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arXiv:2405.03493

Polarization-entangled photon pair generation from an epsilon-near-zero metasurface

Wenhe Jia, Grégoire Saerens, Ülle‐Linda Talts, Helena Weigand, Robert J. Chapman, Liu Li, Rachel Grange, Yuanmu Yang

Published May 6, 2024• 5 citations
arXivHTMLPDF

Abstract

Polarization-entangled photon pair sources are essential for diverse quantum technologies, such as quantum communication, computation, and imaging. However, the generation of complex polarization-entangled quantum states has long been constrained by the available nonlinear susceptibility tensor of natural nonlinear crystals, necessitating a cumbersome and intricate setup for additional coherent superposition or post-selection. In this study, we introduce and experimentally demonstrate a nanoscale polarization-entangled photon pair source utilizing an artificially-engineered metamaterial platform. This platform is based on a plasmonic metasurface that is strongly coupled to an epsilon-near-zero (ENZ) material. By precisely engineering resonances at both pump and signal/idler wavelengths, and leveraging the field enhancement provided by the ENZ effect, the photon pair generation efficiency of the 68-nm-thick metasurface is significantly boosted. More notably, the ENZ metasurface platform facilitates versatile manipulation of the system's anisotropic second-order nonlinear susceptibility tensor, enabling direct control over the polarization states of the photon pairs, which leads to the generation of a polarization-entangled Bell state without the need for additional components. Our approach opens a new avenue for the simultaneous photon pair generation and quantum state engineering in a compact platform.

DOI
10.48550/arxiv.2405.03493

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Polarization-entangled photon pair sources are essential for diverse quantum technologies, such as quantum communication, computation, and imaging. However, the generation of complex polarization-entangled quantum states has long been constrained by the available nonlinear susceptibility tensor of natural nonlinear crystals, necessitating a cumbersome and intricate setup for additional coherent superposition or post-selection. In this study, we introduce and experimentally demonstrate a nanoscale polarization-entangled photon pair source utilizing an artificially-engineered metamaterial platform. This platform is based on a plasmonic metasurface that is strongly coupled to an epsilon-near-zero (ENZ) material. By precisely engineering resonances at both pump and signal/idler wavelengths, and leveraging the field enhancement provided by the ENZ effect, the photon pair generation efficiency of the 68-nm-thick metasurface is significantly boosted. More notably, the ENZ metasurface platform facilitates versatile manipulation of the system's anisotropic second-order nonlinear susceptibility tensor, enabling direct control over the polarization states of the photon pairs, which leads to the generation of a polarization-entangled Bell state without the need for additional components. Our approach opens a new avenue for the simultaneous photon pair generation and quantum state engineering in a compact platform.
Pairs of polarization-entangled photons are important for diverse quantum technologies, such as quantum communication, computation, and imaging. However, generating complex polarization-entangled states has long been constrained by the available nonlinear susceptibility tensor of natural materials, necessitating cumbersome setups for additional coherent superposition or postselection. In this study, we experimentally demonstrate the generation of pairs of polarization-entangled photons using a plasmonic metasurface strongly coupled to an epsilon-near-zero (ENZ) material. By engineering a resonance at the pump wavelength and leveraging the field enhancement provided by the ENZ effect, the photon pair generation efficiency of the 68-nanometer-thick metasurface is substantially boosted compared to that of an unpatterned indium tin oxide film. More notably, the ENZ metasurface platform facilitates versatile manipulation of the system's anisotropic second-order nonlinear susceptibility tensor, enabling direct control over the polarization states of the photon pairs and generating a polarization-entangled Bell state without additional components. This approach enables simultaneous photon pair generation and quantum state engineering in a compact platform.
Polarization-entangled photon pairs are essential resources for quantum information technologies, yet realizing compact sources with intrinsically controllable entanglement remains challenging. Van der Waals (vdW) nonlinear materials such as NbOCl2 provide atomically thin platforms for quantum light generation, yet their native crystalline anisotropies as natural materials impose limitations on accessible quantum states. Here, we develop a resonant vdW nonlinear metasurface based on NbOCl2 that exploits its intrinsic optical anisotropy to engineer polarization-dependent nonlinear responses. The anisotropic optical dispersion enables selective manipulation of resonant modes, resulting in a three-order-of-magnitude enhancement of the nonlinear response along the c axis. By further tailoring these resonant modes, we redistribute the effective second-order nonlinear susceptibility tensor between orthogonal polarization channels, balancing the spontaneous parametric down-conversion pathways along the b and c axes. This enables polarization-entangled photon generation with a measured fidelity of up to 92%. Our work establishes metasurface-enabled nonlinear optical engineering as a strategy for enhancing and controlling quantum light generation in vdW materials, providing a pathway toward scalable quantum photonic platforms.
Complex polarization states of photon pairs are indispensable in various quantum technologies. Conventional methods for preparing desired two-photon polarization states are realized through bulky nonlinear crystals, which can restrict the versatility and tunability of the generated quantum states due to the fixed crystal nonlinear susceptibility. Here we present a solution using a nonlinear metasurface incorporating multiplexed silica metagratings on a lithium niobate film of 300 nm thickness. We fabricate two orthogonal metagratings on a single substrate with an identical resonant wavelength, thereby enabling the spectral indistinguishability of the emitted photons, and we demonstrate in experiments that the two-photon polarization states can be shaped by the metagrating orientation. Leveraging this essential property, we formulate a theoretical approach for generating arbitrary polarization-entangled qutrit states by combining three metagratings on a single metasurface, allowing the encoding of the desired quantum states or information. Our findings enable miniaturized optically controlled quantum devices by using ultrathin metasurfaces as polarization-entangled photon sources.
Photon-based polarization entanglement in the form of Bell states and qutrits is an essential tool for understanding complex quantum phenomena and implementing various quantum technologies such as free-space quantum communication and quantum imaging. Polarization-entangled photons are conventionally generated in bulky nonlinear crystals through spontaneous parametric down-conversion (SPDC). In this approach, the photon polarization is intrinsically defined by the nonlinear tensor of the material, restricting the versatility of the generated quantum states. The recent developments of dielectric nanostructures with sub-wavelength thickness called metasurfaces [1] enable miniaturization of quantum light sources, while dramatically enhancing the photon-pair generation and allowing the preparation of complex quantum states with spectral [2] and spatial [3] entanglement. However, optically reconfigurable generation of biphoton polarization states with metasurfaces remained unexplored.
Flat optics has emerged as a promising platform for ultrathin polarization-entangled sources via spontaneous parametric downconversion in subwavelength-thick nonlinear films or metasurfaces. However, previous schemes typically required multiplexing two films or two meta-structures with different orientations. Here, we propose a nonlinear metasurface composed of a single silica grating atop a lithium niobate film to generate polarization-entangled photon pairs. By engineering the angular dispersion of metasurface resonances, adjusting the pump frequency, and leveraging the polarization correlated transverse phase matching, the |HH〉 and |VV〉 states are simultaneously enhanced by over 2000 times, while the |HV〉 and |VH〉 states remain similar when compared to the pure film. Therefore, the degree of polarization entanglement is significantly improved. Furthermore, by tuning the pump polarization and film orientation, and applying spatial filtering, the concurrence of the two-photon state is optimized to near one, meaning maximal entanglement. Such an ultrathin and spatial-separated-entangled photon-pair source will be useful in realizing miniaturized quantum photonic systems for various applications.
Tunable photonic quantum entanglement promises to advance information processing beyond classical approaches, facilitating applications in quantum communications, imaging and computing. A practical approach to preparing quantum entanglement at room temperature is to engineer photon-pair generation through spontaneous parametric down-conversion (SPDC). Nonlinear flat-optics devices, incorporating subwavelength-thick nonlinear materials, are emerging as new platforms for generating photon pairs at the nanoscale. In particular, nanostructured metasurfaces supporting optical resonances can enhance and tailor SPDC processes, allowing for the generation of spectral, polarization, and spatial entanglement [1]. However, the tunability of polarization entanglement is subject to the symmetry of nonlinear tensors of materials, where the pump photon polarization serves as the only tuning parameter [2].