The rotation of trapped molecules offers a promising platform for quantum technologies and quantum information processing. In parallel, quantum error correction codes that can protect quantum information encoded in rotational states of a single molecule have been developed. These codes are currently an abstract concept, as no implementation strategy is yet known. Here, we present a step towards experimental implementation of one family of such codes, namely absorption-emission codes. We first construct architecture-agnostic check and correction operators. These operators are then decomposed into elements of the quantum logic spectroscopy toolbox that is available for molecular ions. We then describe and analyze a measurement-based sequential as well as an autonomous implementation strategy in the presence of thermal background radiation, a major noise source for rotation in polar molecules. The presented strategies and methods might enable robust sensing or even fault-tolerant quantum computing using the rotation of individual molecules.
The rotation of trapped molecules offers a promising platform for quantum technologies and quantum information processing. In parallel, quantum error correction codes that can protect quantum information encoded in rotational states of a single molecule have been developed. These codes are currently an abstract concept, as no implementation strategy is yet known. Here, we present a step towards experimental implementation of one family of such codes, namely absorption-emission codes. We first construct architecture-agnostic check and correction operators. These operators are then decomposed into elements of the quantum logic spectroscopy toolbox that is available for molecular ions. We then describe and analyze a measurement-based sequential as well as an autonomous implementation strategy in the presence of thermal background radiation, a major noise source for rotation in polar molecules. The presented strategies and methods might enable robust sensing or even fault-tolerant quantum computing using the rotation of individual molecules.
The construction of a large-scale fault-tolerant quantum computer is an outstanding scientific and technological goal. It holds the promise to allow us to solve a variety of complex problems such as factoring large numbers, quick database search, and the quantum simulation of many-body quantum systems in fields as diverse as condensed matter, quantum chemistry, and even high-energy physics. Sophisticated theoretical protocols for reliable quantum information processing under imperfect conditions have been de-veloped, when errors affect and corrupt the fragile quantum states during storage and computations. Arguably, the most realistic and promising ap-proach towards practical fault-tolerant quantum computation are topologi-cal quantum error-correcting codes, where quantum information is stored in interacting, topologically ordered 2D or 3D many-body quantum systems. This approach offers the highest known error thresholds, which are already today within reach of the experimental accuracy in state-of-the-art setups. A combination of theoretical and experimental research is needed to store, protect and process fragile quantum information in logical qubits effectively so that they can outperform their constituting physical qubits. Whereas small-scale quantum error correction codes have been implemented, one of the main theoretical challenges remains to develop new and improve existing efficient strategies (so-called decoders) to derive (near-)optimal error cor-rection operations in the presence of experimentally accessible measurement information and realistic noise sources. One main focus of this project is the development and numerical implementation of scalable, efficient decoders to operate topological color codes. Additionally, we study the feasibility of im-plementing quantum error-correcting codes fault-tolerantly in near-term ion traps. To this end, we use realistic modeling of the different noise sources, computer simulations, and most modern quantum information approaches to quantum circuitry and noise suppression techniques.
Polar molecules trapped in optical tweezer arrays offer a promising platform for quantum information processing, providing precise control and long-range interactions that enable high-fidelity gate operations. We investigate quantum error correction in this system and show the influence of underlying physical noise. A mapping is constructed from a molecular tweezer array onto a rotated surface code in which a single specification of the array, namely, which code qubits share a molecule and where those molecules are located, determines both the correlated erasure structure and the dipolar exchange graph. We compare molecular encodings with rotational qudit dimensions (D), two and four under heralded molecular loss, coherent dipolar exchange, and imperfect heralding. It is found that a D= 4 encoding with spatially dispersed pairing exhibits a finite distance crossing at approximately the same per molecule loss rate as D= 2, while using 48-49 % fewer molecules, at the cost of a 6-10 % increase in sub-threshold logical error. Fixing the encoding and varying only the spatial embedding produces substantially larger effects: pairing the two co-located qubits along a lattice direction yields a logical-sector asymmetry of approximately fifty times. Over the simulated distances (d = 5, 7, 9), the disfavoured sector shows little or no suppression of logical error with increasing code distance, whereas the favoured sector improves by a factor of 1.5-2.3. We also find that Pauli twirl of the exchange interaction overestimates the logical error rate, which we attribute to the excitation-conserving structure of the interaction. These results reveal that the spatial embedding of correlated loss units is an important design parameter for molecular architectures and that single-sector benchmarks may be insufficient when correlated loss has directional structure.
Quantum computation promises to revolutionize information processing by exploiting superposition and entanglement, enabling applications such as quantum simulation, combinatorial optimization, and secure quantum communication. Beyond individual processors, the quantum internet aims to connect quantum nodes through entanglement distribution, enabling distributed computation. However, quantum states are fragile: environmental interactions, imperfect gate operations, and measurement errors can quickly degrade encoded information. Reliable quantum computation therefore requires carefully designed quantum error-correcting codes and fault-tolerant protocols. Unlike classical redundancy schemes, quantum error correction must preserve delicate phase relationships and relies on indirect error detection through syndrome extraction with ancillary qubits, enabling error identification without collapsing encoded states. Topological codes, in particular, emerged early as the preferred choice for many architectures due to their planar structure, local interactions, and natural support for fault-tolerant logical operations. Color codes, for instance, allow transversal implementation of all Clifford gates, whereas non-Clifford operations require magic-state injection. More recent constructions, including quantum low-density parity-check codes, offer higher encoding rates and reduced resource overhead, but require long-range qubit connectivity and more complex protocols. Despite experimental progress, several challenges remain. Many platforms exhibit biased noise, motivating codes that exploit channel asymmetry. Real-time decoding remains a critical bottleneck, as fault-tolerant computation requires low-latency processing of rapidly generated syndrome data. Fault-tolerant logical state initialization also remains resource-intensive and scales poorly with code distance. Addressing these challenges, this thesis develops a unified framework spanning theory and experiment. It provides precise performance analysis of quantum error-correcting codes in the low physical error-rate regime, introduces codes tailored to biased noise, develops fast low-complexity decoding algorithms for real-time operation, and presents modular and efficient protocols for fault-tolerant state preparation of CSS codes. The latter is demonstrated experimentally through the preparation of a logical zero state of the Golay code on the Quantinuum H2 trapped-ion quantum computer.
Noise is one of the central obstacles to building useful quantum computers, and quantum error correction (QEC) provides the framework for protecting quantum information against it. Unlike classical error correction, QEC must preserve fragile quantum states without copying them, measuring them directly, or destroying the information they encode. Driven by rapid progress in both theory and experiment, this challenge has grown into one of the most active areas of quantum information science. This tutorial gives a guided introduction to modern QEC, developing the core concepts of codes, syndromes, stabilizers, decoding, and fault tolerance before connecting them to major code families and current research directions. We cover both established constructions and newer developments, including topological and subsystem codes, bosonic and qudit codes, dynamical codes, and quantum low-density parity-check (qLDPC) codes. The emphasis is on building operational understanding: explaining not only what the main objects are, but how they are used in code design, error diagnosis, decoding, and fault-tolerant computation. The tutorial is intended for newcomers seeking a first path through QEC, as well as researchers looking for a coherent reference for the concepts, code families, and tools that arise in current work.
Diatomic molecular codes [V. V. Albert, J. P. Covey, and J. Preskill, Robust encoding of a qubit in a molecule, Phys. Rev. X 10, 031050 (2020).PRXHAE2160-330810.1103/PhysRevX.10.031050] are designed to encode quantum information in the orientation of a diatomic molecule, allowing error correction from small torques and changes in angular momentum. Here, we directly study noise native to atomic and molecular platforms-spontaneous emission, stray electromagnetic fields, and Raman scattering-and show that diatomic molecular codes fail against this noise. We derive simple conditions that are sufficient for codes to protect against such noise. We also identify existing and develop new absorption-emission (Æ) codes that are more practical than molecular codes, require lower average momentum, can directly protect against photonic processes up to arbitrary order, and are applicable to a broader set of atomic and molecular systems.
Abstract Molecular Nanomagnets may enable the implementation of qudit-based quantum error-correction codes which exploit the many spin levels naturally embedded in a single molecule, a promising step towards scalable quantum processors. To fully realize the potential of this approach, a microscopic understanding of the errors corrupting the quantum information encoded in a molecular qudit is essential, together with the development of tailor-made quantum error correction strategies. We address these central points by first studying dephasing effects on the molecular spin qudit produced by the interaction with surrounding nuclear spins, which are the dominant source of errors at low temperatures. Numerical quantum error correction codes are then constructed, by means of a systematic optimization procedure based on simulations of the coupled system-bath dynamics, that provide a striking enhancement of the coherence time of the molecular computational unit. The sequence of pulses needed for the experimental implementation of the codes is finally proposed.