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arXiv:2405.14685 · Physical review. B./Physical review. B

Controlling dephasing of coupled qubits via shared bath coherence

L. M. J. Hall, L. S. Sirkina, A. Morreau, W. Langbein, Egor A. Muljarov

Published Jun 9, 2025• 2 citations
arXivHTMLPDF

Abstract

The interaction of a quantum system with its environment limits its coherence time. This, in particular, restricts the utility of qubits in quantum information processing applications. In this paper, we show that the decoherence of a coupled qubit system can be minimized, or even eliminated, by exploiting the quantum coherence of the bath itself. We investigate the dephasing in a system of two spatially separated, electronically decoupled qubits, with direct or mediated coupling, interacting with a shared bath. For illustration, we treat Förster or cavity-mediated coupling between semiconductor quantum dots interacting with acoustic phonons. Using the rigorous method of Trotter's decomposition with cumulant expansion, we demonstrate a reduction in the dephasing rates at specific distances between the dots. The control of dephasing with distance is a coherent effect of the shared bath and is absent for independent baths. It can be understood in terms of phonon-assisted transitions between the entangled qubit states of the coupled system.

DOI
10.1103/ltk8-fpv3

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The interaction of a quantum system with its environment limits its coherence time. This, in particular, restricts the utility of qubits in quantum information processing applications. In this paper, we show that the decoherence of a coupled qubit system can be minimized, or even eliminated, by exploiting the quantum coherence of the bath itself. We investigate the dephasing in a system of two spatially separated, electronically decoupled qubits, with direct or mediated coupling, interacting with a shared bath. For illustration, we treat Förster or cavity-mediated coupling between semiconductor quantum dots interacting with acoustic phonons. Using the rigorous method of Trotter's decomposition with cumulant expansion, we demonstrate a reduction in the dephasing rates at specific distances between the dots. The control of dephasing with distance is a coherent effect of the shared bath and is absent for independent baths. It can be understood in terms of phonon-assisted transitions between the entangled qubit states of the coupled system.
We analyse various phonon-assisted mechanisms which contribute to the decoherence of excitonic qubits in quantum dot systems coupled by the Förster-type transfer process. We show the significant loss of coherence accompanied by dissipation due to charge carrier oscillations between qubit states by using a model of one-phonon assisted Förster-type transfer process. We obtain explicit expressions for the relaxation and dephasing times for excitonic qubits interacting with acoustic phonons via both deformation potential and piezoelectric coupling. We compare the decoherence times of the GaAs/AlGaAs material system with half times of concurrence decay in a 2$\otimes$2 bipartite mixed excitonic qubit system. We extend calculations to determine the influence of phonon mediated interactions on the non-unitary evolution of Berry phase in quantum dot systems.
It has recently been shown that interactions among the spins of a bath can result in an effective suppression of the decoherence of a single qubit embedded in a multi-spin environment. However, the effects of such intrabath interaction on the dynamics of entanglement are still not well understood. Here we study the dynamics of a system composed of two entangled qubits coupled to (1) independent self-interacting spin baths, and (2) a common self-interacting spin bath. We find that, as in the case of a single qubit, strong interactions among the spins in the bath may induce an effective decoupling between the bath and the system—this in turn suppresses the loss of entanglement that a non-, or weakly, interacting bath would typically cause. However we find that the intrabath interaction strength needed to achieve such effects is much larger than in the single qubit case, especially when the two qubits share the same environment. Our results illustrate the system's size effects in the entanglement sharing condition, where the entanglement within the bath limits the entanglement between the bath and the system.
We consider pure dephasing of Bell states of electron spin qubits interacting with a sparse bath of nuclear spins. Using the newly developed two-qubit generalization of cluster-correlation expansion method, we calculate the spin-echo decay of $|\mathrm{\ensuremath{\Psi}}\ensuremath{\rangle}$ and $|\mathrm{\ensuremath{\Phi}}\ensuremath{\rangle}$ states for various interqubit distances. Comparing the results with calculations in which dephasing of each qubit is treated independently, we identify signatures of influence of common part of the bath on the two qubits. At large interqubit distances, this common part consists of many nuclei weakly coupled to both qubits, so that decoherence caused by it can be modeled by considering multiple uncorrelated sources of noise (clusters of nuclei), each of them weakly affecting the qubits. Consequently, the resulting genuinely two-qubit contribution to decoherence can be described as being caused by classical Gaussian noise. On the other hand, for small interqubit distances the common part of the environment contains clusters of spins that are strongly coupled to both qubits, and their contribution to two-qubit dephasing has visibly non-Gaussian character. We show that one can easily obtain information about non-Gaussianity of environmental noise affecting the qubits from the comparison of dephasing of $|\mathrm{\ensuremath{\Psi}}\ensuremath{\rangle}$ and $|\mathrm{\ensuremath{\Phi}}\ensuremath{\rangle}$ Bell states. Numerical results are obtained for two nitrogen vacancy centers interacting with a bath of 13C^{13}\mathrm{C}13C nuclei of natural concentration, for which we obtain that Gaussian description of a correlated part of environmental noise starts to hold for centers separated by about 3 nm.
A semiconductor quantum dot (QD) embedded within an optical microcavity is a system of fundamental importance within quantum information processing. The optimization of quantum coherence is crucial in such applications, requiring an in-depth understanding of the relevant decoherence mechanisms. We provide herein a critical review of prevalent theoretical treatments of the QD-cavity system coupled to longitudinal acoustic phonons, comparing predictions against a recently obtained exact solution. Within this review we consider a range of temperatures and exciton-cavity coupling strengths. Predictions of the polaron Nakajima-Zwanzig (NZ) and time-convolutionless (TCL) master equations, as well as a variation of the former adapted for adiabatic continuous wave excitation (CWE), are compared against an asymptotically exact solution based upon Trotter's decomposition (TD) theorem. The NZ and TCL implementations, which apply a polaron transformation to the Hamiltonian and subsequently treat the exciton-cavity coupling to second order, do not offer a significant improvement accuracy relative to the polaron transformation alone. The CWE adaptation provides a marked improvement, capturing the broadband features of the absorption spectrum (not present in NZ and TCL implementations). We attribute this difference to the effect of the Markov approximation, and particularly its unsuitability in pulsed excitation regime. Even the CWE adaptation, however, breaks down in the regime of high temperature (50K50K50K) and strong exciton-cavity coupling (g≳0.2g \gtrsim 0.2g≳0.2 meV). The TD solution is of comparable computational complexity to the above-mentioned master equation approaches, yet remains accurate at higher temperatures and across a broad range of exciton-cavity coupling strengths (at least up to g=1.5g=1.5g=1.5 meV).
Methods that preserve coherence broadly impact all quantum information processing and metrology applications. Dynamical decoupling methods accomplish this by protecting qubits in noisy environments but are typically constrained to the limit where the qubits themselves are non-interacting. Here we consider the alternate regime wherein the inter-qubit couplings are of the same order as dephasing interactions with the environment. We propose and demonstrate a multi-pulse protocol that protects transverse spin states by suitably Hamiltonian engineering the inter-spin coupling while simultaneously suppressing dephasing noise on the qubits. We benchmark the method on 13C nuclear spin qubits in diamond, dipolar coupled to each other and embedded in a noisy electronic spin bath, and hyperpolarized via optically pumped NV centers. We observe effective state lifetimes of 13C nuclei $T_2^{\prime}\approx$2.5s at room temperature, an extension of over 4700-fold over the conventional T2∗T_2^{\ast}T2∗​ free induction decay. The spins are continuously interrogated during the applied quantum control, resulting in 13C NMR line narrowing and an $>$500-fold boost in SNR due to the lifetime extension. Together with hyperpolarization spin interrogation is accelerated by >1011>10^{11}>1011 over conventional 7T NMR. This work suggests strategies for the dynamical decoupling of coupled qubit systems with applications in a variety of experimental platforms.
We investigate the influence of phonon mediated interactions on the non-unitary evolution of geometrical phases in excitonic qubits formed in quantum dots entangled by pure Förster coupling. We consider decoherence to occur via acoustic phonons interacting through the deformation potential and piezoelectric coupling mechanisms. The influences of bath temperature, external electric field, quantum dot size and interdot distance on the evolution of geometrical phases are examined for the GaAs/AlGaAs material system. We extend the theory to determine the effect of dynamic decoupling employing ultrafast π-pulses on the evolution of geometrical phases in the presence of dephasing processes.