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arXiv:2408.07068 · Optica Quantum

Atomic fluorescence collection into planar photonic devices

Orion Smedley, Vighnesh Natarajan, Oscar Jaramillo, Hamim Mahmud Rivy, Karan K. Mehta

Published Dec 16, 2024• 5 citations
arXivHTMLPDF

Abstract

Fluorescence collection from individual emitters plays a key role in state detection and remote entanglement generation, fundamental functionalities in many quantum platforms. Planar photonics have been demonstrated for robust and scalable addressing of trapped-ion systems, motivating consideration of similar elements for the complementary challenge of photon collection. Here, using an argument from the reciprocity principle, we show that far-field photon collection efficiency can be simply expressed in terms of the fields associated with the collection optic at the emitter position alone. We calculate collection efficiencies into ideal paraxial and fully vectorial focused Gaussian modes parameterized in terms of focal waist, and further quantify the modest enhancements possible with more general beam profiles, establishing design requirements for efficient collection. Toward practical implementation, we design, fabricate, and characterize two diffractive collection elements operating at λ = 397 nm; a forward emitting design is predicted to offer 0.25% collection efficiency into a single waveguide mode, while a more efficient reverse-emitting design offers 1.14% collection efficiency, albeit with more demanding fabrication requirements. Close agreement between simulated and measured emission for both designs indicates practicality of these collection efficiencies, and we indicate avenues to improved devices approaching the limits predicted for ideal beams. We point out a particularly simple integrated waveguide configuration for polarization-based remote entanglement generation enabled by integrated collection.

DOI
10.1364/opticaq.540626

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Fluorescence collection from individual emitters plays a key role in state detection and remote entanglement generation, fundamental functionalities in many quantum platforms. Planar photonics have been demonstrated for robust and scalable addressing of trapped-ion systems, motivating consideration of similar elements for the complementary challenge of photon collection. Here, using an argument from the reciprocity principle, we show that far-field photon collection efficiency can be simply expressed in terms of the fields associated with the collection optic at the emitter position alone. We calculate collection efficiencies into ideal paraxial and fully vectorial focused Gaussian modes parameterized in terms of focal waist, and further quantify the modest enhancements possible with more general beam profiles, establishing design requirements for efficient collection. Toward practical implementation, we design, fabricate, and characterize two diffractive collection elements operating at λ = 397 nm; a forward emitting design is predicted to offer 0.25% collection efficiency into a single waveguide mode, while a more efficient reverse-emitting design offers 1.14% collection efficiency, albeit with more demanding fabrication requirements. Close agreement between simulated and measured emission for both designs indicates practicality of these collection efficiencies, and we indicate avenues to improved devices approaching the limits predicted for ideal beams. We point out a particularly simple integrated waveguide configuration for polarization-based remote entanglement generation enabled by integrated collection.
Spontaneously emitted photons are entangled with the electronic and nuclear degrees of freedom of the emitting atom, so interference and measurement of these photons can entangle separate matter-based quantum systems as a resource for quantum information processing. Since confinement in a single-mode facilitates the photon interference needed for generating entanglement, the dipole emission patterns relevant in spontaneous emission present a mode-matching challenge. Current demonstrations rely on bulk photon-collection and manipulation optics that suffer from large component size and system-to-system variability-factors that impede scaling to the large numbers of entangled pairs needed for quantum information processing. To address these limitations, we demonstrate a collection method that enables passive phase stability, straightforward photonic manipulation, and intrinsic reproducibility. Specifically, we engineer a waveguide-integrated grating to couple photons emitted from a trapped ion into a single optical mode within a microfabricated ion-trap chip. Using the integrated collection optic, we characterize the collection efficiency, image the ion, and detect the ion's quantum state. The integrated optic covers 2.18% of the solid angle and collects 1.97 ± 0.3% of the spontaneously emitted light incident on the grating for a total collection efficiency of 0.043% into a single-mode waveguide. This proof-of-principle demonstration lays the foundation for leveraging the inherent stability and reproducibility of integrated photonics to create, manipulate, and measure multipartite quantum states in arrays of quantum emitters.
Trapped atomic ions are natural candidates for quantum information processing and have the potential to realize or improve quantum computing, sensing, and networking. These applications often require the collection of individual photons emitted from ions into guided optical modes, in some cases for the production of entanglement between separated ions. Proof-of-principle demonstrations of such photon collection from trapped ions have been performed using high-numerical-aperture lenses or cavities and single-mode fibers, but integrated photonic elements in ion-trap structures offer advantages in scalability and manufacturability over traditional optics. In this paper we analyze structures monolithically fabricated with an ion trap for collecting ion-emitted photons, coupling them into waveguides, and manipulating them via interference. We calculate geometric limitations on collection efficiency for this scheme, simulate a single-layer grating that shows performance comparable to demonstrated free-space optics, and discuss practical fabrication and fidelity considerations. Based on this analysis, we conclude that integrated photonics can support scalable systems of trapped ions that can distribute quantum information via photon-mediated entanglement.
Fluorescence collection sets the efficiency of state detection and the rate of entanglement generation between remote trapped ion qubits. Despite efforts to improve light collection using various optical elements, solid angle capture is limited to ≈10% for implementations that are scalable to many ions. We present an approach based on fluorescence detection through a transparent trap using an integrated photodetector, combining collection efficiency approaching 50% with scalability. We microfabricate transparent surface traps with indium tin oxide and verify stable trapping of single ions. The fluorescence from a cloud of ions is detected using a photodiode sandwiched with a transparent trap.
Trapped, laser-cooled atoms and ions produce intense fluorescence of the order 107~108 photons per second. Detection of this fluorescence enables efficient measurement of the quantum state of qubits based on trapped atoms. It is desirable to collect a large fraction of the photons to make the detection faster and more reliable. Additionally, efficient fluorescence collection can improve the speed and fidelity of remote ion entanglement and quantum gates. Refractive and reflective optics, and optical cavities have all been used to collect the trapped ion fluorescence with up to about 10% efficiency. Here we show a novel ion trap design that incorporates a metallic spherical mirror as the integral part of the trap itself, being its RF electrode. The mirror geometry enables up to 35% solid angle collection of trapped ion fluorescence. The movable central pin electrode of this trap allows precise placement of the ion at the focus of the reflector. We characterize the performance of the mirror, and measure 25% collection efficiency, likely limited by the imperfections of the mirror surface. We also study the properties of the images of single ions formed by the spherical mirror and apply aberration correction with an aspherical element placed outside the vacuum system. Owing to the simplicity of its design, this trap structure can be adapted for microfabrication and integration into more complex trap architectures.
Ion trap systems allow the faithful storage and manipulation of qubits encoded in the energy levels of the ions, and can be interfaced with photonic qubits that can be transmitted to connect remote quantum systems. Single photons transmitted from two remote sites, each entangled with one quantum memory, can be used to entangle distant quantum memories by interfering on a beam splitter. Efficient remote entanglement generation relies upon efficient light collection from single ions into a single mode fiber. This can be realized by integrating an ion trap with an optical cavity and employing the Purcell effect for enhancing the light collection. Remote entanglement can be used as a resource for a quantum repeater for provably secure long-distance communication or as a method for communicating within a distributed quantum information processor. I present the integration of a 1 mm optical cavity with a micro-fabricated surface ion trap. The plano-concave cavity is oriented normal to the chip surface where the planar mirror is attached underneath the trap chip. The cavity is locked using a 780 nm laser which is stabilized to Rubidium and shifted to match the 369 nm Doppler transition in Ytterbium. The linear ion trap allows ions to be shuttled in and out of the cavity mode. The Purcell enhancement of spontaneous emission into the cavity mode would then allow efficient collection of the emitted photons, enabling faster remote entanglement generation.
Efficient collection of fluorescence light is essential for all optically adressable qubit platforms. For the nitrogen-vacancy (NV) center in diamond, the high refractive index of the host medium poses a major challenge as it limits the solid angle under which fluorescence light can leave the crystal. To enhance collection efficiency from single NV centers, we design and simulate micro-optical elements that shall be directly fabricated on the diamond surface using two-photon polymerization. Several optical designs and photoresists are evaluated for their expected coupling efficiency into single-mode fibers and their tolerance to fabrication errors. Additionally, an analytical solution for single lens collimation of the emission of a point source in diamond at a specific wavelength is presented, as well as considerations regarding the degradation of wavefront quality in multi-wavelength Fresnel designs.