We demonstrate the emergence of nonreciprocal superradiant phase transitions and novel multicriticality in a cavity quantum electrodynamics system, where a two-level atom interacts with two counterpropagating modes of a whispering-gallery-mode microcavity. The cavity rotates at a certain angular velocity and is directionally squeezed by a unidirectional parametric pumping χ^{(2)} nonlinearity. The combination of cavity rotation and directional squeezing leads to nonreciprocal first- and second-order superradiant phase transitions. These transitions do not require ultrastrong atom-field couplings and can be easily controlled by the external pump field. Through a full quantum description of the system Hamiltonian, we identify two types of multicritical points in the phase diagram, both of which exhibit controllable nonreciprocity. These results open a new door for all-optical manipulation of superradiant transitions and multicritical behaviors in light-matter systems, with potential applications in engineering various integrated nonreciprocal quantum devices.
We demonstrate the emergence of nonreciprocal superradiant phase transitions and novel multicriticality in a cavity quantum electrodynamics system, where a two-level atom interacts with two counterpropagating modes of a whispering-gallery-mode microcavity. The cavity rotates at a certain angular velocity and is directionally squeezed by a unidirectional parametric pumping χ^{(2)} nonlinearity. The combination of cavity rotation and directional squeezing leads to nonreciprocal first- and second-order superradiant phase transitions. These transitions do not require ultrastrong atom-field couplings and can be easily controlled by the external pump field. Through a full quantum description of the system Hamiltonian, we identify two types of multicritical points in the phase diagram, both of which exhibit controllable nonreciprocity. These results open a new door for all-optical manipulation of superradiant transitions and multicritical behaviors in light-matter systems, with potential applications in engineering various integrated nonreciprocal quantum devices.
Precise control of criticality in superradiant phase transitions is essential for quantum state engineering and the simulation of nonequilibrium phase transitions. Here, we investigate theoretically multicritical phenomena in a dissipative two-Rydberg-atom cavity--QED system. The intrinisic dipole--dipole interaction between the two Rydberg atoms restructures the energy-level landscape of the atomic subsystem, thereby significantly modifying the boundary of the continuous second-order superradiant phase transition, and shifting both the phase boundary and the multicritical point toward weaker atom--cavity strengths. For sufficiently strong dipole--dipole interactions, the continuous second-order phase transition and the multicritical point both disappear, leaving only a discontinuous first--order phase transition that enables the emergence of a superradiant phase even at arbitrarily weak atom--cavity coupling. This work is of fundamental interest for studying dissipative quantum phase transitions, with potential implications for quantum precision measurement and quantum sensing.
We theoretically investigate the quantum phase transition in the collective systems of qubits in a high quality cavity, where the cavity field is squeezed via the optical parametric amplification process. We show that the squeezed light induced symmetry breaking can result in quantum phase transition without the ultrastrong coupling requirement. Using the standard mean field theory, we derive the condition of the quantum phase transition. Surprisingly, we show that there exists a tricritical point where the first- and second-order phase transitions meet. With specific atom-cavity coupling strengths, both the first- and second-order phase transition can be controlled by the nonlinear gain coefficient, which is sensitive to the pump field. These features also lead to an optical switching from the normal phase to the superradiant phase by just increasing the pump field intensity. The signature of these phase transitions can be observed by detecting the phase space Wigner function distribution with different profiles controlled by the squeezed light intensity. Such superradiant phase transition can be implemented in various quantum systems, including atoms, quantum dots, and ions in optical cavities as well as the circuit quantum electrodynamics system.
Abstract Quantum phase transitions with multicritical points are fascinating phenomena occurring in interacting quantum many-body systems. However, multicritical points predicted by theory have been rarely verified experimentally; finding multicritical points with specific behaviors and realizing their control remains a challenging topic. Here, we propose a system that a quantized light field interacts with a two-level atomic ensemble coupled by microwave fields in optical cavities, which is described by a generalized Dicke model. Multicritical points for the superradiant quantum phase transition are shown to occur. We determine the number and position of these critical points and demonstrate that they can be effectively manipulated through the tuning of system parameters. Particularly, we find that the quantum critical points can evolve into a Lifshitz point (LP) if the Rabi frequency of the light field is modulated periodically in time. Remarkably, the texture of atomic pseudo-spins can be used to characterize the quantum critical behaviors of the system. The magnetic orders of the three phases around the LP, represented by the atomic pseudo-spins, are similar to those of an axial next-nearest-neighboring Ising model. The results reported here are beneficial for unveiling intriguing physics of quantum phase transitions and pave the way towards to find novel quantum multicritical phenomena based on the generalized Dicke model.
Dissipation can fundamentally reconstruct the multicritical structure of driven-dissipative light–matter systems. In the interpolating Dicke–Tavis–Cummings model, cavity loss eliminates the U(1)-symmetric superradiant phase on the Tavis–Cummings line λx=λy and splits the original multicritical point into a pair of dissipation-induced tricritical points. Here, we show that intracavity optical squeezing provides a coherent means of continuously reshaping this loss-generated multicritical structure. The single-mode parametric interaction acts asymmetrically on the two cavity quadratures, thereby deforming the phase boundaries and continuously tuning the dissipation-induced tricritical points. We analytically determine the phase boundaries and the evolution of the tricritical structure with the parametric gain and cavity dissipation, and show that the two tricritical points coalesce in the weak-loss limit. Photon-number fluctuations provide clear quantum signatures of the squeezing-controlled multicritical structure.
In the present article, we investigate the behavior of a large collection of three-level $\mathrm{\ensuremath{\Lambda}}$ atoms interacting with two quantized electromagnetic fields inside a second-order nonlinear quantum cavity. The nonlinearity of the cavity is supposed to be activated by the application of two classical pump fields. The total Hamiltonian of the combination, with due attention to the nonlinearity effects, is diagonalized. The corresponding ground-state energy then follows from minimizing the total Hamiltonian. The structure of the ground state indicates that four distinct optical phases can occur in such a system. These possible phases turn out to be trivial, dark, left-arm and right-arm superradiant ones. Conditions under which any of the four optical phases can actually occur are also analyzed and discussed. The analysis of the conditions, accompanied by several figures, then reveals that with a suitable choice of the pump field amplitudes and/or geometrical phases, one can intensify the two superradiant phases drastically. Moreover, we demonstrate that the dark optical phase cannot occur at all, while the trivial and superradiant ones can, in fact, coexist. Our calculations also show that transition from the trivial phase to left-arm (right-arm) superradiant one is continuous (discrete) and second (first) order in nature. Another important result of our investigation is that by adjusting the pump field strength, one can switch from the left-arm superradiant phase to the right-arm one and vice versa. This point, in turn, provides an alternative mechanism for the development of quantum optical switching devices.
(τ) of the transmitted probe light from the cavity is determined by the nonlinearity of the atom in the cavity. Therefore, the system provides a platform for controlling the photon statistics by manipulating nonlinearity. In this paper, we experimentally demonstrate nonreciprocal quantum statistics in a cavity QED system with several atoms strongly coupled to an asymmetric optical cavity, which is composed of two mirrors with different transmittivities. When the direction of the probe light is reversed, the intracavity light field alternates to a different level. Distinct photon statistics are then observed due to the quantum nonlinearity associated with strongly coupled atoms. Sub-Poissonian photon-number statistics for forward light and a Poissonian distribution for backward light are then realized. Our work provides an effective approach for realizing nonreciprocal quantum devices, which have potential applications in the unidirectional generation of nonclassical light fields and quantum sensing.