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arXiv:2406.18348 · Physical Review Letters

Quantum Speed Limit in Quantum Sensing

Konstantin Herb, Christian L. Degen

Published Nov 19, 2024• 20 citations
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Abstract

Quantum sensors capitalize on advanced control sequences for maximizing sensitivity and precision. However, protocols are not usually optimized for temporal resolution. Here, we establish the limits for time-resolved sensing of dynamical signals using qubit probes. We show that the best possible time resolution is closely related to the quantum speed limit (QSL), which describes the minimum time needed to transform between basis states. We further show that a composite control sequence consisting of two phase-shifted pulses reaches the QSL. Practical implementation is discussed based on the example of the spin-1 qutrit of a nitrogen-vacancy center in diamond.

DOI
10.1103/physrevlett.133.210802

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Quantum sensors capitalize on advanced control sequences for maximizing sensitivity and precision. However, protocols are not usually optimized for temporal resolution. Here, we establish the limits for time-resolved sensing of dynamical signals using qubit probes. We show that the best possible time resolution is closely related to the quantum speed limit (QSL), which describes the minimum time needed to transform between basis states. We further show that a composite control sequence consisting of two phase-shifted pulses reaches the QSL. Practical implementation is discussed based on the example of the spin-1 qutrit of a nitrogen-vacancy center in diamond.
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Quantum mechanics establishes a fundamental bound for the minimum evolution time between two states of a given system. Known as the quantum speed limit (QSL), it is a useful tool in the context of quantum control, where the speed of some control protocol is usually intended to be as large as possible. While QSL expressions for time-independent Hamiltonians have been well studied, the time-dependent regime has remained somewhat unexplored, albeit being usually the relevant problem to be compared with when studying systems controlled by external fields. In this paper we explore the relation between optimal times found in quantum control and the QSL bound, in the (relevant) time-dependent regime, by discussing the ubiquitous two-level Landau-Zener–type Hamiltonian.
Quantum mechanics establishes a fundamental bound for the minimum evolution time between two states of a given system. Known as the quantum speed limit (QSL), it is a useful tool in the context of quantum control, where the speed of some control protocol is usually intended to be as large as possible. While QSL expressions for time-independent Hamiltonians have been well studied, the time-dependent regime has remained somewhat unexplored, albeit being usually the relevant problem to be compared with when studying systems controlled by external fields. In this paper we explore the relation between optimal times found in quantum control and the QSL bound, in the (relevant) time-dependent regime, by discussing the ubiquitous two-level Landau-Zener-type Hamiltonian.
The notion of a quantum speed limit (QSL) refers to the fundamental fact that two quantum states become completely distinguishable upon dynamical evolution only after a finite amount of time, called the QSL time. A different but related concept is that of minimum control time (MCT), which is the minimum evolution time needed for a state to be driven (by suitable, generally time-dependent, control fields) to a given target state. While the QSL can give information about the MCT, it usually imposes little restrictions on it and is thus impractical for control purposes. In this work, we revisit this issue by first presenting a theory of geometrical QSL for unitary transformations, rather than for states, and discuss its implications and limitations. Then, we propose a framework for bounding the MCT for realizing unitary transformations that goes beyond the QSL results and gives much more meaningful information to understand the controlled dynamics of the system at short times.
Recent advances in engineering and control of nanoscale quantum sensors have opened new paradigms in precision metrology. Unfortunately, hardware restrictions often limit the sensor performance. In nanoscale magnetic resonance probes, for instance, finite sampling times greatly limit the achievable sensitivity and spectral resolution. Here we introduce a technique for coherent quantum interpolation that can overcome these problems. Using a quantum sensor associated with the nitrogen vacancy center in diamond, we experimentally demonstrate that quantum interpolation can achieve spectroscopy of classical magnetic fields and individual quantum spins with orders of magnitude finer frequency resolution than conventionally possible. Not only is quantum interpolation an enabling technique to extract structural and chemical information from single biomolecules, but it can be directly applied to other quantum systems for superresolution quantum spectroscopy.
In quantum sensing, precision is typically limited by the maximum time interval over which phase can be accumulated. Memories have been used to enhance this time interval beyond the coherence lifetime and thus gain precision. Here, we demonstrate that by using a quantum memory an increased sensitivity can also be achieved. To this end, we use entanglement in a hybrid spin system comprising a sensing and a memory qubit associated with a single nitrogen-vacancy centre in diamond. With the memory we retain the full quantum state even after coherence decay of the sensor, which enables coherent interaction with distinct weakly coupled nuclear spin qubits. We benchmark the performance of our hybrid quantum system against use of the sensing qubit alone by gradually increasing the entanglement of sensor and memory. We further apply this quantum sensor-memory pair for high-resolution NMR spectroscopy of single (13)C nuclear spins.