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arXiv:2407.12228 · Physical Review A

Variational approach to light-matter interaction: Bridging quantum and semiclassical limits

Yiying Yan, Zhiguo Lü, JunYan Luo

Published Jul 17, 2024• 2 citations
arXivHTMLPDF

Abstract

We present a time-dependent variational approach with the multiple-Davydov-${\text{D}}_{2}$ trial state to simulate the dynamics of light-matter systems when the field is initially in a coherent state with an arbitrary finite mean photon number. The variational approach captures not only the system dynamics but also the field dynamics and is applicable to a variety of quantum models of light-matter interaction such as the Jaynes-Cummings model, Rabi model, and Dicke model and is capable of tackling multimode quantized fields. With a comparison of the variational and semiclassical dynamics of both the system and field, we illustrate that the variational dynamics from the quantum models agrees with those from the corresponding semiclassical models as long as the mean number of photons is sufficiently large. Moreover, we illustrate that in the crossover between the quantum and semiclassical limits, the quantum corrections lead to the collapse of the oscillations in dynamics, which is absent in the semiclassical models. The variational approach provides a unified treatment of light-matter interaction from the quantum to the semiclassical limit.

DOI
10.1103/physreva.110.013706

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We present a time-dependent variational approach with the multiple-Davydov-D2{\text{D}}_{2}D2​ trial state to simulate the dynamics of light-matter systems when the field is initially in a coherent state with an arbitrary finite mean photon number. The variational approach captures not only the system dynamics but also the field dynamics and is applicable to a variety of quantum models of light-matter interaction such as the Jaynes-Cummings model, Rabi model, and Dicke model and is capable of tackling multimode quantized fields. With a comparison of the variational and semiclassical dynamics of both the system and field, we illustrate that the variational dynamics from the quantum models agrees with those from the corresponding semiclassical models as long as the mean number of photons is sufficiently large. Moreover, we illustrate that in the crossover between the quantum and semiclassical limits, the quantum corrections lead to the collapse of the oscillations in dynamics, which is absent in the semiclassical models. The variational approach provides a unified treatment of light-matter interaction from the quantum to the semiclassical limit.
The crossover from quantum to semiclassical behavior in the seminal Rabi model of light-matter interaction still, surprisingly, lacks a complete and rigorous understanding. A formalism for deriving the semiclassical model directly from the quantum Hamiltonian is developed here. Working in a displaced Fock-state basis |α,n⟩, the semiclassical limit is obtained by taking |α|→∞ and the coupling to zero. This resolves the discrepancy between coherent-state dynamics and semiclassical Rabi oscillations in both standard and ultrastrong coupling and driving regimes. Furthermore, it provides a framework for studying the quantum-to-semiclassical transition, with potential applications in quantum technologies.
Simulation of the interaction of light with matter, including at the few-photon level, is important for understanding the optical and optoelectronic properties of materials and for modeling next-generation nonlinear spectroscopies that use entangled light. At the few-photon level the quantum properties of the electromagnetic field must be accounted for with a quantized treatment of the field, and then such simulations quickly become intractable, especially if the matter subsystem must be modeled with a large number of degrees of freedom, as can be required to accurately capture many-body effects and quantum noise sources. Motivated by this we develop a quantum simulation framework for simulating such light-matter interactions on platforms with controllable bosonic degrees of freedom, such as vibrational modes in the trapped ion platform. The key innovation in our work is a scheme for simulating interactions with a continuum field using only a few discrete bosonic modes, which is enabled by a Green's function (response function) formalism. We develop the simulation approach, sketch how the simulation can be performed using trapped ions, and then illustrate the method with numerical examples. Our work expands the reach of quantum simulation to important light-matter interaction models and illustrates the advantages of extracting dynamical quantities such as response functions from quantum simulations.
We compare the semiclassical and quantum predictions for the unitary dynamics of a two-level atom interacting with a single-mode electromagnetic field under parametric modulation of the atomic parameters in the regime of multiphoton atom–field resonances. We derive approximate analytic solutions for the semiclassical Rabi model when the atomic transition frequency and the atom–field coupling strength undergo harmonic external modulations. These solutions are compared to the predictions of the quantum Rabi model, which we solve numerically for an initial coherent state with a large average photon number (on the order of 104), in the regime of three-photon resonance. We show that, for short enough times and sufficiently intense coherent states, the semiclassical dynamics agrees quite well with the quantum dynamics, although it inevitably fails at longer times due to the absence of collapse–revival behavior. Furthermore, we describe how the field state evolves throughout the interaction, presenting numerical results for the average photon number, entropies (related to atom–field entanglement), and other quantities characterizing the photon number statistics of the electromagnetic field.
Abstract In this chapter we study with the tools developed in Chapter 3 the basic models that are the foundations of light–matter interaction. We start with Rabi dynamics, then consider the optical Bloch equations that add phenomenologically the lifetime of the populations. As decay and pumping are often important, we cover the Lindblad form, a correct, simple and powerful way to describe various dissipation mechanisms. Then we go to a full quantum picture, quantizing also the optical field. We first investigate the simpler coupling of bosons and then culminate with the Jaynes–Cummings model and its solution to the quantum interaction of a two-level system with a cavity mode. Finally, we investigate a broader family of models where the material excitation operators differ from the ideal limits of a Bose and a Fermi field.
Many field states in quantum optics may be regarded as quasiclassical in that they possess a fairly well-defined phase and amplitude in the limit in which the average number of photons is large. Examples include coherent states and squeezed states that have a coherent component substantially larger than the squeezed noise contribution. For such states, calculations involving sums over the coefficients in the Fock-state basis can be considerably simplified in the limit of large photon number. The Jaynes-Cummings model and its extensions (to, e.g., three-level, two-mode configurations) may be advantageously studied from this perspective. New results on the three-level, two-mode problems, on the influence of cavity losses, and on the various time scales of interest will be presented here. The method typically identifies a set of privileged, long-lived atomic states, which lead to a quasiclassical evolution that agrees with the prediction of semiclassical treatments over a characteristic time scale; linear combinations of the long-lived states, on the other hand, become superpositions of macroscopically distinct states in time and result in an evolution that exhibits many uniquely quantum effects.
Polaritonic chemistry has ushered in new avenues for controlling molecular dynamics. However, two key questions remain: (i) Can classical light sources elicit the same effects as certain quantum light sources on molecular systems? (ii) Can semiclassical treatments of light-matter interaction capture nontrivial quantum effects observed in molecular dynamics? This work presents a quantum-classical approach addressing issues of realizing cavity chemistry effects without actual cavities. It also highlights the limitations of the standard semiclassical light-matter interaction. It is demonstrated that classical light sources can mimic quantum effects up to the second order of light-matter interaction, provided that the mean-field contribution, symmetrized two-time correlation function, and the linear response function are the same in both situations. Numerical simulations show that the quantum-classical method aligns more closely with exact quantum molecular-only dynamics for quantum light states such as Fock states, superpositions of Fock states, and vacuum squeezed states than the conventional semiclassical approach.