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arXiv:2406.17439 · Optics Express

Efficient generation of broadband photon pairs in shallow-etched lithium niobate nanowaveguides

Xiao‐Xu Fang, Leiran Wang, He Lu

Published May 30, 2024• 19 citations
arXivHTMLPDF

Abstract

We design and fabricate shallow-etched periodically poled lithium niobate waveguides to realize highly efficient broadband spontaneous parametric down-conversion (SPDC) on nanophotonic chips. The shallow-etched waveguide can tolerate the non-uniformities of waveguide width induced by fabrication imperfections, enabling the generation of photon pairs with high count rate and bandwidth. We demonstrate photon-pair generation with a high brightness of 11.7 GHz/mW and bandwidth of 22 THz in a 5.7-mm-long PPLN waveguide. The generated photon pairs exhibit a strong temporal correlation with a coincidence-to-accidental ratio of up to 16262±850. Our results confirm the feasibility of shallow etching in the fabrication of an efficient SPDC device on the platform of lithium niobate on an insulator, and benefit quantum information processing with a broadband photon source.

DOI
10.1364/oe.519265

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We design and fabricate shallow-etched periodically poled lithium niobate waveguides to realize highly efficient broadband spontaneous parametric down-conversion (SPDC) on nanophotonic chips. The shallow-etched waveguide can tolerate the non-uniformities of waveguide width induced by fabrication imperfections, enabling the generation of photon pairs with high count rate and bandwidth. We demonstrate photon-pair generation with a high brightness of 11.7 GHz/mW and bandwidth of 22 THz in a 5.7-mm-long PPLN waveguide. The generated photon pairs exhibit a strong temporal correlation with a coincidence-to-accidental ratio of up to 16262±850. Our results confirm the feasibility of shallow etching in the fabrication of an efficient SPDC device on the platform of lithium niobate on an insulator, and benefit quantum information processing with a broadband photon source.
Broadband nonlinear optical devices play a critical role in both classical and quantum optics. Here, we design and fabricate a 6.82-mm-long step-chirped periodically poled lithium niobate~(CPPLN) waveguide on lithium niobate on insulator, which enables quasi-phase matching over a broad bandwidth for second-harmonic generation~(SHG) and spontaneous parametric down-conversion~(SPDC). The SHG achieves an average efficiency of 54.4\%/W/cm2^22 over the first-harmonic wavelength range of 1510~nm-1620~nm, paving the way for realizing SPDC across a wide range of pump wavelengths. For SPDC, by tuning the pump wavelength to 775~nm, 780~nm, and 785~nm, we achieve broadband photon-pair generation with a maximum full bandwidth and brightness up to 99~THz~(846~nm) and 20~GHz/mW/nm, respectively. Our findings provide an efficient and experiment-friendly approach for generating broadband photon pairs, which holds significant promise for advancing applications in quantum metrology.
Broadband nonlinear optical devices play a critical role in both classical and quantum optics. Here, we design and fabricate a 6.82-mm-long step-chirped periodically poled lithium niobate (CPPLN) waveguide on lithium niobate on insulator, which enables quasi-phase matching over a broad bandwidth for second-harmonic generation (SHG) and spontaneous parametric down-conversion (SPDC). The SHG achieves an average efficiency of 91%/W/cm 2 over the first-harmonic wavelength range of 1510 nm–1620 nm, paving the way for realizing SPDC across a wide range of pump wavelengths. For SPDC, by tuning the pump wavelength to 775 nm, 780 nm, and 785 nm, we achieve broadband photon-pair generation with a maximum full bandwidth and brightness up to 99 THz (846 nm) and 21 MHz/mW/nm, respectively. Our findings provide an efficient and experiment-friendly approach for generating broadband photon pairs, which holds significant promise for advancing applications in quantum metrology.
Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.
Chip-integrated nonlinear photonics holds the key for advanced optical information processing with superior performance and novel functionalities. Here, we present an optimally mode-matched, periodically poled lithium niobate nanowaveguide for efficient parametric frequency conversions on chip. Using a 4-mm nanowaveguide with subwavelength mode confinement, we demonstrate second harmonic generation with efficiency over 2200% W −1 c m −2, and broadband difference frequency generation over a 4.3-THz spectral span. These allow us to generate correlated photon pairs over multiple frequency channels via spontaneous parametric down conversion, all in their fundamental spatial modes, with a coincidence to accidental ratio as high as 600. The high efficiency and dense integrability of the present chip devices may pave a viable route to scalable nonlinear applications in both classical and quantum domains.
Integrated photon-pair sources, providing scalability solutions, are crucial for large-scale realizations of quantum photonic technologies. Their traditional fabrication techniques, such as etching, are often complex, require long development cycles, and are resource inefficient in case of fabrication imperfections or failures. The two-photon polymerization (2PP) technique can offer a rapid, efficient, and reproducible alternative for the fabrication of integrated photonic devices. Here, we demonstrate an integrated photon-pair source based on a 2PP-defined strip-loaded waveguide on a periodically poled thin-film lithium niobate (TFLN) platform. The device generates photon pairs through type-II spontaneous parametric down-conversion (SPDC), employing first-order quasi-phase matching (QPM) with TM-polarized excitation light. The device achieves an on-chip pair generation rate of 4.357 MHz and a coincidence-to-accidental ratio (CAR) of ∼404. To prove the flexibility and versatility of the fabrication technique, the waveguides were erased from the LN substrate and reprinted, reaching comparable performance. This work demonstrates the potential of 2PP as a rapid production technique for high-performance integrated photon-pair sources, offering a practical solution to the limitations of traditional fabrication techniques and showcasing both reproducibility of the fabrication and the reusability of the substrate.