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arXiv:2407.15919

Lectures on the quantum phase transitions of metals

Subir Sachdev A

Published Jul 22, 2024• 1 citation
arXivHTMLPDF

Abstract

Quantum phase transitions of metals involve changes in the Fermi surface, and can be divided into three categories. The first two categories involve symmetry breaking, and lead to a deformation or reconstruction of the Fermi surface. The third category involves a change in the volume enclosed by the Fermi surface without any symmetry breaking: one phase is a Fermi liquid (FL) with the conventional Luttinger volume, while the other phase is a `fractionalized Fermi liquid' (FL*), which has a non-Luttinger volume Fermi surface accompanied by a spin liquid with fractionalized excitations. It is a relatively simple matter to obtain a FL*-FL transition in Kondo lattice models. However, the FL*-FL transition can also be present in single-band Hubbard-like models: this is efficiently described by the `ancilla' method, which shows that the transition is a `flipped' Kondo lattice transition. This single-band FL*-FL transition is argued to apply to the metallic states of the hole-doped cuprates. In the clean limit, the critical properties of the quantum transitions in the three categories are distinct, but all lead to perfect metal transport in the quantum-critical regime. Impurity-induced `Harris disorder', with spatial fluctuations in the local position of the quantum critical point, is a relevant perturbation to the clean critical points. In the presence of Harris disorder, all three categories exhibit strange metal behavior, which can be described by a universal two-dimensional Yukawa-Sachdev-Ye-Kitaev model.

DOI
10.48550/arxiv.2407.15919

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Quantum phase transitions of metals involve changes in the Fermi surface, and can be divided into three categories. The first two categories involve symmetry breaking, and lead to a deformation or reconstruction of the Fermi surface. The third category involves a change in the volume enclosed by the Fermi surface without any symmetry breaking: one phase is a Fermi liquid (FL) with the conventional Luttinger volume, while the other phase is a fractionalized Fermi liquid' (FL*), which has a non-Luttinger volume Fermi surface accompanied by a spin liquid with fractionalized excitations. It is a relatively simple matter to obtain a FL*-FL transition in Kondo lattice models. However, the FL*-FL transition can also be present in single-band Hubbard-like models: this is efficiently described by the ancilla' method, which shows that the transition is a flipped' Kondo lattice transition. This single-band FL*-FL transition is argued to apply to the metallic states of the hole-doped cuprates. In the clean limit, the critical properties of the quantum transitions in the three categories are distinct, but all lead to perfect metal transport in the quantum-critical regime. Impurity-induced Harris disorder', with spatial fluctuations in the local position of the quantum critical point, is a relevant perturbation to the clean critical points. In the presence of Harris disorder, all three categories exhibit strange metal behavior, which can be described by a universal two-dimensional Yukawa-Sachdev-Ye-Kitaev model.
We describe a solvable model of a quantum transition in a single band model involving a change in the size of the electron Fermi surface without any symmetry breaking. In a model with electron density $1\ensuremath{-}p$, we find a ``large'' Fermi surface state with the conventional Luttinger volume $1\ensuremath{-}p$ of electrons for p>pcp>{p}_{c}p>pc​, and a first-order transition to a ``small'' Fermi surface state with a non-Luttinger volume ppp of holes for p<pcp<{p}_{c}p<pc​. As required by extended Luttinger theorems, the small Fermi surface state also has fractionalized spinon excitations. The model has electrons with strong local interactions in a single band; after a canonical transformation, the interactions are transferred to a coupling to two layers of ancilla qubits, as proposed by Zhang and Sachdev [Phys. Rev. Research 2, 023172 (2020)]. Solvability is achieved by employing random exchange interactions within the ancilla layers, and taking the large MMM limit with SU(M)\mathrm{SU}(M)SU(M) spin symmetry, as in the Sachdev-Ye-Kitaev models. The local electron spectral function of the small Fermi surface phase displays a particle-hole asymmetric pseudogap, and maps onto the spectral function of a lightly doped Kondo insulator of a Kondo-Heisenberg lattice model. We discuss connections to the physics of the hole-doped cuprates: the asymmetric pseudogap observed in STM, and the sudden change from incoherent to coherent antinodal spectra observed recently in photoemission. A holographic analogy to wormhole transitions between multiple black holes is briefly noted.
This modern text describes the remarkable developments in quantum condensed matter physics following the experimental discoveries of quantum Hall effects and high temperature superconductivity in the 1980s. After a review of the phases of matter amenable to an independent particle description, entangled phases of matter are described in an accessible and unified manner. The concepts of fractionalization and emergent gauge fields are introduced using the simplest resonating valence bond insulator with an energy gap, the Z2 spin liquid. Concepts in band topology and the parton method are then combined to obtain a large variety of experimentally relevant gapped states. Correlated metallic states are described, beginning with a discussion of the Kondo effect on magnetic impurities in metals. Metals without quasiparticle excitations are introduced using the Sachdev-Ye-Kitaev model, followed by a discussion of critical Fermi surfaces and strange metals. Numerous end-of-chapter problems expand readers' comprehension and reinforce key concepts.
Topology of the Fermi surface and universality of the metal-metal and metal-insulator transitions: ddd-dimensional Hatsugai-Kohmoto model as an example
The earlier theory [1] of the quantum phase transitions related to the change of the Fermi Surface Topology (FST) is advanced. For such transitions the Fermi surface as a quantum critical manifold determined by the Lee-Yang zeros, the order parameter P\mathcal{P}P as the ddd-volume of the Fermi sea, and the special FST universality class were introduced in [1]. The exactly solvable Hatsugai-Kohmoto (HK) ddd-dimensional (d=1,2,3d=1,2,3d=1,2,3) model of interacting fermions is analyzed. We explore the relation between the Lee-Yang zeros, the Luttinger and the plateau (Oshikawa) theorems. The validity of the Luttinger theorem in the HK model is confirmed. It is shown that the order parameter P\mathcal{P}P and the FST universality class describe the transitions between metal and band/Mott insulators, as well as the Lifshitz and van Hove gapless-to-gapless transitions. The gapless phases are established to be the Landau Fermi liquids (metals). In addition to the conventional paradigm with a continuous order parameter, we apply the homology theory to analyze the FST transitions. They are critical points of the Morse function. To quantify FST we use the Euler characteristic, which is calculated for each phase of the HK model. We claim that the FST universality class is robust with respect to interactions and other model details, under the condition that the critical points are non-degenerate.
The quantum phase transitions of metals have been extensively studied in the rare-earth "heavy electron" materials, the cuprates, and related compounds. The Fermi surface of the metal often has different shapes in the states well away from the critical point. It has been proposed that these differences can persist up to the critical point, setting up a discontinuous Fermi surface change across a continuous quantum transition. We study square lattice antiferromagnets undergoing a continuous transition from a Neel state to a valence bond solid, and examine the fate of a small density of holes in the two phases. Fermi surfaces of charge e, spin 1/2 quasiparticles appear in both phases, enclosing the usual Luttinger area. However, additional quantum numbers cause the area enclosed by each Fermi surface pocket to jump by a factor of 2 across the transition in the limit of small density. We demonstrate that the electronic spectrum across this transition is described by a critical theory of a localized impurity coupled to a 2+1 dimensional conformal field theory. This critical theory also controls the more complex Fermi surface crossover at fixed density, which likely involves intermediate phases with exotic fractionalized excitations. We suggest that such theories control the electronic spectrum in the pseudogap phase of the cuprates.
One of the fundamental questions about high-temperature cuprate superconductors is the size of the Fermi surface underlying the superconducting state. By analyzing the single-particle spectral function for the Fermi-Hubbard model as a function of repulsion UUU and chemical potential $\ensuremath{\mu}$, we find that the Fermi surface in the normal state undergoes a transition from a large Fermi surface matching the Luttinger volume as expected in a Fermi liquid, to a Fermi surface that encloses fewer electrons that we dub the ``Luttinger breaking'' phase, as the Mott insulator is approached. This transition into a non-Fermi-liquid phase that violates the Luttinger count occurs at a critical density in the absence of any other broken symmetry. We obtain the Fermi-surface contour from the spectral weight ${A}_{\mathbf{k}}(\ensuremath{\omega}=0)$ and from an analysis of the singularities of the Green's function ReGk(E=0)\mathrm{Re}\phantom{\rule{0.16em}{0ex}}{G}_{\mathbf{k}}(E=0)ReGk​(E=0), calculated using determinantal quantum Monte Carlo and analytic continuation methods. We discuss our numerical results in connection with experiments on Hall measurements, scanning tunneling spectroscopy, and angle-resolved photoemission spectroscopy.
I begin with a review of quantum impurity models in condensed matter physics, in which a localized spin degree of freedom is coupled to an interacting conformal field theory in \\(d\\) = 2 spatial dimensions. Their properties are similar to those of supersymmetric generalizations which can be solved by the AdS/CFT correspondence; the low energy limit of the latter models is described by a \\(AdS_2\\) geometry. Then I turn to Kondo lattice models, which can be described by a mean- field theory obtained by a mapping to a quantum impurity coupled to a self-consistent environment. Such a theory yields a 'fractionalized Fermi liquid' phase of conduction electrons coupled to a critical spin liquid state, and is an attractive mean-field theory of strange metals. The recent holographic description of strange metals with a \\(AdS_2 \\times R^2\\) geometry is argued to be related to such mean-field solutions of Kondo lattice models.