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arXiv:2407.01133

Chiral Quantum-Optical Elements for Waveguide-QED with Sub-wavelength Rydberg-Atom Arrays

Lida Zhang, Fan Yang, Klaus Mølmer, Thomas Pohl

Published Jul 1, 2024• 1 citation
arXivHTMLPDF

Abstract

We describe an approach to achieve near-perfect unidirectional light-matter coupling to an effective quantum emitter that is formed by a subwavelength array of atoms in the Rydberg-blockade regime. The nonlinear reflection and transmission of such two-dimensional superatoms are exploited in different interferometric setups for the deterministic generation of tunable single photons and entangling two-photon operations with high fidelities, $\mathcal{F}\gtrsim0.999$. The described setup can function as a versatile nonlinear optical element in a free-space photonic quantum network with simple linear elements and without the need of additional mode confinement, optical resonators, or optical isolators.

DOI
10.48550/arxiv.2407.01133

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We describe an approach to achieve near-perfect unidirectional light-matter coupling to an effective quantum emitter that is formed by a subwavelength array of atoms in the Rydberg-blockade regime. The nonlinear reflection and transmission of such two-dimensional superatoms are exploited in different interferometric setups for the deterministic generation of tunable single photons and entangling two-photon operations with high fidelities, F≳0.999\mathcal{F}\gtrsim0.999F≳0.999. The described setup can function as a versatile nonlinear optical element in a free-space photonic quantum network with simple linear elements and without the need of additional mode confinement, optical resonators, or optical isolators.
We describe an approach to achieve near-perfect unidirectional light–matter coupling to an effective quantum emitter that is formed by a subwavelength array of atoms in the Rydberg-blockade regime. The nonlinear reflection and transmission of such two-dimensional superatoms are exploited in different interferometric setups for the deterministic generation of tunable single photons and entangling two-photon operations with high fidelities, F ≳0.999. The described setup can function as a versatile nonlinear optical element in a free-space photonic quantum network with simple linear elements and without the need of additional mode confinement, optical resonators, or optical isolators.
Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
The scattering between light and individual saturable quantum emitters can induce strong optical nonlinearities and correlations between individual light quanta. Typically, this leads to an effective attraction that can generate exotic bound states of photons, which form quantum mechanical precursors of optical solitons, as found in many optical media. Here, we study the propagation of light through an optical waveguide that is chirally coupled to three-level quantum emitters. We show that the additional laser coupling to a third emitter state not only enables control of the properties of the bound state but can even eliminate it entirely. This makes it possible to turn an otherwise focusing nonlinearity into a repulsive photon-photon interaction. We demonstrate this emerging photon-photon repulsion by analyzing the quantum dynamics of multiple photons in large emitter arrays and reveal a dynamical fragmentation of incident uncorrelated light fields and self-ordering into regular trains of single photons. These striking effects expand the rich physics of waveguide quantum electrodynamics into the domain of repulsive photons and establish a conceptually simple platform to explore optical self-organization phenomena at the quantum level. We discuss implementations of this setting in cold-atom experiments and propose an approach based on arrays of mesoscopic Rydberg-atom ensembles.
We propose the combination of subwavelength, two-dimensional atomic arrays and Rydberg interactions as a powerful platform to realize strong, coherent interactions between individual photons with high fidelity. The atomic spatial ordering guarantees efficient atom-light interactions without the possibility of scattering light into unwanted directions, allowing the array to act as a perfect mirror for individual photons. In turn, Rydberg interactions enable single photons to alter the optical response of the array within a potentially large blockade radius R_{b}, which can effectively punch a large "hole" for subsequent photons. We show that such a system enables a coherent photon-photon gate or switch, with a significantly better error scaling (∼R_{b}^{-4}) than in a disordered ensemble. We also investigate the optical properties of the system in the limit of strong input intensities and show that this many-body quantum driven dissipative system can be modeled well by a semiclassical model based on holes punched in a classical mirror.
Enhancing light-matter coupling at the level of single quanta is essential for numerous applications in quantum science. The cooperative optical response of subwavelength atomic arrays has been found to open new pathways for such strong light-matter couplings, while simultaneously offering access to multiple spatial modes of the light field. Efficient single-mode free-space coupling to such arrays has been reported, but the spatial control over the modes of outgoing light fields has remained elusive. Here, we demonstrate such spatial control over the optical response of an atomically thin mirror formed by a subwavelength array of atoms in free space using a single controlled ancilla atom excited to a Rydberg state. The switching behavior is controlled by the admixture of a small Rydberg fraction to the atomic mirror, and consequently strong dipolar Rydberg interactions with the ancilla. Driving Rabi oscillations on the ancilla atom, we demonstrate coherent control of the transmission and reflection of the array. These results represent a step towards the realization of quantum coherent metasurfaces, the demonstration of controlled atom-photon entanglement and deterministic engineering of quantum states of light.