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arXiv:2408.09596

Coherent expansion of the motional state of a massive nanoparticle beyond its linear dimensions

Rafael Muffato, Tiberius Georgescu, Matteo Carlesso, Mauro Paternostro, H. Ulbricht

Published Aug 18, 2024• 0 citations
arXivHTMLPDF

Abstract

Quantum mechanics predicts that massive particles exhibit wave-like behavior. Matterwave interferometry has been able to validate such predictions through ground-breaking experiments involving microscopic systems like atoms and molecules. The wavefunction of such systems coherently extends over a distance much larger than their size, an achievement that is incredibly challenging for massive and more complex objects. Yet, reaching similar level of coherent diffusion will enable tests of fundamental physics at the genuinely macroscopic scale, as well as the development of quantum sensing apparata of great sensitivity. We report on experimentally achieving an unprecedented degree of position diffusion in a massive levitated optomechanical system through frequency modulation of the trapping potential. By starting with a pre-cooled state of motion and employing a train of sudden pulses yet of mild modulation depth, we surpass previously attained values of position diffusion in this class of systems to reach diffusion lengths that exceed the physical dimensions of the trapped nanoparticle.

DOI
10.48550/arxiv.2408.09596

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Quantum mechanics predicts that massive particles exhibit wave-like behavior. Matterwave interferometry has been able to validate such predictions through ground-breaking experiments involving microscopic systems like atoms and molecules. The wavefunction of such systems coherently extends over a distance much larger than their size, an achievement that is incredibly challenging for massive and more complex objects. Yet, reaching similar level of coherent diffusion will enable tests of fundamental physics at the genuinely macroscopic scale, as well as the development of quantum sensing apparata of great sensitivity. We report on experimentally achieving an unprecedented degree of position diffusion in a massive levitated optomechanical system through frequency modulation of the trapping potential. By starting with a pre-cooled state of motion and employing a train of sudden pulses yet of mild modulation depth, we surpass previously attained values of position diffusion in this class of systems to reach diffusion lengths that exceed the physical dimensions of the trapped nanoparticle.
Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments, and towards quantum-enhanced force sensing with levitated particles.
Abstract Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules [1, 2]. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself [3]. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances [4–7]. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments [8], and towards quantum-enhanced force sensing with levitated particles [9].
Matter waves have been observed in double-slit experiments with microscopic objects, such as atoms or molecules. The wave function describing the motion of these objects must extend over a distance comparable to the slit separation, much larger than the characteristic size of the objects. Preparing such states for more massive objects, such as mechanical oscillators, remains an outstanding challenge. Here we delocalize the quantum ground state of an optically levitated nanosphere by modulating the stiffness of the confining potential. We show a more than threefold increase of the initial coherence length, which corresponds to mechanical momentum squeezing of more than 7 dB. Our work is a stepping stone toward the generation of coherence lengths comparable to the object size, a crucial regime for macroscopic quantum experiments.
Levitated nanoparticles in vacuum are prime candidates for generating macroscopic quantum superposition states of massive objects. Most protocols for preparing these states necessitate coherent expansion beyond the scale of the zero-point motion to produce sufficiently delocalized and pure phase-space distributions. Here, we spatially expand and subsequently recontract the thermal state of a levitated nanoparticle by modifying the stiffness of the trap holding the particle. We achieve state-expansion factors of 25 in standard deviation for a particle initially feedback-cooled to a center-of-mass thermal state of \SI{155}{\milli\kelvin}. Our method relies on a hybrid scheme combining an optical trap, for cooling and measuring the particle's motion, with a Paul trap for expanding its state. Consequently, state expansion occurs devoid of measurement backaction from photon recoil, making this approach suitable for coherent wavefunction expansion in future experiments.
Quantum control of complex objects in the regime of large size and mass provides opportunities for sensing applications and tests of fundamental physics. The realization of such extreme quantum states of matter remains a major challenge. We demonstrate a quantum interface that combines optical trapping of solids with cavity-mediated light-matter interaction. Precise control over the frequency and position of the trap laser with respect to the optical cavity allowed us to laser-cool an optically trapped nanoparticle into its quantum ground state of motion from room temperature. The particle comprises 108 atoms, similar to current Bose-Einstein condensates, with the density of a solid object. Our cooling technique, in combination with optical trap manipulation, may enable otherwise unachievable superposition states involving large masses.
Abstract The quantum superposition principle is a fundamental concept of physics 1 and the basis of numerous quantum technologies 2,3 . Yet, it is still often regarded counterintuitive because we do not observe its key features on the macroscopic scales of our daily lives. It is, therefore, interesting to ask how quantum properties persist or change as we increase the size and complexity of objects 4 . A model test for this question can be realized by matter-wave interferometry, in which the motion of individual massive particles becomes delocalized and needs to be described by a wave function that spans regions far larger than the particle itself 5 . Over the years, this has been explored with a series of objects of increasing mass and complexity 6–9 and a growing community aims at pushing this to ever larger limits. Here we present an experimental platform that extends matter-wave interference to large metal clusters, a qualitatively new material class for quantum experiments. We specifically demonstrate quantum interference of sodium nanoparticles, which can each contain more than 7,000 atoms at masses greater than 170,000 Da. They propagate in a Schrödinger cat state with a macroscopicity 10 of μ = 15.5, surpassing previous experiments 5,9,11 by an order of magnitude.