We theoretically investigate the out-of-equilibrium dynamics of irregular one- and two-dimensional arrays of Rydberg dipoles featuring spatially anisotropic interactions. Starting from a collectively polarized initial state, we map out the dynamical phase diagram and identify a crossover between regimes of regular and anomalously slow relaxation of the initial collective order that strongly depends on both the degree of interaction disorder and anisotropy. In addition, we find that the regime of slow relaxation is characterized by a subballistic propagation of correlations that remained confined to short distances even at long times. To explain our findings we develop an analytic model based on decoupled clusters of interacting dipoles that goes beyond prior theoretical works and enables us to identify multiple relaxation timescales. Our findings can be relevant for a wide variety of quantum science platforms naturally featuring disordered dipolar interactions, including polar molecules, frozen Rydberg gases, and nitrogen-vacancy centers.
We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the dynamics lead to spatially correlated collective relaxation reminiscent of glasses. We study and quantify the evolution towards equilibrium in one and two dimensions, and analyze how the degree of glassiness and the relaxation time are controlled by the interaction strength between Rydberg atoms. We also find that spontaneous decay of Rydberg excitations leads to an interruption of glassy relaxation that takes the system to a highly correlated nonequilibrium stationary state. The results presented here, which are in principle also applicable to other systems such as polar molecules and atoms with large magnetic dipole moments, show that the collective behavior of cold atomic and molecular ensembles can be similar to that found in soft condensed-matter systems.
We study the decoherence dynamics of dipole-coupled two-level quantum systems in Ramsey-type experiments. We focus on large networks of two-level systems, confined to two spatial dimensions and with positional disorder giving rise to disordered dipolar couplings. This setting is relevant for modeling the decoherence dynamics of the rotational excitations of polar molecules confined to deep optical lattices, where disorder arises from the random filling of lattice sites with occupation probability
p. We show that the decoherence dynamics exhibits a phase transition at a critical filling ${p}_{c}\ensuremath{\simeq}0.15$. For
p<pc the dynamics is disorder dominated and the Ramsey interference signal decays on a time scale ${T}_{2}\ensuremath{\propto}{p}^{\ensuremath{-}3/2}$. For
p>pc the dipolar interactions dominate the disorder, and the system behaves as a collective spin-ordered phase, representing synchronization of the two-level systems and persistent Ramsey oscillations with divergent
T2 for large systems. For a finite number of two-level systems
N, the spin-ordered phase at
p>pc undergoes a crossover to a collective spin-squeezed state on a time scale ${\ensuremath{\tau}}_{\mathrm{sq}}\ensuremath{\propto}\sqrt{N}$. We develop a self-consistent mean-field theory that is capable of capturing the synchronization transition at
pc, and provide an intuitive theoretical picture that describes the phase transition in the long-time dynamics. We also show that the decoherence dynamics appear to be ergodic in the vicinity of
pc, the long-time behavior being well described by the predictions of equilibrium thermodynamics. The results are supported by the results of exact diagonalization studies of small systems.
Abstract Topological phases of matter can appear in noninteracting systems, as in band topology, or interacting systems, such as in spin models, with their defining features typically robust against weak disorder. Intriguingly, disorder itself can also induce topological phases--exemplified by the Anderson topological insulator in noninteracting systems. Experimental studies on disorder-induced topology have so far been limited to band topology. Here we report direct observations of disorder-induced many-body interacting average topological order in an atom array at half-filling, whereby random offsets to tweezer locations forming a lattice implement structural disorder, causing fluctuating long-range dipolar interactions between tweezer confined single atoms. The ground state degeneracy in disordered configurations is detected and compared to the regular lattice. The induced topological phase is vindicated by the spatially resolved atom-atom correlation functions for different forms of dimer compositions. By probing the quench dynamics of a highly excited state, we observe markedly slower decay of edge spin magnetization in comparison to the bulk spin, consistent with the presence of topologically protected edge modes in disordered lattices. Our experiments open a new direction for studying the interplay between disorder and strongly interacting topological matter in Rydberg atom arrays.
When a strongly disordered system of interacting quantum dipoles is locally excited, the excitation relaxes on some (potentially very long) timescale. We analyze this relaxation process, both for electron glasses with strong Coulomb interactions---in which particle-hole dipoles are emergent excitations---and for systems (e.g., quantum magnets or ultracold dipolar molecules) made up of microscopic dipoles. We consider both energy relaxation rates (
T1 times) and dephasing rates (
T2 times), and their dependence on frequency, temperature, and polarization. Systems in both two and three dimensions are considered, along with the dimensional crossover in quasi-two-dimensional geometries. A rich set of scaling laws is found.
Spin squeezed entanglement enables metrological precision beyond the classical limit. Understood through the lens of continuous symmetry breaking, dipolar spin systems exhibit the remarkable ability to generate spin squeezing via their intrinsic quench dynamics. To date, this understanding has primarily focused on lattice spin systems; in practice however, dipolar spin systems$\unicode{x2014}$ranging from ultracold molecules to nuclear spin ensembles and solid-state color centers$\unicode{x2014}$often exhibit significant amounts of positional disorder. Here, we develop a theory for scalable spin squeezing in a two-dimensional randomly diluted lattice of quantum dipoles, which naturally realize a dipolar XXZ model. Via extensive quantum Monte Carlo simulations, we map out the phase diagram for finite-temperature XY order, and by extension scalable spin squeezing, as a function of both disorder and Ising anisotropy. As the disorder increases, we find that scalable spin squeezing survives only near the Heisenberg point. We show that this behavior is due to the presence of rare tightly-coupled dimers, which effectively heat the system post-quench. In the case of strongly-interacting nitrogen-vacancy centers in diamond, we demonstrate that an experimentally feasible strategy to decouple the problematic dimers from the dynamics is sufficient to enable scalable spin squeezing.
How quantum matter relaxes far from equilibrium is a central open problem in many-body physics, and one for which analog quantum simulators are well positioned to move from confirming theory to discovering new physics. Here, we use a two-dimensional Rydberg atom array of 256 qubits to map the relaxation landscape of the two-dimensional transverse-field Ising model across its phase diagram. Beyond the expected rapid thermalization, we identify two further regimes. The first is a prethermal regime whose dynamics are governed by an effective XY model. The second, and most unexpected, is a crossover regime characterized by a slowdown in relaxation. This slowdown occurs precisely where state-of-the-art classical tensor-network methods lose control at late times, whereas the quantum simulation remains consistent across system sizes. These results establish Rydberg atom arrays as a platform for scientific discovery in nonequilibrium quantum many-body dynamics.