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arXiv:2404.07967 · Physical Review Applied

Spin-energy entanglement of a time-focused neutron

J. Leiner, Stephen J. Kuhn, S. McKay, Johanna K. Jochum, Fankang Li, Abu Ashik Irfan, Fumiaki Funama, Denis Mettus, L. Beddrich, Christian Franz, Jiazhou Shen, Steven R. Parnell, Robert M. Dalgliesh, Matthew Loyd, Niels Geerits, Gerardo Ortíz, C. Pfleiderer, R. Pynn

Published Sep 25, 2024• 3 citations
arXivHTMLPDF

Abstract

Quantum entanglement in a neutron beam? Yup. The spectroscopic technique known as neutron resonant spin echo (NRSE) extracts the dynamical correlation function with comparatively high resolution. Underlying the unique capabilities of NRSE beamlines is how they label the velocity (energy) of neutrons with Larmor spin precession to set up a spin-echo signal. This Letter provides proof of concept that the way such beamlines manipulate the spin and energy of an individual neutron in fact entangles those degrees of freedom, which can be observed with a quantum contextuality witness. This suggests that the technique could serve as a direct probe of entanglement in condensed matter.

DOI
10.1103/physrevapplied.22.l031005

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Quantum entanglement in a neutron beam? Yup. The spectroscopic technique known as neutron resonant spin echo (NRSE) extracts the dynamical correlation function with comparatively high resolution. Underlying the unique capabilities of NRSE beamlines is how they label the velocity (energy) of neutrons with Larmor spin precession to set up a spin-echo signal. This Letter provides proof of concept that the way such beamlines manipulate the spin and energy of an individual neutron in fact entangles those degrees of freedom, which can be observed with a quantum contextuality witness. This suggests that the technique could serve as a direct probe of entanglement in condensed matter.
The development of direct probes of entanglement is integral to the rapidly expanding field of complex quantum materials.Here we test the robustness of entangled neutrons as a quantum probe by measuring the Clauser-Horne-Shimony-Holt contextuality witness while varying the beam properties.Specifically, we show that the mode entanglement of the spin and path subsystems of individual neutrons prepared in two different experiments using two different apparatuses persists even after varying the entanglement length, coherence length, and neutron energy difference of the paths.The two independent apparatuses acting as entangler-disentangler pairs are static-field magnetic Wollaston prisms and resonance-field radio-frequency flippers.Our results show that the spatial and energy properties of the neutron beam may be significantly altered without reducing the contextuality witness value below the Tsirelson bound, meaning that maximum entanglement is preserved.We also show that two paths may be considered distinguishable even when the path states significantly overlap.Therefore, we have shown that our experimental results are consistent with the distinguishable subsystem assumption down to a separation of less than 100 nm, proving entanglement and the contextual nature of reality on short length scales.This work is the key step in the realization of the modular, robust technique of entangled neutron scattering, which can extract entanglement information from a sample without the knowledge of the microscopic sample Hamiltonian: only semiquantitative knowledge of the correlation lengths of the relevant degrees of freedom and the timescales of the characteristic dynamics is required.
Neutron resonance spin-echo (NRSE) phenomena are investigated experimentally and theoretically. In our experiments, spin precession produced in a classical manner and by neutron resonance is combined as two arms of a spin-echo machine. A magnetic-field scan in the classical SE coil reveals a spin-echo signal of the precession produced by the NRSE arm. The neutron spin-flip probability $\ensuremath{\rho}$ in the resonance coils turns out to be a key parameter of the NRSE arm. The limiting cases $\ensuremath{\rho}=0$ and $\ensuremath{\rho}=1$ lead, respectively, to Larmor precession with phase ${\ensuremath{\varphi}}_{1}$ in the static magnetic fields of the NR flippers or to NRSE precession with ${\ensuremath{\varphi}}_{2}.$ The case $0<\ensuremath{\rho}<1$ produces quantum interference resulting in additional echoes with phases ${\ensuremath{\varphi}}_{3}=({\ensuremath{\varphi}}_{1}+{\ensuremath{\varphi}}_{2})/2$ and ${\ensuremath{\varphi}}_{4}=\ifmmode\pm\else\textpm\fi{}({\ensuremath{\varphi}}_{1}\ensuremath{-}{\ensuremath{\varphi}}_{2})/2.$ The amplitude of each pattern depends on the spin-flip probability $\ensuremath{\rho}$ and the initial polarization. These experiments demonstrate explicitly the quantum-mechanical principle of linear spin state superposition of neutron particle waves, and the interference as a result of that.
The development of qualitatively new measurement capabilities is often a prerequisite for critical scientific and technological advances. Here we introduce an unconventional quantum probe, an entangled neutron beam, where individual neutrons can be entangled in spin, trajectory and energy. The spatial separation of trajectories from nanometers to microns and energy differences from peV to neV will enable investigations of microscopic magnetic correlations in systems with strongly entangled phases, such as those believed to emerge in unconventional superconductors. We develop an interferometer to prove entanglement of these distinguishable properties of the neutron beam by observing clear violations of both Clauser-Horne-Shimony-Holt and Mermin contextuality inequalities in the same experimental setup. Our work opens a pathway to a future of entangled neutron scattering in matter.
Neutrons are proper tools for testing basic laws of quantum physics since they are massive and can be handled and measured with high efficiency. Suitable postselection experiments demonstrate coherence features of sub-ensembles even when the whole ensemble seems to have lost its coherence. All experiments have the capacity to explain more details by additional pre- and post-selection methods. It will be shown that specific losses are unavoidable in any interaction. Coherence and decoherence are intrinsic quantum effects and can shed light on the measurement problem. Quantum contextuality is a consequence of the entanglement of different degrees of freedom. This makes quantum phenomena more strongly correlated than classical ones. Most experiments have been performed with perfect neutron interferometers and some others by using ultracold neutrons and spin-echo systems. An event by event based interpretation can also be brought into agreement with the experimental results. In many cases parasitic beams carry the same information as the main beam and this relates such measurements to "weak" measurements. The coupling and entanglement of various parameter spaces guide us to a more elaborate discussion of quantum effects.
The transition between the quantum and classical world is a topical problem in quantum physics, which can be investigated by neutron interferometric methods. Here we discuss unavoidable quantum losses as they appear in neutron phase-echo and spin rotation experiments and we show how entanglement effects in a single-particle system demonstrate quantum contextuality, i.e. an entanglement between external and internal degrees of freedom in single-particle systems. This contextuality phenomenon also shows that a quantum system carries much more information than usually extracted. In all cases of an interaction, parasitic beams are produced which cannot be recombined completely with the original beam. This means that a complete reconstruction of the original state is, in principle, impossible which causes a kind of intrinsic irreversibility. Even small interaction potentials can have huge effects when they are applied in quantum Zeno-like experiments. The path towards advanced neutron quantum optics will be discussed.
Neutron matter-wave optics provides the basis for new quantum experiments and a step towards applications of quantum phenomena. Most experiments have been performed with a perfect crystal neutron interferometer where widely separated coherent beams can be manipulated individually. Various geometric phases have been measured and their robustness against fluctuation effects has been proven, which may become a useful property for advanced quantum communication. Quantum contextuality for single particle systems shows that quantum correlations are to some extent more demanding than classical ones. In this case entanglement between external and internal degrees of freedom offers new insights into basic laws of quantum physics. Non-contextuality hidden variable theories can be rejected by arguments based on the Kochen-Specker theorem.