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arXiv:2408.12075 · Physical Review Letters

Electromagnetically Induced Transparency Cooling of High-Nuclear-Spin Ions

Chuanxin Huang, Chenxi Wang, Hongxuan Zhang, Hongyuan Hu, Z.-Q. Wang, Zhichao Mao, Shijiao Li, Pan‐Yu Hou, Yukai Wu, Z.-C. Zhou, Luming Duan

Published Sep 13, 2024• 13 citations
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Abstract

We report the electromagnetically induced transparency (EIT) cooling of ^{137}Ba^{+} ions with a nuclear spin of I=3/2, which are a good candidate of qubits for future large-scale trapped-ion quantum computing. EIT cooling of atoms or ions with a complex ground-state level structure is challenging due to the lack of an isolated Λ system, as the population can escape from the Λ system to reduce the cooling efficiency. We overcome this issue by leveraging an EIT pumping laser to repopulate the cooling subspace, ensuring continuous and effective EIT cooling. We cool the two radial modes of a single ^{137}Ba^{+} ion to average motional occupations of 0.08(5) and 0.15(7), respectively. Using the same laser parameters, we also cool all the ten radial modes of a five-ion chain to near their ground states. Our approach can be adapted to atomic species possessing similar level structures. It allows engineering of the EIT Fano-like spectrum, which can be useful for simultaneous cooling of modes across a wide frequency range, aiding in large-scale trapped-ion quantum information processing.

DOI
10.1103/physrevlett.133.113204

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We report the electromagnetically induced transparency (EIT) cooling of ^{137}Ba^{+} ions with a nuclear spin of I=3/2, which are a good candidate of qubits for future large-scale trapped-ion quantum computing. EIT cooling of atoms or ions with a complex ground-state level structure is challenging due to the lack of an isolated Λ system, as the population can escape from the Λ system to reduce the cooling efficiency. We overcome this issue by leveraging an EIT pumping laser to repopulate the cooling subspace, ensuring continuous and effective EIT cooling. We cool the two radial modes of a single ^{137}Ba^{+} ion to average motional occupations of 0.08(5) and 0.15(7), respectively. Using the same laser parameters, we also cool all the ten radial modes of a five-ion chain to near their ground states. Our approach can be adapted to atomic species possessing similar level structures. It allows engineering of the EIT Fano-like spectrum, which can be useful for simultaneous cooling of modes across a wide frequency range, aiding in large-scale trapped-ion quantum information processing.
Cooling of atomic motion is a crucial tool for many branches of atomic physics, ranging from fundamental physics explorations to quantum information and sensing. For trapped ions, electromagnetically-induced-transparency (EIT) cooling has received attention for the relative speed, low laser power requirements, and broad cooling bandwidth of the technique. However, in applications where the ion used for cooling has hyperfine structure to enable long coherence times, it is difficult to find a closed three-level system in which to perform standard EIT cooling. Here, we demonstrate successful EIT cooling on 25Mg+^{25}\mathrm{Mg}^{+}25Mg+ by the addition of an extra laser frequency; this method can be applied to any ion with nonzero nuclear spin. Furthermore, we simultaneously EIT cool all axial modes in mixed-species crystals $^{9}\mathrm{Be}^{+}\text{\ensuremath{-}}^{25}\mathrm{Mg}^{+}$ and $^{9}\mathrm{Be}^{+}\text{\ensuremath{-}}^{25}\mathrm{Mg}^{+}\text{\ensuremath{-}}^{9}\mathrm{Be}^{+}$ through the 25Mg+^{25}\mathrm{Mg}^{+}25Mg+ ion. This demonstrates the viability of EIT cooling in architectures where the laser-cooled species can host high-fidelity hyperfine qubits.
We report the electromagnetically-induced-transparency (EIT) cooling of a large trapped ^{171}Yb^{+} ion chain to the quantum ground state. Unlike conventional EIT cooling, we engage a four-level tripod structure and achieve fast sub-Doppler cooling over all motional modes. We observe simultaneous ground-state cooling across the complete transverse mode spectrum of up to 40 ions, occupying a bandwidth of over 3 MHz. The cooling time is observed to be less than 300 μs, independent of the number of ions. Such efficient cooling across the entire spectrum is essential for high-fidelity quantum operations using trapped ion crystals for quantum simulators or quantum computers.
We theoretically propose and experimentally demonstrate a parallel electromagnetically induced transparency (parallel EIT) cooling technique for ion crystals in the Paul trap. It breaks the stringent cooling requirements of the standard EIT cooling, thus allowing, in principle, to simultaneously cool the motional mode spectrum with an arbitrary range. Experimentally a large cooling range over 5 MHz is proved by using a single trapped 40Ca+{}^{40}{\mathrm{Ca}}^{+}40Ca+ ion. We also observe simultaneous near-ground-state cooling for all motional modes of a 4-ion chain with the best average phonon number of about 0.2. For cooling a large number of modes, we only need to modulate the probe beam of the standard EIT cooling with several rf frequencies. This cooling scheme has no selectivity for the types of ions (e.g., 171Yb+{}^{171}{\mathrm{Yb}}^{+}171Yb+, 40Ca+{}^{40}{\mathrm{Ca}}^{+}40Ca+), therefore it would be a powerful tool for initialization of all kinds of operational trapped-ion quantum computers or simulators.
Electromagnetically-induced-transparency (EIT) cooling is a ground-state cooling technique for trapped particles. EIT offers a broader cooling range in frequency space compared to more established methods. In this work, we experimentally investigate EIT cooling in strings of trapped atomic ions. In strings of up to 18 ions, we demonstrate simultaneous ground-state cooling of all radial modes in under 1 ms. This is a particularly important capability in view of emerging quantum simulation experiments with large numbers of trapped ions. Our analysis of the EIT cooling dynamics is based on a technique enabling single-shot measurements of phonon numbers, by rapid adiabatic passage on a vibrational sideband of a narrow transition.
Motional modes of trapped-ion crystals in Penning traps can now be cooled to near their ground states via electromagnetically induced transparency (EIT) cooling. Numerical simulations are valuable tools for interpreting EIT cooling results and optimizing experimental protocols, but existing molecular dynamics codes are limited to the simulation of Doppler cooling. In this work, we fill this gap by implementing a semiclassical model of EIT cooling in a novel MD code. By simultaneously evolving the ions' internal quantum states and classical motion, we are able to calculate the instantaneous EIT laser forces acting on the ions. We first validate our code by comparing the single-ion cooling rate to fully quantum simulation results. Next, we analyze cooling of the drumhead modes in planar ion crystals, quantifying the effects of planar ion motion and a finite laser beam width. Finally, we demonstrate efficient EIT cooling of the axial modes in 3D ellipsoidal crystals containing up to 500 ions. Such crystals are a promising platform for future quantum sensing experiments with enhanced sensitivity. We find that the mode spectra of 3D crystals can be engineered to enable sympathetic cooling of the low-frequency E×B\boldsymbol{E}\times\boldsymbol{B}E×B modes. This numerical framework provides a powerful tool for modeling sub-Doppler cooling techniques and for optimizing future quantum sensing and quantum information experiments.
Electromagnetically Induced Transparency (EIT) cooling is a well-established method for preparing trapped ion systems in their motional ground state. However, isolating a three-level system, as required for EIT cooling, is often challenging or impractical. Nonetheless, multilevel systems can inherently host dark states. In this work, we extend the EIT cooling framework to such multilevel systems. We develop a formalism to accurately determine the cooling rate in the weak sideband coupling regime and provide an approximate estimate for cooling rates beyond this regime, without the need for explicit simulation of the motional degree of freedom. We clarify the connection between the cooling rate and the absorption spectrum, offering a pathway for efficient near-ground-state cooling of ions with complex electronic structures.