Levitated nanoparticles provide a controllable and isolated platform for probing fundamental quantum phenomena at the macroscopic scale. In this work we introduce an optimization method to determine optimal static potentials for the generation of largely delocalized and non-Gaussian quantum states of levitated nanoparticles. Our optimization strategy accounts for position-dependent noise sources originating from the fluctuations of the potential. We provide key figures of merit that allow for fast computation and capture relevant features of the dynamics, mitigating the computational demands associated with the multiscale simulation of this system. Specifically, we introduce coherence length and coherent cubicity as signatures of large delocalization and quantum non-Gaussian states, respectively. As a proof of principle, we apply the optimization approach to a family of quartic potentials and show that the optimal configuration depends on the strength and nature of the noise in the system. Additionally, we benchmark our results with a full quantum dynamics simulations of the system for the optimal potentials.
Levitated nanoparticles provide a controllable and isolated platform for probing fundamental quantum phenomena at the macroscopic scale. In this work we introduce an optimization method to determine optimal static potentials for the generation of largely delocalized and non-Gaussian quantum states of levitated nanoparticles. Our optimization strategy accounts for position-dependent noise sources originating from the fluctuations of the potential. We provide key figures of merit that allow for fast computation and capture relevant features of the dynamics, mitigating the computational demands associated with the multiscale simulation of this system. Specifically, we introduce coherence length and coherent cubicity as signatures of large delocalization and quantum non-Gaussian states, respectively. As a proof of principle, we apply the optimization approach to a family of quartic potentials and show that the optimal configuration depends on the strength and nature of the noise in the system. Additionally, we benchmark our results with a full quantum dynamics simulations of the system for the optimal potentials.
We propose to optimally control the harmonic potential of a levitated nanoparticle to quantum delocalize its center-of-mass motional state to a length scale orders of magnitude larger than the quantum zero-point motion. Using a bang-bang control of the harmonic potential, including the possibility of inverting it, the initial ground-state-cooled levitated nanoparticle coherently expands to large scales and then contracts to the initial state in a time-optimal way. We show that this fast loop protocol can be used to enhance force sensing as well as to dramatically boost the entangling rate of two weakly interacting nanoparticles. We parameterize the performance of the protocol, and therefore the macroscopic quantum regime that could be explored, as a function of displacement and frequency noise in the nanoparticle's center-of-mass motion. This noise analysis accounts for the sources of decoherence relevant to current experiments.
Realizing quantum superpositions of massive objects provides a pathway to explore the quantum-to-classical transition. Levitated nanoparticles appear as a promising platform for this purpose due to their large mass and unbound motion. This thesis follows the proposal that particle evolution in a double-well potential expands the particle’s motional state within an inverted harmonic region, while the quartic potential generates the non-Gaussian states needed to certify quantum delocalization. As this protocol has been recently developed, we perform experiments in the classical regime as an important milestone to identify the technical challenges and the decoherence sources. While the nanoparticle’s motional state grows linearly under free evolution, inverted harmonic potentials offer exponentially accelerated state expansion. In this thesis, we experimentally demonstrate the expansion of the center-of-mass state of a 125 nm silica nanoparticle from an initial position uncertainty of 45.6 pm to 43.4 nm within 260 μs. This expansion represents a 952-fold increase, reaching a state size comparable to the particle’s radius, and is achieved by employing an electrostatic inverted potential to disable decoherence from photon recoil. The incoherent dynamics allow us to estimate the remaining decoherence sources in the dark. To accomplish dark dynamics, we developed two segmented linear Paul trap devices providing 2D confinement while generating DC potentials in the third axis of motion: a planar micro-fabricated chip and a PCB based wheel trap. Simulations of tunable double-well potentials of tens to hundreds of micrometers based on the device layouts are performed alongside a study of the resulting classical non-Gaussian states. This work marks a key advancement in the effort to generate macroscopic quantum superpositions at unprecedented mass and length scales.
Abstract Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules [1, 2]. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself [3]. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances [4–7]. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments [8], and towards quantum-enhanced force sensing with levitated particles [9].
Levitated high-mass quantum systems provide access to unprecedented regimes in both fundamental science and technological applications. However, deterministic generation and manipulation of quantum non-Gaussian states, which are central to many continuous-variable quantum advantages, remain elusive in such platforms. In this work, we propose a theoretical protocol for preparing a continuous-variable degree of freedom of a levitated massive object in a variety of quantum states, including Fock and Schrödinger cat states, without coupling to auxiliary two-level systems. Our approach enhances otherwise weak nonharmonic effects by transient wave-function delocalization and combines this with optimal control of the potential. Specifically, time-dependent modulation of the linear component of the potential, in the presence of a static cubic nonharmonicity, provides a route to universal control of the mode. We analyze quantum state preparation under such control and estimate the required nonharmonicity, motional delocalization, and maximum tolerable decoherence for generating target non-Gaussian states. The proposed optimal-control scheme can also be readily extended beyond single-particle state preparation, for example, to unitary transformations and nonlinear measurements. As a concrete example, we demonstrate mechanical Bell-state preparation for two interacting particles using only local modulation of weakly nonharmonic potentials, while the interparticle interaction remains effectively linear. We emphasize that the protocols presented here apply to different mechanical degrees of freedom, such as center-of-mass motion and libration, and can also be implemented in other weakly nonharmonic systems with a leading cubic nonharmonicity.
Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments, and towards quantum-enhanced force sensing with levitated particles.
Optically levitated nanoparticles are promising candidates for the generation of macroscopic quantum states of mechanical motion. Protocols to generate such states expose the particle to a succession of different potentials. Limited reproducibility of the alignment of these potentials across experimental realizations introduces additional noise. Here, we experimentally investigate and model how such shot-to-shot noise limits the coherence length of a levitated nanoparticle during a state-expansion protocol using a dark, inverted electrical potential. We identify electric stray fields and mechanical instabilities as major sources of shot-to-shot fluctuations. We discuss the resulting experimental requirements for state expansion protocols exploiting inverted potentials.