Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2406.01769 · Journal of Physics A Mathematical and Theoretical

Provable optimality of the square-tooth atomic frequency comb quantum memory

Allen Zang, Martin Suchara, Tian Zhong

Published Feb 25, 2025• 2 citations
arXivHTMLPDF

Abstract

Abstract Atomic frequency comb (AFC) quantum memories are a promising technology for quantum repeater networks because they enable multi-mode, long-time, and high-fidelity storage of photons with on-demand retrieval. The optimization of the retrieval efficiency of an AFC memory is important because it strongly impacts the entanglement distribution rate in quantum networks. Despite initial theoretical analyses and recent experimental demonstrations, a rigorous proof of the universally optimal configuration for the highest AFC retrieval efficiency has not been presented. In this paper we present a simple analytical proof which shows that the optimized square tooth offers the highest retrieval efficiency among all tooth shapes, under the physical constraint of finite optical depth of an atomic ensemble. The optimality still holds when the non-zero background absorption and the finite optical linewidth of atoms are considered. We further compare square, Lorentzian and Gaussian tooth shapes to reinforce the practical advantage of the square-tooth AFC in retrieval efficiency. Our proof lays rigorous foundation for the recipe of creating optimal AFC under realistic experimental conditions.

DOI
10.1088/1751-8121/adba1f

Related papers

Multimode quantum memory based on atomic frequency combs

Mikael Afzelius, Christoph Simon, Hugues de Riedmatten +1 more

An efficient multimode quantum memory is a crucial resource for long-distance quantum communication based on quantum repeaters. We propose a quantum memory based on spectral shaping of an inhomogeneously broadened optical transition into an atomic frequency comb (AFC). The spectral width of the AFC allows efficient storage of multiple temporal modes without the need to increase the absorption depth of the storage material, in contrast to previously known quantum memories. Efficient readout is possible thanks to rephasing of the atomic dipoles due to the AFC structure. Long-time storage and on-demand readout is achieved by use of spin states in a lambda-type configuration. We show that an AFC quantum memory realized in solids doped with rare-earth-metal ions could store hundreds of modes or more with close to unit efficiency, for material parameters achievable today.

arXiv:0805.4164•Physical Review A•May 21, 2009•642 citations

Quantum memory and quantum cloning in an atomic frequency comb

Ming Tian, Devin Vega

An atomic frequency comb (AFC) made of an ensemble of atoms with a periodic optical resonance was originally proposed as a viable approach for quantum memory for photons. In this paper we examine the quantum cloning capacity of an AFC in terms of the spectral distribution of the atomic populations in the energy levels associated with the optical transition. Expressions are derived for the memory readout efficiency, signal to noise ratio, and fidelity for an input at the single photon level. When applied to a square-toothed AFC, our analysis shows that there is a region where amplification from the excited state population results in greater than unit readout efficiency at a cost of fidelity being less than perfect, but still greater than the classical limit. The theory is developed under the assumption that both AFC and photon wave packets are spatially uniform. This can be regarded as a single spatial location inside an AFC and can be further expanded to study optically thick AFC with atomic population in both levels, which may find applications for quantum memory and quantum cloning machine.

arXiv:1902.01910•Physical Review A•Oct 28, 2019•2 citations

Efficient Quantum Memory Using a Weakly Absorbing Sample

Mahmood Sabooni, Qian Li, Stefan Kröll +1 more

A light-storage experiment with a total (storage and retrieval) efficiency η=56% is carried out by enclosing a sample, with a single-pass absorption of 10%, in an impedance-matched cavity. The experiment is carried out using the atomic frequency comb (AFC) technique in a praseodymium-doped crystal (0.05%Pr(3+):Y2SiO5) and the cavity is created by depositing reflection coatings directly onto the crystal surfaces. The AFC technique has previously by far demonstrated the highest multimode capacity of all quantum memory concepts tested experimentally. We claim that the present work shows that it is realistic to create efficient, on-demand, long storage time AFC memories.

arXiv:1301.0636•Physical Review Letters•Mar 26, 2013•210 citations

Multimode capacity of atomic-frequency comb quantum memories

Antonio Ortu, Jelena V. Rakonjac, Adrian Holzäpfel +5 more

Abstract Ensemble-based quantum memories are key to developing multiplexed quantum repeaters, able to overcome the intrinsic rate limitation imposed by finite communication times over long distances. Rare-earth ion doped crystals are main candidates for highly multimode quantum memories, where time, frequency and spatial multiplexing can be exploited to store multiple modes. In this context the atomic frequency comb (AFC) quantum memory provides large temporal multimode capacity, which can readily be combined with multiplexing in frequency and space. In this article, we derive theoretical formulas for quantifying the temporal multimode capacity of AFC-based memories, for both optical memories with fixed storage time and spin-wave memories with longer storage times and on-demand read out. The temporal multimode capacity is expressed in key memory parameters, such as AFC bandwidth, fixed-delay storage time, memory efficiency, and control field Rabi frequency. Current experiments in europium- and praseodymium-doped Y2SiO5 are analyzed within this theoretical framework, which is also tested with newly acquired data, as prospects for higher temporal capacity in these materials are considered. In addition we consider the possibility of spectral and spatial multiplexing to further increase the mode capacity, with examples given for praseodymium doped Y2SiO5.

arXiv:2202.12383•Quantum Science and Technology•May 26, 2022•53 citations

Towards a realistic model for cavity-enhanced atomic frequency comb quantum memories

Shahrzad Taherizadegan, Jacob H. Davidson, Sourabh Kumar +2 more

Abstract Atomic frequency comb (AFC) quantum memory is a favorable protocol in long distance quantum communication. Putting the AFC inside an asymmetric optical cavity enhances the storage efficiency but makes the measurement of the comb properties challenging. We develop a theoretical model for cavity-enhanced AFC quantum memory that includes the effects of dispersion, and show a close alignment of the model with our own experimental results. Providing semi-quantitative agreement for estimating the efficiency and a good description of how the efficiency changes as a function of detuning, it also captures certain qualitative features of the experimental reflectivity. For comparison, we show that a theoretical model without dispersion fails dramatically to predict the correct efficiencies. Our model is a step forward to accurately estimating the created comb properties, such as the optical depth inside the cavity, and so being able to make precise predictions of the performance of the prepared cavity-enhanced AFC quantum memory.

Quantum Science and Technology•May 22, 2024•1 citation

Towards a Realistic Model for Cavity-Enhanced Atomic Frequency Comb Quantum Memories

Shahrzad Taherizadegan, Jacob H. Davidson, Sourabh Kumar +2 more

Atomic frequency comb (AFC) quantum memory is a favorable protocol in long distance quantum communication. Putting the AFC inside an asymmetric optical cavity enhances the storage efficiency but makes the measurement of the comb properties challenging. We develop a theoretical model for cavity-enhanced AFC quantum memory that includes the effects of dispersion, and show a close alignment of the model with our own experimental results. Providing semi quantitative agreement for estimating the efficiency and a good description of how the efficiency changes as a function of detuning, it also captures certain qualitative features of the experimental reflectivity. For comparison, we show that a theoretical model without dispersion fails dramatically to predict the correct efficiencies. Our model is a step forward to accurately estimating the created comb properties, such as the optical depth inside the cavity, and so being able to make precise predictions of the performance of the prepared cavity-enhanced AFC quantum memory.

arXiv:2309.10332•Sep 19, 2023•0 citations
Abstract Atomic frequency comb (AFC) quantum memories are a promising technology for quantum repeater networks because they enable multi-mode, long-time, and high-fidelity storage of photons with on-demand retrieval. The optimization of the retrieval efficiency of an AFC memory is important because it strongly impacts the entanglement distribution rate in quantum networks. Despite initial theoretical analyses and recent experimental demonstrations, a rigorous proof of the universally optimal configuration for the highest AFC retrieval efficiency has not been presented. In this paper we present a simple analytical proof which shows that the optimized square tooth offers the highest retrieval efficiency among all tooth shapes, under the physical constraint of finite optical depth of an atomic ensemble. The optimality still holds when the non-zero background absorption and the finite optical linewidth of atoms are considered. We further compare square, Lorentzian and Gaussian tooth shapes to reinforce the practical advantage of the square-tooth AFC in retrieval efficiency. Our proof lays rigorous foundation for the recipe of creating optimal AFC under realistic experimental conditions.
An efficient multimode quantum memory is a crucial resource for long-distance quantum communication based on quantum repeaters. We propose a quantum memory based on spectral shaping of an inhomogeneously broadened optical transition into an atomic frequency comb (AFC). The spectral width of the AFC allows efficient storage of multiple temporal modes without the need to increase the absorption depth of the storage material, in contrast to previously known quantum memories. Efficient readout is possible thanks to rephasing of the atomic dipoles due to the AFC structure. Long-time storage and on-demand readout is achieved by use of spin states in a lambda-type configuration. We show that an AFC quantum memory realized in solids doped with rare-earth-metal ions could store hundreds of modes or more with close to unit efficiency, for material parameters achievable today.
An atomic frequency comb (AFC) made of an ensemble of atoms with a periodic optical resonance was originally proposed as a viable approach for quantum memory for photons. In this paper we examine the quantum cloning capacity of an AFC in terms of the spectral distribution of the atomic populations in the energy levels associated with the optical transition. Expressions are derived for the memory readout efficiency, signal to noise ratio, and fidelity for an input at the single photon level. When applied to a square-toothed AFC, our analysis shows that there is a region where amplification from the excited state population results in greater than unit readout efficiency at a cost of fidelity being less than perfect, but still greater than the classical limit. The theory is developed under the assumption that both AFC and photon wave packets are spatially uniform. This can be regarded as a single spatial location inside an AFC and can be further expanded to study optically thick AFC with atomic population in both levels, which may find applications for quantum memory and quantum cloning machine.
A light-storage experiment with a total (storage and retrieval) efficiency η=56% is carried out by enclosing a sample, with a single-pass absorption of 10%, in an impedance-matched cavity. The experiment is carried out using the atomic frequency comb (AFC) technique in a praseodymium-doped crystal (0.05%Pr(3+):Y2SiO5) and the cavity is created by depositing reflection coatings directly onto the crystal surfaces. The AFC technique has previously by far demonstrated the highest multimode capacity of all quantum memory concepts tested experimentally. We claim that the present work shows that it is realistic to create efficient, on-demand, long storage time AFC memories.
Abstract Ensemble-based quantum memories are key to developing multiplexed quantum repeaters, able to overcome the intrinsic rate limitation imposed by finite communication times over long distances. Rare-earth ion doped crystals are main candidates for highly multimode quantum memories, where time, frequency and spatial multiplexing can be exploited to store multiple modes. In this context the atomic frequency comb (AFC) quantum memory provides large temporal multimode capacity, which can readily be combined with multiplexing in frequency and space. In this article, we derive theoretical formulas for quantifying the temporal multimode capacity of AFC-based memories, for both optical memories with fixed storage time and spin-wave memories with longer storage times and on-demand read out. The temporal multimode capacity is expressed in key memory parameters, such as AFC bandwidth, fixed-delay storage time, memory efficiency, and control field Rabi frequency. Current experiments in europium- and praseodymium-doped Y2SiO5 are analyzed within this theoretical framework, which is also tested with newly acquired data, as prospects for higher temporal capacity in these materials are considered. In addition we consider the possibility of spectral and spatial multiplexing to further increase the mode capacity, with examples given for praseodymium doped Y2SiO5.
Abstract Atomic frequency comb (AFC) quantum memory is a favorable protocol in long distance quantum communication. Putting the AFC inside an asymmetric optical cavity enhances the storage efficiency but makes the measurement of the comb properties challenging. We develop a theoretical model for cavity-enhanced AFC quantum memory that includes the effects of dispersion, and show a close alignment of the model with our own experimental results. Providing semi-quantitative agreement for estimating the efficiency and a good description of how the efficiency changes as a function of detuning, it also captures certain qualitative features of the experimental reflectivity. For comparison, we show that a theoretical model without dispersion fails dramatically to predict the correct efficiencies. Our model is a step forward to accurately estimating the created comb properties, such as the optical depth inside the cavity, and so being able to make precise predictions of the performance of the prepared cavity-enhanced AFC quantum memory.
Atomic frequency comb (AFC) quantum memory is a favorable protocol in long distance quantum communication. Putting the AFC inside an asymmetric optical cavity enhances the storage efficiency but makes the measurement of the comb properties challenging. We develop a theoretical model for cavity-enhanced AFC quantum memory that includes the effects of dispersion, and show a close alignment of the model with our own experimental results. Providing semi quantitative agreement for estimating the efficiency and a good description of how the efficiency changes as a function of detuning, it also captures certain qualitative features of the experimental reflectivity. For comparison, we show that a theoretical model without dispersion fails dramatically to predict the correct efficiencies. Our model is a step forward to accurately estimating the created comb properties, such as the optical depth inside the cavity, and so being able to make precise predictions of the performance of the prepared cavity-enhanced AFC quantum memory.