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arXiv:2406.07616 · Physical Review Letters

Breakdown of the Quantum Distinction of Regular and Chaotic Classical Dynamics in Dissipative Systems

David Villaseñor, Léa Ferreira dos Santos, Pablo Barberis-Blostein

Published Dec 12, 2024• 14 citations
arXivHTMLPDF

Abstract

Quantum chaos has recently received increasing attention due to its relationship with experimental and theoretical studies of nonequilibrium quantum dynamics, thermalization, and the scrambling of quantum information. In an isolated system, quantum chaos refers to properties of the spectrum that emerge when the classical counterpart of the system is chaotic. However, despite experimental progress leading to longer coherence times, interactions with an environment can never be neglected, which calls for a definition of quantum chaos in dissipative systems. Advances in this direction were brought by the Grobe-Haake-Sommers (GHS) conjecture, which connects chaos in a dissipative classical system with cubic repulsion of the eigenvalues of the quantum counterpart and regularity with linear level repulsion. Here, we show that the GHS conjecture does not hold for the open Dicke model, which is a spin-boson model of experimental interest. We show that the onset of cubic level repulsion in the open quantum model is not always related with chaotic structures in the classical limit. This result challenges the universality of the GHS conjecture and raises the question of what is the source of spectral correlations in open quantum systems.

DOI
10.1103/physrevlett.133.240404

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Quantum chaos has recently received increasing attention due to its relationship with experimental and theoretical studies of nonequilibrium quantum dynamics, thermalization, and the scrambling of quantum information. In an isolated system, quantum chaos refers to properties of the spectrum that emerge when the classical counterpart of the system is chaotic. However, despite experimental progress leading to longer coherence times, interactions with an environment can never be neglected, which calls for a definition of quantum chaos in dissipative systems. Advances in this direction were brought by the Grobe-Haake-Sommers (GHS) conjecture, which connects chaos in a dissipative classical system with cubic repulsion of the eigenvalues of the quantum counterpart and regularity with linear level repulsion. Here, we show that the GHS conjecture does not hold for the open Dicke model, which is a spin-boson model of experimental interest. We show that the onset of cubic level repulsion in the open quantum model is not always related with chaotic structures in the classical limit. This result challenges the universality of the GHS conjecture and raises the question of what is the source of spectral correlations in open quantum systems.
Dissipative quantum chaos plays a central role in the characterization and control of information scrambling, nonunitary evolution, and thermalization, but it still lacks a precise definition. The Grobe-Haake-Sommers conjecture, which links Ginibre level repulsion to classical chaotic dynamics, was recently shown to fail [Phys. Rev. Lett. 133, 240404 (2024)PRLTAO0031-900710.1103/PhysRevLett.133.240404]. We properly restore the quantum-classical correspondence through a dynamical approach based on the von Neumann entropy (VNE) and out-of-time-order correlators (OTOCs), which reveal signatures of chaos beyond spectral statistics. Focusing on the open anisotropic Dicke model, we identify two distinct regimes: transient chaos, marked by rapid early-time growth of VNE and OTOCs followed by low saturation values, and steady-state chaos, characterized by high long-time values. We introduce a random matrix toy model and show that Ginibre spectral statistics signals short-time chaos rather than steady-state chaos. Our results establish VNE dynamics and OTOCs as reliable diagnostics of dissipative quantum chaos across different timescales.
We investigate the connection between classical and quantum chaos in a dissipative system of two coupled collective spins. Although the classical dynamics possesses a stable fixed-point attractor, we find pronounced signatures of chaos in the transient dynamics preceding relaxation. In the quantum model, such transient chaos is accompanied by a transition to random-matrix statistics in the relevant part of the Liouvillian spectrum and by a qualitative increase in the number of Liouvillian modes contributing to expectation values of physical observables. The transition occurs before the bifurcation at which the stable fixed point disappears and a chaotic attractor emerges. Our results show that Liouvillian quantum chaos can be associated with transient classical chaos, rather than requiring a chaotic asymptotic attractor, and provide a refinement of the Grobe-Haake-Sommers conjecture.
Abstract We compare the entire classical and quantum evolutions of the Dicke model in its regular and chaotic domains. This is a paradigmatic interacting spin-boson model of great experimental interest. By studying the classical and quantum survival probabilities of initial coherent states, we identify features of the long-time dynamics that are purely quantum and discuss their impact on the equilibration times. We show that the ratio between the quantum and classical asymptotic values of the survival probability serves as a metric to determine the proximity to a separatrix in the regular regime and to distinguish between two manifestations of quantum chaos: scarring and ergodicity. In the case of maximal quantum ergodicity, our results are analytical and show that quantum equilibration takes longer than classical equilibration.
For Hamiltonian systems, level statistics provide a faithful diagnostic of quantum chaos. By analogy, the statistics of the Lindbladian spectrum are often used in open quantum systems, and the Grobe-Haake-Sommers conjecture proposes that systems with chaotic classical counterparts should exhibit level repulsion in the Lindbladian spectrum. Here we point out an important flaw in this analogy: Hamiltonian and Lindbladian spectra behave differently and have distinct physical interpretations, and one should therefore not expect the latter to provide a reliable diagnostic. For Lindbladians, the late-time dynamics are not determined by the bulk of the eigenvalues but only by those eigenvalues -- and their corresponding eigenvectors -- with small real parts. Combined with the strong non-normality typical of Lindbladians, this allows situations in which the level statistics can be tuned almost arbitrarily without affecting the dynamics on either short or long time scales. We explicitly demonstrate this phenomenon and provide examples in which Ginibre level repulsion arises while the system dynamics at no time show signatures of chaos. We further relate this mechanism to the emergence of a non-Hermitian skin effect in Liouville space, linking boundary-induced eigenvector localization to the observed spectral instability. Our results show that level statistics cannot universally serve as a reliable diagnostic of quantum chaos in open quantum systems and highlight the need for alternative diagnostics that remain robust in strongly non-normal regimes.
We present an analysis of chaos and regularity in the open Dicke model, when dissipation is due to cavity losses. Due to the infinite Liouville space of this model, we also introduce a criterion to numerically find a complex spectrum which approximately represents the system spectrum. The isolated Dicke model has a well-defined classical limit with two degrees of freedom. We select two case studies where the classical isolated system shows regularity and where chaos appears. To characterize the open system as regular or chaotic, we study regions of the complex spectrum taking windows over the absolute value of its eigenvalues. Our results for this infinite-dimensional system agree with the Grobe-Haake-Sommers (GHS) conjecture for Markovian dissipative open quantum systems, finding the expected 2D Poisson distribution for regular regimes, and the distribution of the Ginibre unitary ensemble (GinUE) for the chaotic ones, respectively.
The effect of a large environment on a finite-size quantum mechanical system is two-fold: It brings dissipation, but also fluctuations of thermal and quantum origin. While dissipation tends to stabilize the dynamics, we question if and how environmental quantum fluctuations can generate chaos in an otherwise classically non-chaotic system. We work out a paradigmatic model of quantum optics: the dissipative Dicke model, where a large spin interacts with a dissipative harmonic mode. We dial in the classical/quantum correspondence by working in the semiclassical regime at large but finite spin. We demonstrate that, starting from a classically regular phase space in the superradiant regime, quantum noise can generate a strange attractor with fractal dimension and a positive Lyapunov exponent. We unveil the deep connection with shear-induced chaos that was recently developed in the mathematical community.