Chiral quantum optics is central to developing scalable quantum networks, yet existing approaches rely predominantly on linear single-photon regimes. It remains unclear how to generate directional multiphotons. Here we show that giant emitters coupled to nonlinear quantum optical baths enable tunable directional correlated photons, revealing a mechanism for multiphoton directional emission. We demonstrate that the propagation phases of correlated photons, together with the coupling phases of giant emitters, can generate destructive interference in one direction while enhancing emission in the opposite direction, making directionality fully tunable. Building on this mechanism, we introduce a nonlinear cascaded quantum network paradigm mediated by “correlated flying qubits”, providing a configurable building block enabling distinct many-body applications beyond linear unidirectional setups. These results reveal a rich landscape for engineering multiphoton propagation and correlations through interference in giant emitter-nonlinear bath architectures, offering pathways for quantum networks and strongly correlated light-matter platforms. Chiral quantum optics is a prerequisite for communication protocols in quantum networks, but current methods are limited to the single-photon regime. The authors demonstrate that multiple giant emitters coupled to a nonlinear waveguide enable tunable multiphoton directional emission via interference, establishing a configurable building block for multiphoton cascaded quantum networks.
Chiral quantum optics is central to developing scalable quantum networks, yet existing approaches rely predominantly on linear single-photon regimes. It remains unclear how to generate directional multiphotons. Here we show that giant emitters coupled to nonlinear quantum optical baths enable tunable directional correlated photons, revealing a mechanism for multiphoton directional emission. We demonstrate that the propagation phases of correlated photons, together with the coupling phases of giant emitters, can generate destructive interference in one direction while enhancing emission in the opposite direction, making directionality fully tunable. Building on this mechanism, we introduce a nonlinear cascaded quantum network paradigm mediated by “correlated flying qubits”, providing a configurable building block enabling distinct many-body applications beyond linear unidirectional setups. These results reveal a rich landscape for engineering multiphoton propagation and correlations through interference in giant emitter-nonlinear bath architectures, offering pathways for quantum networks and strongly correlated light-matter platforms. Chiral quantum optics is a prerequisite for communication protocols in quantum networks, but current methods are limited to the single-photon regime. The authors demonstrate that multiple giant emitters coupled to a nonlinear waveguide enable tunable multiphoton directional emission via interference, establishing a configurable building block for multiphoton cascaded quantum networks.
Chiral interactions enable directional control of quantum light, providing new routes for nonreciprocal photon dynamics. While previous studies focused on single photon regimes, this work explores the non-Markovian multiphoton regime in a giant nonlinear system nonlocally coupled to a one-dimensional waveguide, with a tunable phase difference breaking parity symmetry. We show that single-photon transport remains reciprocal, but multiphoton dynamics become chiral, generating direction-dependent higher-order correlations and enabling deterministic creation of multiphoton states with nontrivial statistics from a single input direction, even under strong dissipation. The non-Markovian nature allows tuning of transmitted photon statistics via the coupling-point separation. At a specific phase, internal dynamics become Markovian while output photons retain non-Markovian features. Under strong coherent driving, we uncover nonreciprocal dissipative phase transitions and demonstrate how non-Markovianity shapes the critical response. This framework offers a general strategy for controlling chiral multiphoton dynamics in nonlocally coupled waveguide QED systems. Chiral light-matter interactions offer directional control of quantum states. This work demonstrates that a giant quantum emitter with tunable nonlocal coupling to a waveguide enables direction-dependent multiphoton correlations and dissipative phase transitions, providing a route to engineer non-Markovian chiral dynamics.
Strongly correlated multi-photon states are indispensable resources for advanced quantum technologies, yet their deterministic generation remains challenging due to the inherent weak nonlinearity in most optical systems. Here, we propose a scalable architecture for producing correlated few-photon entangled states via cascaded inelastic scattering in a nonlinear waveguide. When a single photon scatters off a far detuned excited two-level emitter, it coherently converts into a propagating doublon, a bound photon pair with anomalous dispersion. This doublon can subsequently scatter off a downstream excited emitter to further convert into a triplon, and so on, thereby establishing a photon-number amplification cascade ∣⋅⟩→∣:⟩→∣∴⟩→... Central to this process is the concept of a pseudo-giant atom, which we introduce here to capture the non-local scattering potential emergent from the wave functions of bound states. By implementing this scheme using a real giant atom with multiple engineered coupling points, we achieve unidirectional and full controllable photon conversion without backscattering. The resulting output state forms a programmable superposition of spatially and temporally isolated photon-number components, automatically sorted by their distinct group velocities. This work opens a new paradigm in quantum state engineering, enabling on-demand generation of complex multi-photon resources for quantum simulation, metrology, and scalable quantum networks.
Chiral quantum emitters interact with light only in one propagation direction, allowing them to be linked into cascaded systems in which photons mediate ordered, long-range interactions. Such systems are predicted to host novel regimes of many-body physics of light and matter. Exploring these regimes requires arrays of identical quantum emitters with directional, low-loss coupling to guided photons, a combination that has thus far remained experimentally out of reach. Here we realize a cascaded network of superconducting qubits using an architecture that overcomes these bottlenecks. We implement a four-qubit chain spanning two modules, with separations ranging from millimeters to half a meter, and exploit the shared waveguide as a dissipative resource to stabilize reconfigurable entanglement, reaching a genuinely multipartite regime unavailable in reciprocal baths. By scattering weak pulses off the chain, we observe photons sorted in time by photon number, a signature of the strong photon-photon interactions mediated by the emitters. Together, these results provide experimental access to many-body light-matter regimes that are beyond the reach of reciprocal systems.
The realization of correlated multiphoton processes usually depends on the interaction between nonlinear media and atoms. However, the nonlinearity of optical materials is generally weak, making it still very challenging to achieve correlated multiphoton dynamics at the few-photon level. Meanwhile, giant atoms, with their capability for multipoint coupling, which is a novel paradigm in quantum optics, mostly focus on the single-photon field. In this work, by using the method described in Phys. Rev. Res. 6, 013279 (2024), we reveal that the ladder-type three-level giant atom spontaneously emits strongly correlated photon pairs with high efficiency by designing and optimizing the target function. In addition, by encoding local phases into the optimal coupling sequence, directional two-photon correlated transfer can be achieved. This method does not require a nonlinear waveguide and can be realized in the conventional environment. We show that the photon pairs emitted in both the bidirectional and the chiral case exhibit strong correlation properties in both time and space. Such correlated photon pairs have great potential applications for quantum information processing. For example, numerical results show that our proposal can realize the two-photon mediated cascaded quantum system.
Nonlocal light-matter interactions with giant atoms in high-dimensional environments are not only fundamentally intriguing for testing quantum electrodynamics beyond the dipole approximation but also crucial for building high-dimensional quantum networks and engineering multipartite entangled states. Given the enigmatic and largely uncharted collective signatures exhibited by multiple giant atoms within two-dimensional optical baths, we delve into their nonperturbative collective dynamics within the single-excitation subspace, focusing on the case where they are coupled to a common two-dimensional photonic reservoir and employing a resolvent operator approach. We demonstrate that precisely engineered atomic arrangements lead to unconventional quantum dynamics, featuring non-Markovianity-induced beats and long-lived bound states in the continuum, thereby providing a versatile platform for implementing two-dimensional quantum memory. Phenomenologically, we observe the emergence of exotic photon emission patterns in both two- and three-dimensional (3D) baths. The emission directions are shown to be precisely controllable on demand through exact phase engineering of the coupling parameters, enabling a highly efficient chiral light-matter interface. Moreover, our generalization to a 3D bath reveals that coherent dipole-dipole interactions can survive despite the coupling to a continuum of modes, a finding that challenges conventional wisdom regarding decoherence.
Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects can further result in directionality of the emission, thus offering a complimentary implementation of chiral quantum optics. Waveguide quantum electrodynamics (QED) allows coupling between spatially separated emitters, enabling selective driving. In this work, we control the emission direction for a pair of quantum dots embedded in a bidirectional photonic crystal waveguide offering independent electrical tuning. Notably the emitters are 13 \micro m apart, which corresponds to 26 effective wavelengths, but are nevertheless radiatively coupled. The directionality arises from a dispersive dipole-dipole interaction, which shifts the energy of the collective states, so that the emitter pair effectively forms an artificial molecule. We show that the emission direction can be switched from left- to rightwards by manipulating the relative driving phase while collectively exciting the emitters. In addition, we observe directional photon statistics under continuous driving, with, for example, single photons detected on one output port, and photon pairs on the other. With pulsed excitation, both emitters are fully inverted and correlated photon pairs are observed in time-resolved intensity correlation measurements. This work demonstrates a novel implementation of chiral quantum optics using quantum dots coupled via a non-chiral waveguide, and reports key steps for scaling up as a multi-emitter waveguide QED platform.