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arXiv:2406.18362 · Nature Communications

Non-Markovian quantum exceptional points

Jhen-Dong Lin, Po-Chen Kuo, Neill Lambert, Adam Miranowicz, Franco Nori, Yueh-Nan Chen

Published Feb 3, 2025• 38 citations
arXivHTMLPDF

Abstract

Exceptional points (EPs) are singularities in the spectra of non-Hermitian operators where eigenvalues and eigenvectors coalesce. Open quantum systems have recently been explored as EP testbeds due to their non-Hermitian nature. However, most studies focus on the Markovian limit, leaving a gap in understanding EPs in the non-Markovian regime. This work addresses this gap by proposing a general framework based on two numerically exact descriptions of non-Markovian dynamics: the pseudomode equation of motion (PMEOM) and the hierarchical equations of motion (HEOM). The PMEOM is particularly useful due to its Lindblad-type structure, aligning with previous studies in the Markovian regime while offering deeper insights into EP identification. This framework incorporates non-Markovian effects through auxiliary degrees of freedom, enabling the discovery of additional or higher-order EPs that are inaccessible in the Markovian regime. We demonstrate the utility of this approach using the spin-boson model and linear bosonic systems. The full description of exceptional points in the non-Markovian regime is complicated by the unclear applicability of standard techniques such as spectral analysis. Here, the authors fill this gap by proposing a general framework that combines the pseudomode equation of motion and the hierarchical equations of motion.

DOI
10.1038/s41467-025-56242-w

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Exceptional points (EPs) are singularities in the spectra of non-Hermitian operators where eigenvalues and eigenvectors coalesce. Open quantum systems have recently been explored as EP testbeds due to their non-Hermitian nature. However, most studies focus on the Markovian limit, leaving a gap in understanding EPs in the non-Markovian regime. This work addresses this gap by proposing a general framework based on two numerically exact descriptions of non-Markovian dynamics: the pseudomode equation of motion (PMEOM) and the hierarchical equations of motion (HEOM). The PMEOM is particularly useful due to its Lindblad-type structure, aligning with previous studies in the Markovian regime while offering deeper insights into EP identification. This framework incorporates non-Markovian effects through auxiliary degrees of freedom, enabling the discovery of additional or higher-order EPs that are inaccessible in the Markovian regime. We demonstrate the utility of this approach using the spin-boson model and linear bosonic systems. The full description of exceptional points in the non-Markovian regime is complicated by the unclear applicability of standard techniques such as spectral analysis. Here, the authors fill this gap by proposing a general framework that combines the pseudomode equation of motion and the hierarchical equations of motion.
One of the most remarkable features that distinguish open systems from closed ones is the presence of exceptional points (EPs), where two or more eigenvectors of a non-Hermitian operator coalesce, accompanying the convergence of the corresponding eigenvalues. So far, EPs have been demonstrated on a number of platforms, ranging from classical optical systems to fully quantum-mechanical spin-boson models. In these demonstrations, the reservoir that induced the non-Hermiticity was treated as a Markovian one, without considering its memory effect. We here present the first experimental demonstration of non-Markovian quantum EPs, engineered by coupling a Josephson-junction-based qubit to a leaky electromagnetic resonator, which acts as a non-Markovian reservoir. We map out the spectrum of the extended Liouvillian superoperator by observing the quantum state evolution of the qubit and the pseudomode, in which the memory of the reservoir is encoded. We identify a twofold second-order EP and a third-order EP in the Liouvillian spectrum, which cannot be realized with a Markovian reservoir. Our results pave the way for experimental exploration of exotic phenomena associated with non-Markovian quantum EPs.
The primary pathway to the investigation of exceptional points (EPs) in open quantum systems has been the use of Markovian master equations. However, recently it has been realised that they can arise in settings that show non-Markovian behaviour. The main approach in this direction has been the use of pseudomodes, which allow the influence of a structured environment to be replaced by new damped auxiliary modes. In this work, we use a Heisenberg-equation approach which relies on the reaction-coordinate formalism to obtain exact analytical dynamics. First, we show how our method considerably simplifies the analysis compared to the use of master equations. Second, we utilise it to discuss non-Markovian revivals in systems with second and higher-order EPs, showing that the notion that EPs demarcate the onset of revivals is not generally true. We then utilise our results to discuss the dynamical effects of higher-order non-Markovian EPs, deriving bounds on the number of revivals and investigating enhanced asymptotic relaxation near higher-order EPs. Finally, we investigate non-Markovian EPs with engineered reservoirs and show how they can be utilised to control the rate of irreversible information loss.
Abstract Exceptional points (EPs) occur in non-Hermitian systems where eigenvalues and eigenvectors coalesce. In open quantum systems, EPs are typically studied via non-Hermitian effective Hamiltonians or Liouvillians, but these omit the full generality of quantum dynamics, which requires description using quantum channels. Here, we introduce a general strategy for generating quantum-channel EPs in the single-qubit setting. We show that quantum channels naturally fall into two distinct phases, purely real or complex-conjugate eigenvalues, without the need of enforcing additional symmetries, and interpolating between different phases induces a phase transition where EPs can emerge. We experimentally simulate such channels on a nuclear magnetic resonance quantum computer, observing second-order quantum-channel EPs with 93% fidelity, and extend the approach to three channels to uncover exceptional lines and a third-order quantum-channel EP. Our results promise potential applications from enhanced quantum sensing to quantum control, such as Jordan-chain mediated asymmetric conversion.
Open photonic systems provide a versatile platform for non-Hermitian physics, enabling control over complex spectra, transport, and light-matter interactions. Exceptional points (EPs), at which eigenvalues and eigenvectors coalesce and the governing operator becomes defective, play a central role because they combine branch-point spectral topology, nonanalytic perturbative response, and controllable eigenstate conversion. This Review provides a unified framework for EP photonics by systematically distinguishing exceptional degeneracies according to the underlying operator, spectral variable, boundary conditions, and experimentally accessible observables. We discuss Hamiltonian EPs, absorbing EPs associated with scattering zeros, real-frequency scattering-matrix and Jones-matrix EPs, Bloch and Floquet EPs, and Liouvillian EPs in open quantum systems. We review their spectral topology, static and dynamical encircling, higher-order exceptional structures, and coexistence with bound states in the continuum, together with applications in sensing, lasing, coherent absorption, directional scattering, polarization and wavefront control, nonlinear optics, optical storage, nonreciprocal photonics, and quantum photonics. We also critically assess the current limitations, practical challenges, and future perspectives of EP-based photonic technologies, with particular attention to robustness, noise, scalability, and experimentally measurable performance.
Exceptional points (EPs) occur in non-Hermitian systems where eigenvalues and eigenvectors coalesce. In open quantum systems, EPs are typically studied via non-Hermitian effective Hamiltonians or Liouvillians, but these omit the full generality of quantum dynamics, which requires description using quantum channels. Here, we introduce a general strategy for generating quantum-channel EPs in the single-qubit setting. We show that quantum channels naturally fall into two distinct phases, purely real or complex-conjugate eigenvalues, without the need of enforcing additional symmetries, and interpolating between different phases induces a phase transition where EPs can emerge. We experimentally simulate such channels on a nuclear magnetic resonance quantum computer, observing second-order quantum-channel EPs with 93% fidelity, and extend the approach to three channels to uncover exceptional lines and a third-order quantum-channel EP. Our results promise potential applications from enhanced quantum sensing to quantum control, such as Jordan-chain mediated asymmetric conversion.
Exceptional points (EPs) are the spectral singularities and one of the central concepts of non-Hermitian physics, originating from the inevitable energy exchange with the surrounding environment. EPs exist in diverse physical systems and give rise to many counterintuitive effects, offering rich opportunities to control the dynamics and alter the properties of optical, electronic, acoustic, and mechanical states. The last two decades have witnessed the flourishing of non-Hermitian physics and associated applications related to coalesced eigenstates at EPs in a plethora of classical systems. While stemming from the quantum mechanism, the implementation of EPs in real quantum systems still faces challenges of tuning and stabilizing the systems at EPs, as well as the additional noises that hinder the observation of relevant phenomena. This review mainly focuses on summarizing the current efforts and opportunities offered by quantum EPs that result from or produce observable quantum effects. We introduce the concepts of Hamiltonian and Liouvillian EPs in the quantum regime and focus on their different properties in connection with quantum jumps and decoherence. We then provide a comprehensive discussion covering the theoretical and experimental advances in accessing EPs in diverse quantum systems and platforms. Special attention is paid to EP-based quantum-optics applications with state-of-art technologies. Finally, we present a discussion on the existing challenges of constructing quantum EPs at the nanoscale and an outlook on the fundamental science and applied technologies of quantum EPs, aiming to provide valuable insights for future research and building quantum devices with high performance and advanced functionalities.