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arXiv:2406.19168 · Physical Review Research

Emergent limit cycles, chaos, and bistability in driven-dissipative atomic arrays

Victoria Zhang, Stefan Ostermann, Oriol Rubies-Bigordà, Susanne F. Yelin

Published Feb 10, 2025• 4 citations
arXivHTMLPDF

Abstract

We analyze the driven-dissipative dynamics of subwavelength periodic atomic arrays in free space, where atoms interact via light-induced dipole-dipole interactions. We find that depending on the system parameters, the underlying mean-field model allows four different types of dynamics at late times: a single monostable steady state solution, bistability (where two stable steady state solutions exist), limit cycles and chaotic dynamics. We provide conditions on the parameters required to realize the different solutions in the thermodynamic limit. In this limit, only the monostable or bistable regime can be accessed for the parameter values accessible via light-induced dipole-dipole interactions. For finite size periodic arrays, however, we find that the mean-field dynamics of the many-body system also exhibit limit cycles and chaotic behavior. Notably, the emergence of chaotic dynamics does not rely on the randomness of an external control parameter but arises solely due to the interplay of coherent drive and dissipation.

DOI
10.1103/physrevresearch.7.013144

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We study the quantum dynamics of many-body arrays of two-level atoms in a driven cavity subject to collective decay and interactions mediated by the cavity field. We work in the bad cavity limit accessible, for example, using long-lived electronic clock states of alkaline-earth atoms, for which the bare atomic linewidth is much less than the cavity linewidth. In the absence of interactions, our system reduces to previously studied models of collective fluorescence. We show that while interactions do not qualitatively change the steady-state properties they lead to a drastic change in the dynamical properties. We find that, for some intervals of driving strengths, the system shows two very distinct types of transient behaviors that depend on the initial state of the system. In particular, there is a parameter regime where the system features oscillatory dynamics with a period of oscillation that becomes much shorter than the duration of the overall transient dynamics as the atom number increases. We use both mean-field and exact numerical calculations of the quantum system to investigate the dynamics.
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In recent years, the control of photon-photon interactions in optical nonlinear media has led to the realization of quantum fluids of light. One of the current challenges is to increase the strength of these interactions and enter the so-called strongly correlated regime. To achieve this goal, arrays of nonlinear cavities are a very promising candidate. In this thesis, theoretical results on arrays of nonlinear cavities described by a driven-dissipative Bose-Hubbard model are presented. In particular, a general method to compute the mean-field phase diagram of this model is described. Due to the finite life time of photons, the system is intrinsically dissipative: cavity losses must be compensated by an external driving field. This nonequilibrium nature gives rise to interesting features, such as a transition between monostable and bistable phases induced by tunneling. In the limit of weak dissipation and weak driving, analytical results describing generalized Mott insulating phases are derived. These states survive up to a critical tunneling strength, above which a crossover to a classical coherent state takes place. Finally, the issue of how to go beyond the mean-field approximation is addressed by performing exact numerical simulations. Large arrays of cavities were simulated by implementing a new method specifically tailored for driven-dissipative systems.
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Recent experimental advances in the field of cold-atom cavity QED provide a powerful tool for exploring nonequilibrium correlated quantum phenomena beyond conventional condensed-matter scenarios. We present the dynamical phase diagram of a driven Bose-Einstein condensate coupled with the light field of a cavity, with a transverse driving field red-detuned from atomic resonance. We identify regions in parameter space showing dynamical instabilities in the form of limit cycles, which evolve into chaotic behavior in the strong driving limit. Such limit cycles originate from the interplay between cavity dissipation and atom-induced resonance frequency shift, which modifies the phase of cavity mode and gives excessive negative feedback on the atomic density modulation, leading to instabilities of the superradiant scattering. We find interesting merging of the limit cycles related by a Z2{Z}_{2}Z2​ symmetry, and identify a limit cycle formed by purely atomic excitations. The effects of quantum fluctuations and atomic interactions are also investigated.