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arXiv:2406.19372 · Physical review. B./Physical review. B

Refined phase diagram for a spin-1 system exhibiting a Haldane phase

Mohamad Mousa, Birgit Wehefritz–Kaufmann, Sabre Kais, Shawn Xingshan Cui, Ralph M. Kaufmann

Published Feb 18, 2025• 2 citations
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Abstract

We provide the phase diagram of a two-parameter spin-1 chain that has a symmetry-protected topological (SPT) Haldane phase using computational algorithms along with tensor-network tools. We improve previous results, showing the existence of a new phase and new triple points. New striking features are the triple end of the Haldane phase and the complexity of phases bordering the Haldane phase in proximity---allowing moving to nearby non-SPT phases via small perturbations. These characteristics make the system, which appears in Rydberg excitons, e.g., in ${\mathrm{Cu}}_{2}\mathrm{O}$, a prime candidate for applications.

DOI
10.1103/physrevb.111.085303

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We provide the phase diagram of a two-parameter spin-1 chain that has a symmetry-protected topological (SPT) Haldane phase using computational algorithms along with tensor-network tools. We improve previous results, showing the existence of a new phase and new triple points. New striking features are the triple end of the Haldane phase and the complexity of phases bordering the Haldane phase in proximity---allowing moving to nearby non-SPT phases via small perturbations. These characteristics make the system, which appears in Rydberg excitons, e.g., in Cu2O{\mathrm{Cu}}_{2}\mathrm{O}Cu2​O, a prime candidate for applications.
We present a protocol to implement a spin-1 chain in Rydberg systems using three Rydberg states close to a Förster resonance. In addition to dipole-dipole interactions, strong van der Waals interactions naturally appear due to the presence of the Förster resonance and give rise to a highly tunable Hamiltonian. The resulting phase diagram is studied using the infinite density-matrix renormalization group and reveals a highly robust Haldane phase—a prime example of a symmetry-protected topological phase. We find experimentally accessible parameters to probe the Haldane phase in current Rydberg systems, and demonstrate an efficient adiabatic preparation scheme. This paves the way to probe the remarkable properties of spin fractionalization in the Haldane phase.
We study the phase diagram of the SOq(3){\text{SO}}_{q}(3)SOq​(3) quantum group invariant spin-1 bilinear-biquadratic spin chain for real values of q>1q>1q>1. Numerical computations suggest that the chain has at least three clearly distinguished phases: A chiral analog of the Haldane phase, a dimerized phase, and a ferromagnetic phase. In contrast, the counterpart of the extended critical region that is known to exist for q=1q=1q=1 remains elusive. Our results show that the Haldane phase fails to exhibit a twofold degeneracy in the entanglement spectrum but that the degeneracy is restored upon a suitable qqq deformation of the entanglement Hamiltonian, which can be interpreted as a Zeeman field. The structure of the phase diagram is confirmed through analytical calculations in the extreme anisotropic limit $q\ensuremath{\rightarrow}\ensuremath{\infty}$. Our results suggest that symmetries of the form Uq[su(2)]{\mathcal{U}}_{q}\left[su(2)\right]Uq​[su(2)] for distinct choices of qqq should be interpreted as one single family instead of separate symmetries when defining SPT phases, leading naturally to the notion of a qqq-SPT phase.
Spin-1/2 two-legged ladders respecting interleg exchange symmetry $\ensuremath{\sigma}$ and spin rotation symmetry D2{D}_{2}D2​ have new symmetry-protected topological (SPT) phases which are different from the Haldane phase. Three of the new SPT phases are tx,ty,tz{t}_{x},{t}_{y},{t}_{z}tx​,ty​,tz​, which all have symmetry-protected twofold degenerate edge states on each end of an open chain. However, the edge states in different phases have different responses to magnetic field. For example, the edge states in the tz{t}_{z}tz​ phase will be split by the magnetic field along the zzz direction, but not by the fields in the xxx and yyy directions. We give the Hamiltonian that realizes each SPT phase and demonstrate a proof-of-principle quantum simulation scheme for Hamiltonians of the t0{t}_{0}t0​ and tz{t}_{z}tz​ phases based on the coupled-QED-cavity ladder.
Chiral Haldane phases are examples of one-dimensional topological states of matter which are protected by the projective SU(N)\mathrm{SU}(N)SU(N) group (or its subgroup ${\mathbb{Z}}_{N}\ifmmode\times\else\texttimes\fi{}{\mathbb{Z}}_{N})$ with N>2N>2N>2. The unique feature of these symmetry-protected topological (SPT) phases is that they are accompanied by inversion-symmetry breaking and the emergence of different left and right edge states which transform, for instance, respectively in the fundamental $(\mathbit{N})$ and antifundamental $(\overline{\mathbit{N}})$ representations of SU(N)\mathrm{SU}(N)SU(N). We show, by means of complementary analytical and numerical approaches, that these chiral SPT phases as well as the nonchiral ones are realized as the ground states of a generalized two-leg SU(N)\mathrm{SU}(N)SU(N) spin ladder in which the spins in the first chain transform in $\mathbit{N}$ and the second in $\overline{\mathbit{N}}$. In particular, we map out the phase diagram for N=3N=3N=3 and 4 to show that all the possible symmetry-protected topological phases with projective SU(N)\mathrm{SU}(N)SU(N) symmetry appear in this simple ladder model.
It is well known that the Haldane phase of a one-dimensional spin-1 chain is a symmetry-protected topological (SPT) phase, which is described by a nonlinear sigma model (NLSM) with a $\ensuremath{\Theta}$ term at $\ensuremath{\Theta}=2\ensuremath{\pi}$. In this work we study a three-dimensional (3d) SPT phase of a SU(2NNN) antiferromagnetic spin system with a self-conjugate representation on every site. The spin-ordered N\'eel phase of this system has a ground state manifold $\mathcal{M}=\frac{\mathrm{U}(2N)}{\mathrm{U}(N)\ifmmode\times\else\texttimes\fi{}\mathrm{U}(N)}$, and this system is described by a NLSM defined with manifold M\mathcal{M}M. Since the homotopy group ${\ensuremath{\pi}}_{4}[\mathcal{M}]=\mathbb{Z}$ for N>1N>1N>1, this NLSM can naturally have a $\ensuremath{\Theta}$ term. We will argue that when $\ensuremath{\Theta}=2\ensuremath{\pi}$ this NLSM describes a SPT phase. This SPT phase is protected by the SU(2NNN) spin symmetry, or its subgroup SU(NNN)$\ifmmode\times\else\texttimes\fi{}$SU$(N)\ensuremath{\rtimes}{Z}_{2}$, without assuming any other discrete symmetry. We will also construct a trial SU(2NNN) spin state on a 3d lattice; we argue that the long-wavelength physics of this state is precisely described by the aforementioned NLSM with $\ensuremath{\Theta}=2\ensuremath{\pi}$.
We review the basic properties of the Haldane phase in spin-1 Heisenberg antiferromagnetic chains, including its persistence in quasi-one-dimensional (Q1D) geometries. Using large-scale numerical simulations, we map out the phase diagram for a realistic model applicable to experimental Haldane compounds. We also investigate the effect of different chain coupling geometries and confirm a general mean-field universality of the critical coupling times the coordination number of the lattice. Inspired by recent developments in the characterization of symmetry protected topological (SPT) states, of which the Haldane phase of the spin-1 Heisenberg antiferromagnetic chain is a preeminent example, we provide direct evidence that the Q1D Haldane phase is indeed a nontrivial SPT state.