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arXiv:2406.10503 · Physical review. B./Physical review. B

Quantum criticality and optical conductivity in a two-valley system

Yasha Gindikin, Songci Li, Alex Levchenko, Alex Kamenev, Andrey V. Chubukov, Dmitrii L. Maslov

Published Aug 20, 2024• 3 citations
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Abstract

We demonstrate that the optical conductivity of a Fermi liquid (FL) in the absence of umklapp scattering is dramatically affected by the topology of the Fermi surface (FS). Specifically, electron-electron ($\mathit{ee}$) scattering leads to rapid current relaxation in systems with multiple, or multiply connected, FSs, provided that the valleys have different effective masses. This effect results from intervalley drag. We microscopically derive the optical conductivity of a two-valley system, both within the FL regime and near a quantum critical point (QCP) of the Ising-nematic type. In the FL regime, intervalley drag restores the Gurzhi-like scaling of the conductivity, $\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\sim}{\ensuremath{\omega}}^{0}$. This dependence contrasts sharply with the previously identified subleading contribution to the conductivity of a two-dimensional FL with a single convex FS, where $\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\sim}{\ensuremath{\omega}}^{2}ln|\ensuremath{\omega}|$. The vanishing of the leading term in the optical conductivity is a signature of geometric constraints on $\mathit{ee}$ scattering channels, which are lifted for a multiply connected FS. A large differential response, $d\mathrm{Re}\ensuremath{\sigma}/d\ensuremath{\mu}$ with $\ensuremath{\mu}$ being the chemical potential, is predicted at the Lifshitz transition from a single-valley to a multivalley FS, which should be observable within the experimentally accessible frequency range. Near a QCP, intervalley drag leads to a ${|\ensuremath{\omega}|}^{\ensuremath{-}2/3}$ scaling of $\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})$ in two dimensions, thus providing a specific current-relaxing process for this long-standing conjecture.

DOI
10.1103/physrevb.110.085139

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We demonstrate that the optical conductivity of a Fermi liquid (FL) in the absence of umklapp scattering is dramatically affected by the topology of the Fermi surface (FS). Specifically, electron-electron (ee\mathit{ee}ee) scattering leads to rapid current relaxation in systems with multiple, or multiply connected, FSs, provided that the valleys have different effective masses. This effect results from intervalley drag. We microscopically derive the optical conductivity of a two-valley system, both within the FL regime and near a quantum critical point (QCP) of the Ising-nematic type. In the FL regime, intervalley drag restores the Gurzhi-like scaling of the conductivity, Re\ensuremathσ(\ensuremathω)\ensuremath∼\ensuremathω0\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\sim}{\ensuremath{\omega}}^{0}Re\ensuremathσ(\ensuremathω)\ensuremath∼\ensuremathω0. This dependence contrasts sharply with the previously identified subleading contribution to the conductivity of a two-dimensional FL with a single convex FS, where Re\ensuremathσ(\ensuremathω)\ensuremath∼\ensuremathω2ln∣\ensuremathω∣\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\sim}{\ensuremath{\omega}}^{2}ln|\ensuremath{\omega}|Re\ensuremathσ(\ensuremathω)\ensuremath∼\ensuremathω2ln∣\ensuremathω∣. The vanishing of the leading term in the optical conductivity is a signature of geometric constraints on ee\mathit{ee}ee scattering channels, which are lifted for a multiply connected FS. A large differential response, dRe\ensuremathσ/d\ensuremathμd\mathrm{Re}\ensuremath{\sigma}/d\ensuremath{\mu}dRe\ensuremathσ/d\ensuremathμ with \ensuremathμ\ensuremath{\mu}\ensuremathμ being the chemical potential, is predicted at the Lifshitz transition from a single-valley to a multivalley FS, which should be observable within the experimentally accessible frequency range. Near a QCP, intervalley drag leads to a ∣\ensuremathω∣\ensuremath−2/3{|\ensuremath{\omega}|}^{\ensuremath{-}2/3}∣\ensuremathω∣\ensuremath−2/3 scaling of Re\ensuremathσ(\ensuremathω)\mathrm{Re}\ensuremath{\sigma}(\ensuremath{\omega})Re\ensuremathσ(\ensuremathω) in two dimensions, thus providing a specific current-relaxing process for this long-standing conjecture.
We analyze optical conductivity of a clean two-dimensional electron system in a Fermi liquid regime near a T=0T=0T=0 Ising-nematic quantum critical point (QCP) and extrapolate the results to a QCP. We employ direct perturbation theory up to the two-loop order to elucidate how the Fermi surface's geometry (convex vs concave) and fermionic dispersion (parabolic vs nonparabolic) affect the scaling of the optical conductivity $\ensuremath{\sigma}(\ensuremath{\omega})$ with frequency $\ensuremath{\omega}$ and correlation length $\ensuremath{\xi}$. We find that for a convex Fermi surface the leading terms in the optical conductivity cancel out, leaving a subleading contribution $\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\propto}{\ensuremath{\omega}}^{2}{\ensuremath{\xi}}^{4}\mathcal{L}$, where L=const\mathcal{L}=\mathrm{const}L=const for a parabolic dispersion and $\mathcal{L}\ensuremath{\propto}ln\ensuremath{\omega}{\ensuremath{\xi}}^{3}$ in a generic case. For a concave Fermi surface, the leading terms do not cancel, and $\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\propto}{\ensuremath{\xi}}^{2}$. We extrapolate these results to a QCP and obtain $\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\propto}{\ensuremath{\omega}}^{2/3}$ for a convex Fermi surface and $\ensuremath{\sigma}(\ensuremath{\omega})\ensuremath{\propto}1/{\ensuremath{\omega}}^{2/3}$ for a concave Fermi surface.
We study the optical conductivity of a pristine two-dimensional electron system near an Ising-nematic quantum critical point. We discuss the relation between the frequency scaling of the conductivity and the shape of the Fermi surface, namely, whether it is isotropic, convex, or concave. We confirm the cancellation of the leading order terms in the optical conductivity for the cases of isotropic and convex Fermi surfaces and show that the remaining contribution scales as ${|\ensuremath{\omega}|}^{2/3}$ at T=0T=0T=0. On the contrary, the leading term, $\ensuremath{\propto}{|\ensuremath{\omega}|}^{\ensuremath{-}2/3}$, survives for a concave FS. We also address the frequency dependence of the optical conductivity near the convex-to-concave transition. Explicit calculations are carried out for the Fermi-liquid regime using the modified (but equivalent to the original) version of the Kubo formula, while the quantum-critical regime is accessed by employing the space-time scaling of the Z=3Z=3Z=3 critical theory.
Recent progress in experimental techniques has made it possible to extract detailed information on dynamics of carriers in a correlated electron material from its optical conductivity, [Formula: see text]. This review consists of three parts, addressing the following three aspects of optical response: (1) the role of momentum relaxation; (2) [Formula: see text] scaling of the optical conductivity of a Fermi-liquid metal, and (3) the optical conductivity of non-Fermi-liquid metals. In the first part (section 2), we analyze the interplay between the contributions to the conductivity from normal and umklapp electron-electron scattering. As a concrete example, we consider a two-band metal and show that although its optical conductivity is finite it does not obey the Drude formula. In the second part (sections 3 and 4), we re-visit the Gurzhi formula for the optical scattering rate, [Formula: see text], and show that a factor of [Formula: see text] is the manifestation of the 'first-Matsubara-frequency rule' for boson response, which states that [Formula: see text] must vanish upon analytic continuation to the first boson Matsubara frequency. However, recent experiments show that the coefficient b in the Gurzhi-like form, [Formula: see text], differs significantly from b = 4 in most of the cases. We suggest that the deviations from Gurzhi scaling may be due to the presence of elastic but energy-dependent scattering, which decreases the value of b below 4, with b = 1 corresponding to purely elastic scattering. In the third part (section 5), we consider the optical conductivity of metals near quantum phase transitions to nematic and spin-density-wave states. In the last case, we focus on 'composite' scattering processes, which give rise to a non-Fermi-liquid behavior of the optical conductivity at T = 0: [Formula: see text] at low frequencies and [Formula: see text] at higher frequencies. We also discuss [Formula: see text] scaling of the conductivity and show that [Formula: see text] in the same model scales in a non-Fermi-liquid way, as [Formula: see text].
We study the frequency dependence of the electron self-energy and the optical conductivity in a recently developed field theory of the spin-density-wave quantum phase transition in two-dimensional metals. We focus on the interplay between the Fermi surface ``hot spots'' and the remainder of the ``cold'' Fermi surface. Scattering of electrons off the fluctuations of the spin-density-wave order parameter, $\ensuremath{\varphi}$, is strongest at the hot spots; we compute the conductivity due to this scattering in a rainbow approximation. We point out the importance of composite operators, built of products of the primary electron or $\ensuremath{\varphi}$ fields: These have important effects also away from the hot spots. The simplest composite operator, ${\ensuremath{\varphi}}^{2}$, leads to deviations from Landau Fermi-liquid behavior on the entire Fermi surface. We also find an intermediate frequency window in which the cold electrons lose their quasiparticle form due to effectively one-dimensional scattering processes. The latter processes are part of umklapp scattering, which leads to singular contributions to the optical conductivity at the lowest frequencies at zero temperature.
Electrical transport properties near an electronic Ising-nematic quantum critical point in two dimensions are of both theoretical and experimental interest. In this work, we derive a kinetic equation valid in a broad regime near the quantum critical point using the memory matrix approach. The formalism is applied to study the effect of the critical fluctuations on the dc resistivity through different scattering mechanisms, including umklapp, impurity scattering, and electron-hole scattering in a compensated metal. We show that electrical transport in the quantum critical regime exhibits a rich behavior that depends sensitively on the scattering mechanism and the band structure. In the case of a single large Fermi surface, the resistivity due to umklapp scattering crosses over from $\ensuremath{\rho}\ensuremath{\sim}{T}^{2}$ at low temperature to sublinear at high temperature. The crossover temperature scales as q03{q}_{0}^{3}q03​, where q0{q}_{0}q0​ is the minimal wave vector for umklapp scattering. Impurity scattering leads to $\ensuremath{\rho}\ensuremath{-}{\ensuremath{\rho}}_{0}\ensuremath{\sim}{T}^{\ensuremath{\alpha}}$ (${\ensuremath{\rho}}_{0}$ being the residual resistivity), where $\ensuremath{\alpha}$ is either larger than 2 if there is only a single Fermi sheet present, or 4/34/34/3 in the case of multiple Fermi sheets. Finally, in a perfectly compensated metal with an equal density of electrons and holes, the low-temperature behavior depends strongly on the structure of ``cold spots'' on the Fermi surface, where the coupling between the quasiparticles and order parameter fluctuations vanishes by symmetry. In particular, for a system where cold spots are present on some (but not all) Fermi sheets, $\ensuremath{\rho}\ensuremath{\sim}{T}^{5/3}$. At higher temperatures, there is a broad crossover regime where $\ensuremath{\rho}$ either saturates or $\ensuremath{\rho}\ensuremath{\sim}T$, depending on microscopic details. We discuss these results in the context of recent quantum Monte Carlo simulations of a metallic Ising nematic critical point, and experiments in certain iron-based superconductors.
Electronic transport in Fermi liquids is usually Ohmic, because of momentum-relaxing scattering due to defects and phonons. These processes can become sufficiently weak in two-dimensional materials, giving rise to either ballistic or hydrodynamic transport, depending on the strength of electron-electron scattering. We show that the ballistic regime is a quantum critical point (QCP) on the regime boundary separating Ohmic and hydrodynamic transport. The QCP corresponds to a \emph{free} conformal field theory (CFT) with a dynamical scaling exponent z=1z = 1z=1. Its nontrivial aspects emerge in device geometries with shear, wherein the regime has an intrinsic universal dissipation, a nonlocal current-voltage relation, and exhibits the critical scaling of the underlying CFT. The Fermi surface has electron-hole pockets across all angular scales and the current flow has \emph{vortices} at all spatial scales. We image the fluctuations in high-definition and animate their emergence as experimental parameters are tuned to the QCP (movie links in comments). The vortices clearly demonstrate that Pauli exclusion alone can produce collective effects, with low-frequency AC transport mediated by vortex dynamics. The scale-invariant spatial structure is much richer than that of an interaction-dominated hydrodynamic regime, which only has a single vortex at the device scale. Our findings provide a theoretical framework for both interaction-free and interaction-dominated non-Ohmic transport in two-dimensional materials, as seen in several contemporary experiments.