Recent experiments on Cooper pair splitters using superconductor-quantum dot hybrids have embarked on creating entanglement in the solid-state, by engineering the sub-gap processes in the superconducting region. Using the thermoelectric Cooper pair splitter setup [Nat. Comm., 12, 21, (2021)] as a prototype, we present a comprehensive analysis of the fundamental components of the observed transport signal, aiming to critically clarify the operating regimes and confirm the nonlocal and nonclassical nature of correlations arising from crossed Andreev processes. By making a nexus with quantum discord, we identify operating points of nonlocal quantum correlations in the CPS device—information that cannot be extracted from the transport signal alone. A notable consequence of our analysis is the finding that contact-induced level broadening of the quantum dot’s discrete energy spectrum, along with its hybridization with the superconducting segment, can lead to shifted resonances in the crossed Andreev process as well as a parity reversal in the thermoelectric current. Our work thereby provides detailed insights into the gate voltage control of the quantum correlations in superconducting-hybrid Cooper pair splitters, revealing new avenues for harnessing quantum correlations in solid-state systems.
Recent experiments on Cooper pair splitters using superconductor-quantum dot hybrids have embarked on creating entanglement in the solid-state, by engineering the sub-gap processes in the superconducting region. Using the thermoelectric Cooper pair splitter setup [Nat. Comm., 12, 21, (2021)] as a prototype, we present a comprehensive analysis of the fundamental components of the observed transport signal, aiming to critically clarify the operating regimes and confirm the nonlocal and nonclassical nature of correlations arising from crossed Andreev processes. By making a nexus with quantum discord, we identify operating points of nonlocal quantum correlations in the CPS device—information that cannot be extracted from the transport signal alone. A notable consequence of our analysis is the finding that contact-induced level broadening of the quantum dot’s discrete energy spectrum, along with its hybridization with the superconducting segment, can lead to shifted resonances in the crossed Andreev process as well as a parity reversal in the thermoelectric current. Our work thereby provides detailed insights into the gate voltage control of the quantum correlations in superconducting-hybrid Cooper pair splitters, revealing new avenues for harnessing quantum correlations in solid-state systems.
Abstract Entanglement of electrons is studied by means of current–current correlations in two Cooper pair splitter devices: with one and two proximized quantum dots (1QD and 2QD), in presence of intra- and inter-dot Coulomb interactions, and weakly coupled with metallic electrodes. The 1QD system, where Cooper pairs can be transmitted to the same or split to different normal electrodes, is contrasted with the 2QD device, where double occupancy of a single quantum dot is forbidden and transport is only through an inter-dot singlet due to non-local crossed Andreev reflection processes deep in the superconducting energy gap. Separating the current correlation function into components for partial currents of electrons and holes through various Andreev bound states, one can see bunching and antibunching of split particles: inter-level components between electron and hole currents flowing to different electrodes are positive, while intra-level electron–electron or hole–hole components are negative, respectively. Spectral decomposition of the frequency-dependent current cross-correlation is performed to get better insight into mechanisms of entanglement and dynamics of split Cooper pairs, and to extract various charge fluctuation processes with different relaxation times, related to electron and hole currents flowing through the Andreev bound states. Only low frequency polarization fluctuations are seen in the current cross-correlations, while various negative and positive high frequency (charge fluctuations) components compensate each other in the symmetric system.
We consider the subgap physics of a hybrid double-quantum dot Cooper-pair splitter with large single-level spacings, in the presence of tunneling between the dots and finite Coulomb intra- and interdot Coulomb repulsion. In the limit of a large superconducting gap, we treat the coupling of the dots to the superconductor exactly. We employ a generalized master-equation method, which easily yields currents, noise, and cross-correlators. In particular, for finite inter- and intradot Coulomb interaction, we investigate how the transport properties are determined by the interplay between local and nonlocal tunneling processes between the superconductor and the dots. We examine the effect of interdot tunneling on the particle-hole symmetry of the currents with and without spin-orbit interaction. We show that spin-orbit interaction in combination with finite Coulomb energy opens the possibility to control the nonlocal entanglement and its symmetry (singlet/triplet). We demonstrate that the generation of nonlocal entanglement can be achieved even without any direct nonlocal coupling to the superconducting lead.
A Cooper pair splitter consists of two quantum dots side-coupled to a conventional superconductor. Usually, the quantum dots are assumed to have a large charging energy compared to the superconducting gap, in order to suppress processes other than the coherent splitting of Cooper pairs. In this work, in contrast, we investigate the limit in which the charging energy is smaller than the superconducting gap. This allows us, in particular, to study the effect of a Zeeman field comparable to the charging energy. We find analytically that in this parameter regime the superconductor mediates an interdot tunneling term with a spin symmetry determined by the Zeeman field. Together with electrostatically tunable quantum dots, we show that this makes it possible to engineer a spin triplet state shared between the quantum dots. Compared to previous works, we thus extend the capabilities of the Cooper pair splitter to create entangled nonlocal electron pairs.
In a device with a superconductor coupled to two parallel quantum dots (QDs) the electrical tunability of the QD levels can be used to exploit nonclassical current correlations due to the splitting of Cooper pairs. We experimentally investigate the effect of a finite potential difference across one quantum dot on the conductance through the other completely grounded QD in a Cooper pair splitter fabricated on an InAs nanowire. We demonstrate that the nonlocal electrical transport through the device can be tuned by electrical means and that the energy dependence of the effective density of states in the QDs is relevant for the rates of Cooper pair splitting (CPS) and elastic cotunneling. Such experimental tools are necessary to understand and develop CPS-based sources of entangled electrons in solid-state devices.
We begin this dissertation by studying noise correlations in superconducting heterostructures of various geometries. In recent years there has been a resurgence of interest in the nonlocal transport properties of superconducting heterostructures due to the possibility of their serving as a source of electronic entanglement in solid state quantum information processors. Devices designed for this purpose are called Cooper pair splitting devices. The utility of these devices as entanglement sources is known to have connections to the positivity of noise cross correlations in spatially separated leads. In Chapter 1 we outline the theoretical prerequisites for this work, outlining the scattering theory framework based on the Bogoliubov-de Gennes equations we adopt. Within this framework we apply a methodology first introduced by Demers and by Blonder, Tinkham and Klapwijk (BTK) in the early 1980s to find the scattering matrix for our superconducting structures. The current, local and nonlocal shot noise can all be expressed in terms of the underlying scattering processes. This framework allows us to investigate the behavior of the current and noise correlations in the structure as we change the geometry and other key system parameters such as the system size, superconducting phase difference and temperature. We also introduce the Andreev approximation, a commonly used approximation which simplifies the scattering theory for superconducting heterostructures. In Chapter 2, we study the local and nonlocal shot noise in a quasi-1D normal-superconducting-normal (NSN) geometry using material parameters relevant to high-T [subscript c] superconductivity. The scattering and shot noise distributions are studied in the short, intermediate and long system size limits, allowing us to examine the qualitative differences in these three parameter regimes. This allows us to, for example, identify the signatures of over-the-gap geometric resonances in the shot noise distributions that appear in the long system size limit. We also break the nonlocal shot noise distributions down further and study the individual contributions to the nonlocal shot due to particle-particle, hole-hole and particle-hole scattering processes. In Chapter 3, we extend our investigation of superconducting heterostructures to the more complicated NSNSN geometry. A novel feature introduced in the geometry is the presence of subgap quasibound states, which show up as resonances in the scattering matrix. We show that these quasibound states dramatically impact the nonlocal shot noise distributions in the system. At energies near the quasibound states the dominant transmission channel through the system is a process called particle-hole transmission, which results in sharp positive peaks in the nonlocal shot noise distribution of the system. The behavior of the nonlocal noise correlations as we change the size of the superconducting and normal regions is investigated and it is found that there is a "sweet spot'' with respect to the size of the superconducting regions that maximizes the positivity of the nonlocal noise distributions as well as a periodic-like behavior in the positivity of the noise distributions with respect to the normal region size. The results of the full scattering theory for the NSNSN geometry are compared to the results obtained using the Andreev approximation, where we find that the Andreev approximation breaks down at energies close to the quasibound state energies. In the second half of this dissertation we focus on work related to the development of a prototype special-purpose quantum circuit simulation device based on commercial off-the-shelf high-speed analog signal processing hardware. In Chapter 4 we introduce the embedding scheme used to represent quantum states and quantum gates in the frequency domain of a classical analog voltage signal. Experimental results are presented from an early two-qubit prototype device for the fidelity of the state generation and gate application circuits. In Chapter 5, a more in-depth investigation into the modeling of classical errors within our signal processing based simulation method is performed in terms of the effects this noise has on the results of the quantum computation being simulatied. It is shown, for example, that additive white gaussian noise (AWGN) in our system has the same effect as applying a depolarizing channel to the qubits in the simulation. We then perform a simulation of a simple quantum error correction (QEC) protocol using the device and show that, even in the presence of classical noise in the simulation hardware, an overall enhancement in the performance of gate operations as a result of applying QEC is observed.
Abstract Correlations are fundamental in describing many body systems - not only in natural sciences. However, in experiments, correlations are notoriously difficult to assess on the microscopic scale, especially for electron spins. Here, we demonstrate a direct measurement of the spin cross-correlations between the currents of a Cooper pair splitter, an electronic device that emits electrons originating from Cooper pairs in a superconductor. While it is firmly established theoretically that these electron pairs form maximally spin-entangled singlet states with opposite spin projections, no spin correlation experiments have been demonstrated so far. We use ferromagnetic sidegates, compatible with superconducting electronic structures, to individually spin polarize the transmissions of two quantum dots fabricated in the two electronic paths, which act as tunable spin filters. The signals are detected in standard transport and in highly sensitive transconductance experiments. We find that the spin-cross correlation is negative, compatible with spin singlet emission, and deviates from the ideal value mostly due to a finite overlap of the Zeeman split quantum dot states. Our results demonstrate a new route to perform spin auto- and cross correlation experiments in nanometer scaled electronic devices, especially suitable for those relying on magnetic field sensitive superconducting elements, like unconventional, triplet or topologically non-trivial superconductors, or to perform Bell tests with massive particles, like electrons.