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arXiv:2408.12306 · Optics Express

Pulse characterization at the single-photon level through chronocyclic Q -function measurements

Abhinandan Bhattacharjee, Patrick Folge, Laura Serino, Jaroslav Řeháček, Z. Hradil, Christine Silberhorn, Benjamin Brecht

Published Dec 6, 2024• 2 citations
arXivHTMLPDF

Abstract

The characterization of the complex spectral amplitude, that is, the spectrum and spectral phase, of single-photon-level light fields is a crucial capability for modern photonic quantum technologies. Since established pulse characterization techniques are not applicable at low intensities, alternative approaches are required. Here, we demonstrate the retrieval of the complex spectral amplitude of single-photon-level light pulses through measuring their chronocyclic Q −function. Our approach draws inspiration from quantum state tomography by exploiting the analogy between quadrature phase space and time-frequency phase space. In the experiment, we perform time-frequency projections with a quantum pulse gate (QPG), which directly yield the chronocyclic Q −function. We evaluate the complex spectral amplitude from the measured chronocyclic Q −function data with maximum likelihood estimation (MLE), which is the established technique for quantum state tomography. The MLE yields not only an unambigious estimate of the complex spectral amplitude of the state under test that does not require any a priori information, but also allows for, in principle, estimating the spectral-temporal coherence properties of the state. Our method accurately recovers features such as jumps in the spectral phase and is resistant against regions with zero spectral intensity, which makes it immediately beneficial for classical pulse characterization problems.

DOI
10.1364/oe.540125

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The characterization of the complex spectral amplitude, that is, the spectrum and spectral phase, of single-photon-level light fields is a crucial capability for modern photonic quantum technologies. Since established pulse characterization techniques are not applicable at low intensities, alternative approaches are required. Here, we demonstrate the retrieval of the complex spectral amplitude of single-photon-level light pulses through measuring their chronocyclic Q −function. Our approach draws inspiration from quantum state tomography by exploiting the analogy between quadrature phase space and time-frequency phase space. In the experiment, we perform time-frequency projections with a quantum pulse gate (QPG), which directly yield the chronocyclic Q −function. We evaluate the complex spectral amplitude from the measured chronocyclic Q −function data with maximum likelihood estimation (MLE), which is the established technique for quantum state tomography. The MLE yields not only an unambigious estimate of the complex spectral amplitude of the state under test that does not require any a priori information, but also allows for, in principle, estimating the spectral-temporal coherence properties of the state. Our method accurately recovers features such as jumps in the spectral phase and is resistant against regions with zero spectral intensity, which makes it immediately beneficial for classical pulse characterization problems.
Summary form only given. The goal of any pulse characterization protocol is to describe how the spectral components of the electric field are changing in time. Apart from linear methods such as streak cameras, characterization techniques based on nonlinear processes have been developed. Those processes require broad spectral acceptance bandwidths, i.e. to be capable of resolving ultrashort features of the pulse. For many of those techniques, the pulses are reconstructed by iterative or deconvolution algorithms where the electric field is assumed to be fully coherent and do not account for the possibility of reduced coherence from pulse to pulse, or within a single pulse. In general, the chronocyclic Wigner function should be reconstructed in order to provide full information about an ensemble of partially coherent pulses. To make a parallel with quantum mechanics, most quantum systems cannot be considered as closed and interact with the environment, and subsequently, undergo decoherence. Therefore, a noisy quantum state cannot be described by a single pure state only but as a classical mixture of pure states.
Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate characterization of such pulses, including spectral coherence, remains challenging because current methods require substantial experimental resources and complex reconstruction algorithms. Here, we introduce frequency-bin interferometry for reconstructing electric fields with low intensity (FIREFLY), a technique that directly provides spectral amplitude, phase, and coherence profiles of single-photon pulses without requiring intensive reconstruction algorithms. Our approach measures the two-point spectral correlation function of the pulse by interfering its different frequency components using a quantum pulse gate (QPG) driven by a reference pump pulse. We demonstrate its compatibility with quantum light by characterizing partially coherent pulses generated by a type-0 parametric down-conversion process. We also overcome this requirement of a known pump pulse by introducing spectral shear into our interferometric scheme using a multi-output QPG (mQPG). This enables simultaneous characterization of a single-photon-level input pulse alongside an unknown pump pulse. Notably, our method achieves theory-experiment similarity above 95\% across all retrieved profiles, which demonstrates the reliability of this scheme for quantum information applications based on time-frequency encodings.
Temporal-spectral modes of light provide a fundamental window into the nature of quantum systems and offer a robust means for information encoding. Methods to precisely characterize the temporal-spectral state of light at the single-photon level thus play a central role in understanding single-photon sources and their applications in emerging optical quantum technologies. Here we demonstrate an optical reference-free method, which melds techniques from ultrafast metrology and single-photon spectral detection, to characterize the pulse-mode structure of heralded single photons.
Encoding quantum information in the photon temporal mode (TM) offers a robust platform for high-dimensional quantum protocols. The main practical challenge, however, is to design a device that operates on single photons in specific TMs and all coherent superpositions. The quantum pulse gate (QPG) is a mode-selective sum-frequency generation designed for this task. Here, we perform a full modal characterization of a QPG using weak coherent states in well-defined TMs. We reconstruct a full set of measurement operators, which show an average fidelity of 0.85 to a theoretically ideal device when operating on a seven-dimensional space. Then we use these characterized measurement operators of the QPG to calibrate the device. Using the calibrated device and a tomographically complete set of measurements, we show that the QPG can perform high-dimensional TM state tomography with 0.99 fidelity.
Accessing a high dimensional Hilbert space spanned by temporal modes (TMs) of single-photons is an intriguing idea for quantum information protocols, though it is experimentally challenging. The quantum pulse gate (QPG), a group-velocity matched sum-frequency process, can perform arbitrary TM resolved measurement. We present a thorough characterisation of measurement operators of a QPG and we show that this device is capable of performing full state tomography with 99% fidelity. Moreover, we use this device for TM tomography of pure and mixed heralded single-photon states in 7-dimensional Hilbert space.