, which are fundamental models for many metals and semiconductors, are key examples of quantum disordered hyperuniform states with important connections to random matrix theory. However, the effects of electron-electron interactions as well as the polarization of the electron liquid on hyperuniformity have not been explored thus far. In this paper, we systematically address these questions by deriving the analytical small-$k$ behaviors (and, associated, $\ensuremath{\alpha}$ and $\mathcal{B}$) of the total and spin-resolved structure factors of quasi-one-dimensional, two-dimensional, and three-dimensional electron liquids for varying polarizations and interaction parameters. We validate that these equilibrium disordered ground states are hyperuniform, as dictated by the fluctuation-compressibility relation. Interestingly, free fermions, partially polarized interacting fermions, and fully polarized interacting fermions are characterized by different values of the small-$k$ scaling exponent $\ensuremath{\alpha}$ and coefficient $\mathcal{B}$. In particular, partially polarized fermionic liquids exhibit a unique form of multihyperuniformity, in which the net configuration exhibits a stronger form of hyperuniformity (i.e., larger $\ensuremath{\alpha}$) than each individual spin component. The detailed theoretical analysis of such small-$k$ behaviors enables the construction of corresponding equilibrium classical systems under effective one- and two-body interactions that mimic the pair statistics of quantum electron liquids. Our paper thus reveals that highly unusual hyperuniform and multihyperuniform states can be achieved in simple fermionic systems and paves the way for harnessing unique hyperuniform scaling relations for applications, such as the construction of accurate density functionals.

DOI
10.1103/physrevb.110.104201

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Disordered hyperuniform many-body systems are exotic states of matter with novel optical, transport, and mechanical properties. These systems are characterized by an anomalous suppression of large-scale density fluctuations compared to ordinary liquids. The structure factor of disordered hyperuniform systems often obeys the scaling relation S(k)\ensuremath∼Bk\ensuremathαS(k)\ensuremath{\sim}\mathcal{B}{k}^{\ensuremath{\alpha}}S(k)\ensuremath∼Bk\ensuremathα with B,\ensuremathα>0\mathcal{B},\ensuremath{\alpha}>0B,\ensuremathα>0 in the limit k\ensuremath→0k\phantom{\rule{0.16em}{0ex}}\ensuremath{\rightarrow}\phantom{\rule{0.16em}{0ex}}0k\ensuremath→0. Ground states of ddd-dimensional free fermionic gases, which are fundamental models for many metals and semiconductors, are key examples of quantum disordered hyperuniform states with important connections to random matrix theory. However, the effects of electron-electron interactions as well as the polarization of the electron liquid on hyperuniformity have not been explored thus far. In this paper, we systematically address these questions by deriving the analytical small-kkk behaviors (and, associated, \ensuremathα\ensuremath{\alpha}\ensuremathα and B\mathcal{B}B) of the total and spin-resolved structure factors of quasi-one-dimensional, two-dimensional, and three-dimensional electron liquids for varying polarizations and interaction parameters. We validate that these equilibrium disordered ground states are hyperuniform, as dictated by the fluctuation-compressibility relation. Interestingly, free fermions, partially polarized interacting fermions, and fully polarized interacting fermions are characterized by different values of the small-kkk scaling exponent \ensuremathα\ensuremath{\alpha}\ensuremathα and coefficient B\mathcal{B}B. In particular, partially polarized fermionic liquids exhibit a unique form of multihyperuniformity, in which the net configuration exhibits a stronger form of hyperuniformity (i.e., larger \ensuremathα\ensuremath{\alpha}\ensuremathα) than each individual spin component. The detailed theoretical analysis of such small-kkk behaviors enables the construction of corresponding equilibrium classical systems under effective one- and two-body interactions that mimic the pair statistics of quantum electron liquids. Our paper thus reveals that highly unusual hyperuniform and multihyperuniform states can be achieved in simple fermionic systems and paves the way for harnessing unique hyperuniform scaling relations for applications, such as the construction of accurate density functionals.
Hyperuniform states of matter are characterized by anomalous suppression of long-wavelength density fluctuations. While most of the interesting cases of disordered hyperuniformity are provided by complex many-body systems such as liquids or amorphous solids, classical spin chains with certain long-range interactions have been shown to demonstrate the same phenomenon. Such spin-chain systems are ideal models for exploring the effects of quantum mechanics on hyperuniformity. It is well-known that the transverse field Ising model shows a quantum phase transition (QPT) at zero temperature. Under the quantum effects of a transverse magnetic field, classical hyperuniform spin chains are expected to lose their hyperuniformity. High-precision simulations of these cases are complicated because of the presence of highly nontrivial long-range interactions. We perform an extensive analysis of these systems using density matrix renormalization group simulations to study the possibilities of phase transitions and the mechanism by which they lose hyperuniformity. Even for a spin chain of length 30, we see discontinuous changes in properties like the ``$\ensuremath{\tau}$ order metric'' of the ground state, the measure of hyperuniformity, and the second cumulant of the total magnetization along the xxx-direction, all suggestive of first-order QPTs. An interesting feature of the phase transitions in these disordered hyperuniform spin chains is that, depending on the parameter values, the presence of a transverse magnetic field may lead remarkably to an increase in the order of the ground state as measured by the ``$\ensuremath{\tau}$ order metric,'' even if hyperuniformity is lost. Therefore, it would be possible to design materials to target specific novel quantum behaviors in the presence of a transverse magnetic field. Our numerical investigations suggest that these spin chains can show no more than two QPTs. We further analyze the long-range interacting spin chains via the Jordan-Wigner mapping onto a system of spinless fermions, showing that under the pairwise-interaction approximation and a mean-field treatment, there can be at most two quantum phase transitions. Based on these numerical and theoretical explorations, we conjecture that for spin chains with long-range pair interactions that have convergent cosine transforms, there can be a maximum of two quantum phase transitions at zero temperature.
Classical spin liquids (CSLs) are intriguing states of matter that do not exhibit long-range magnetic order and are characterized by an extensive ground-state degeneracy. Adding quantum fluctuations, which induce dynamics between these different classical ground states, can give rise to quantum spin liquids (QSLs). QSLs are highly entangled quantum phases of matter characterized by fascinating emergent properties, such as fractionalized excitations and topological order. One such exotic quantum liquid is the [Formula: see text] QSL, which can be regarded as a resonating valence bond (RVB) state formed from superpositions of dimer coverings of an underlying lattice. In this work, we unveil a hidden large-scale structural property of archetypal CSLs and QSLs known as hyperuniformity, i.e., normalized infinite-wavelength density fluctuations are completely suppressed in these systems. In particular, we first demonstrate that classical ensembles of close-packed dimers and their corresponding quantum RVB states are perfectly hyperuniform in general. Subsequently, we focus on a ruby-lattice spin liquid that was recently realized in a Rydberg-atom quantum simulator, and show that the QSL remains effectively hyperuniform even in the presence of a finite density of spinon and vison excitations, as long as the dimer constraint is still largely preserved. Moreover, we demonstrate that metrics based on the framework of hyperuniformity can be used to distinguish the QSL from other proximate quantum phases. These metrics can help identify potential QSL candidates, which can then be further analyzed using more advanced, computationally intensive quantum numerics to confirm their status as true QSLs.
Using higher-dimensional bosonization we study correlation functions of fermions with singular forward scattering. Following Bares and Wen [Phys. Rev. B 48, 8636 (1993)] we consider density-density interactions in ddd dimensions that diverge in Fourier space for small momentum transfers |q| as $|\mathbf{q}{|}^{\ensuremath{-}\ensuremath{\eta}}$ with $\ensuremath{\eta}=2(d\ensuremath{-}1).$ In this case the single-particle Green's function shows Luttinger-liquid behavior. However, in contrast to d=1,d=1,d=1, in higher dimensions the singularity of the momentum distribution nk{n}_{\mathbf{k}}nk​ for wave vectors k close to the Fermi wave vector kF{k}_{F}kF​ is characterized by a different exponent than the singularity of the density of states \ensuremath{\rho}(\ensuremath{\omega}) for frequencies \ensuremath{\omega} close to zero. We also calculate the irreducible polarization ${\ensuremath{\Pi}}_{\ensuremath{\star}}(\mathbf{q},\ensuremath{\omega})$ for $|\mathbf{q}|\ensuremath{\approx}{2k}_{F}.$ Whereas in the one-dimensional Tomonaga-Luttinger model ${\ensuremath{\Pi}}_{\ensuremath{\star}}(\ifmmode\pm\else\textpm\fi{}{2k}_{F}+q,\ensuremath{\omega})$ exhibits anomalous scaling, we show that in d>1d>1d>1 the leading singular corrections cancel. Thus, even though singular density-density interactions in d>1d>1d>1 lead to Luttinger liquid behavior of the single-particle Green's function, gauge invariant correlation functions such as the polarization or the conductivity show conventional Fermi-liquid behavior. We discuss consequences for the effect of disorder on higher-dimensional Luttinger liquids.
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In this thesis, symmetry and related transformation laws under a suitable unitary transformation are used in the study of the superconducting and magnetic properties of strongly correlated electronic systems. Such a study profits from a recently found global SO(3)×SO(3)×U(1) = [SO(4)×U(1)]/Z2 symmetry in the Hubbard model on a bipartite lattice. The introduction of the square-lattice quantum liquid relies on a general description of the Hubbard model consistent with its exact global SO(3) × SO(3) × U(1) symmetry. Such a quantum liquid is expected to play the same role for many-electron problems with short-range interactions on a square lattice, as a Fermi liquid for three-dimensional isotropic metals. It refers to the Hubbard model on the square lattice in the subspace spanned by the ground state, and the excited states generated by application onto it of one- and two-electron operators. For such a square-lattice quantum liquid only the charge c fermions and spin-neutral two-spinon s1 fermions play an active role. Part of the studies of this thesis use an effective superconductivity theory according to which, for zero spin density m = 0 and the range 0 < x < x∗ of finite hole concentrations of a short-range spin ordered phase, the ground state of the square-lattice quantum liquid of c and s1 fermions with residual interactions is superconducting. (For U/4t > ui ≈ 3/4 the critical hole concentration x∗ increases continuously upon increasing the U/4t value from x∗ = 1/√2 ≈ 0.225 at U/4t = ui to x∗ = 1/ ≈ 0.318 for U/4t → ∞.) Superconductivity emerges naturally from the effects of the residual interactions of the c and s1 fermions and as a side product of the short-range spin correlations. The phase of the c fermion pairs reads = 0 + 1 where the fluctuations of the phases 0 and 1 become large for x → 0 and x → x∗, respectively. For 0 < x < x∗ and x = 0, the symmetry of the action for the phase is a global superconducting U(1) symmetry and a local compact gauge symmetry, respectively. The former U(1) symmetry is identified with the U(1) symmetry of the Hubbard-model global SO(3) × SO(3) × U(1) = [SO(4) × U(1)]/Z2 symmetry. The amplitudes g = g0 g1, g0 = |heiθ0i|, and g1 = |heiθ1i|, their zero-temperature values ˘g ≈ (x/x∗)(1−x/x∗), ˘g0 ≈ (x/x∗), and ˘g1 ≈ (1−x/x∗) and the fluctuations of the phase , play an important role in the physics of the square-lattice quantum liquid. Together with the energy scale 2 0, which gives the maximum magnitude of the s1 fermion spinon pairing energy, they fully control the order parameters of both the short-range spin and long-range superconducting correlations. Indeed, for temperatures T < Tc, the short-range spin ordered phase has both a macroscopic quantum phase-coherent pair superconducting order so that |heiθi| > 0, and a short-range spin order, whereas for Tc < T < T∗ only the latter order prevails yet there remain c fermion pairing correlations such that |heiθ1i| > 0 but heiθ0i = 0. Here the critical temperature Tc and the crossover pseudogap temperature T∗ are fully controlled by the absolute value of the order parameters of the two above orders, respectively. However, the square-lattice quantum liquid alone does not describe quantitatively the unusual properties of the hole-doped cuprates. To fulfill such a goal we profit from a suitable theory according to which the interplay of electronic correlations described by the square-lattice quantum liquid of charge c fermions and spin-neutral two-spinon s1 fermions with intrinsic disorder, is behind the unusual properties of the holedoped hight-temperature cuprate superconductors. By profiting from such an interplay, an excellent quantitative agreement with experiments for the physical quantities of several families of hole-doped cuprates is reached. That includes universal properties such as a dome-like critical-temperature hole-concentration dependence and normal-state linear-T resistivity near optimal doping, extending over a wide temperature window. The results confirm a coexisting two-gap scenario associated with an incoherent two-spinon pairing and a coherent twoc- fermion pairing, respectively. While most of our studies focus on the superconducting and magnetic properties of the square-lattice quantum liquid associated with the Hubbard model on the square lattice, the magnetic properties of a related model – the periodic Anderson model – are also addressed, on the cubic lattice.
The metal–insulator transition (MIT) observed in a two-dimensional dilute electron liquid raises the question about the applicability of the scaling theory of disordered electrons, the approach pioneered by Phil Anderson and his collaborators,8 for the description of this transition. In this context, we review here the scaling theory of disordered electrons with electron–electron interactions. We start with the disordered Fermi liquid, and show how to adjust the microscopic Fermi-liquid theory to the presence of disorder. Then we describe the non-linear sigma model (NLSM) with interactions. This model has a direct relation with the disordered Fermi liquid, but can be more generally applicable, since it is a minimal model for disordered interacting electrons. The discussion is mostly about the general structure of the theory emphasizing the connection of the scaling parameters entering the NLSM with conservation laws. Next, we show that the MIT, as described by the NLSM with interactions, is a quantum phase transition and identify the parameters needed for the description of the kinetics and thermodynamics of the interacting liquid in the critical region of the transition. Finally, we discuss the MIT observed in Si -MOSFETs. We consider it as an example of the Anderson transition in the presence of the electron interactions. We demonstrate that the two-parameter RG equations, which treat disorder in the one-loop approximation but incorporate the full dependence on the interaction amplitudes, describe accurately the experimental data in Si -MOSFETs including the observed non-monotonic behavior of the resistance and its strong drop at low temperatures. The fact that this drop can be reproduced theoretically, together with the argument that Anderson localization should occur at strong disorder, justified the existence of the MIT within the scaling theory.