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arXiv:2404.06426 · Physical review. E

Quantum stochastic thermodynamics in the mesoscopic-leads formulation

Laetitia P. Bettmann, Michael J. Kewming, Gabriel Teixeira Landi, John Goold, Mark T. Mitchison

Published Jun 5, 2025• 4 citations
arXivHTMLPDF

Abstract

We introduce a numerical method to sample the distributions of charge, heat, and entropy production in open quantum systems coupled strongly to macroscopic reservoirs, with both temporal and energy resolution and beyond the linear-response regime. Our method exploits the mesoscopic-leads formulation, where macroscopic reservoirs are modeled by a finite collection of modes that are continuously damped toward thermal equilibrium by an appropriate Gorini-Kossakowski-Sudarshan-Lindblad master equation. Focussing on noninteracting fermionic systems, we access the time-resolved full counting statistics through a trajectory unraveling of the master equation. We show that the integral fluctuation theorems for the total entropy production, as well as the martingale and uncertainty entropy production, hold. Furthermore, we investigate the fluctuations of the dissipated heat in finite-time information erasure. Conceptually, our approach extends the continuous-time trajectory description of quantum stochastic thermodynamics beyond the regime of weak system-environment coupling.

DOI
10.1103/3msj-9qgb

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We introduce a numerical method to sample the distributions of charge, heat, and entropy production in open quantum systems coupled strongly to macroscopic reservoirs, with both temporal and energy resolution and beyond the linear-response regime. Our method exploits the mesoscopic-leads formulation, where macroscopic reservoirs are modeled by a finite collection of modes that are continuously damped toward thermal equilibrium by an appropriate Gorini-Kossakowski-Sudarshan-Lindblad master equation. Focussing on noninteracting fermionic systems, we access the time-resolved full counting statistics through a trajectory unraveling of the master equation. We show that the integral fluctuation theorems for the total entropy production, as well as the martingale and uncertainty entropy production, hold. Furthermore, we investigate the fluctuations of the dissipated heat in finite-time information erasure. Conceptually, our approach extends the continuous-time trajectory description of quantum stochastic thermodynamics beyond the regime of weak system-environment coupling.
We study the thermalization dynamics and thermodynamics of a qubit coupled to a structured, memory-carrying environment modeled as a single bosonic mode continuously thermalized by a Markovian bath. The competition between coherent qubit-mode coupling g and thermalization rate κ is controlled by the dimensionless ratio μ=g/κ, which drives a crossover between Markovian and strongly non-Markovian regimes. In the strongly non-Markovian limit, coherent energy exchange produces transient shortcuts to local thermalization, whereby the qubit approaches its thermal state long before global equilibration. In the opposite limit, we derive an original convolution master equation with an exponential memory kernel, which reduces to a thermal GKSL equation as μ→0. The crossover between the two regimes closely mirrors the underdamped-to-overdamped transition of a classical damped oscillator. From the thermodynamic side, we derive an original decomposition of the reduced entropy production in terms of qubit-ancilla mutual information and ancilla relative entropy, providing a quantitative fingerprint of non-Markovian corrections. We then extend this framework to the stochastic level via two monitoring protocols — Fock-state tracking and energy-exchange detection — constructing trajectory-level entropy productions and establishing fluctuation theorems tailored to each scheme. Together, these results demonstrate that a self-consistent stochastic thermodynamics can be formulated for non-Markovian open quantum systems under continuous monitoring.
Understanding the entropy production of systems strongly coupled to thermal baths is a core problem of both quantum thermodynamics and mesoscopic physics. While many techniques exist to accurately study entropy production in such systems, they typically require a microscopic description of the baths, which can become numerically intractable to study for large systems. Alternatively an open-systems approach can be employed with all the nuances associated with various levels of approximation. Recently, the mesoscopic leads approach has emerged as a powerful method for studying such quantum systems strongly coupled to multiple thermal baths. In this method, a set of discretized lead modes, each locally damped, provide a Markovian embedding. Here we show that this method proves extremely useful to describe entropy production of a strongly coupled open quantum system. We show numerically, for both noninteracting and interacting setups, that a system coupled to a single bath exhibits a thermal fixed point at the level of the embedding. This allows us to use various results from the thermodynamics of quantum dynamical semigroups to infer the nonequilibrium thermodynamics of the strongly coupled, non-Markovian central systems. In particular, we show that the entropy production in the transient regime recovers the well-established microscopic definitions of entropy production with a correction that can be computed explicitly for both the single- and multiple-lead cases.
Thermodynamics typically concerns the physical behaviour of macroscopic systems comprised of many particles. However, recent theoretical progress has extended the theory to both the classical-stochastic and quantum regimes, where systems are comprised of just a small number of particles. In this thesis I investigate a range of situations in which new thermodynamic phenomena emerge due to the reduced size of the systems involved. One central assumption in macroscopic thermodynamics is the weak coupling approximation, which posits that the equilibrium properties of a system are not influenced by the interactions with its surrounding environment. However, for microscopic systems this assumption can break down, and I derive new fluctuation relations that provide a refined form of the second law of thermodynamics in this strong-coupling regime, taking into account corrections stemming from these interactions. In this work I provide a characterisation of stochastic heat and entropy production for small scale classical systems that are defined regardless of the strength of interaction. I then show that these definitions lead to a consistent thermodynamic framework valid beyond the usual weak-coupling regime. The thesis also concerns the effect of interactions on the equilibrium properties of strongly-coupled quantum systems, and I investigate how these interactions can influence the resulting temperature fluctuations in this regime. Using tools from quantum estimation theory, I derive an uncertainty relation between energy and temperature valid at all coupling strengths and system sizes. The relation reveals how quantum energy coherences contribute to statistical fluctuations in the estimated temperature of small- scale systems. Finally, I investigate how quantum fluctuations influence the statistics of work extracted from slowly-driven quantum systems. I prove that, unlike in classical systems, the work dissipated by a general quantum system is no longer proportional to its statistical fluctuations. This result reveals new subtleties involved in designing optimal quantum thermodynamic processes.
I formulate a quantum stochastic thermodynamics for the quantum trajectories of a continuously monitored forced harmonic oscillator coupled to a thermal reservoir. Consistent trajectory-dependent definitions are introduced for work, heat, and entropy, through engineering the thermal reservoir from a sequence of two-level systems. Within this formalism the connection between irreversibility and entropy production is analyzed and confirmed by proving a detailed fluctuation theorem for quantum trajectories. Finally, possible experimental verifications are discussed.
We build an exact framework to evaluate heat, energy, and particle transport between Gaussian reservoirs mediated by a quadratic quantum system. By combining full counting statistics with newly developed non-Markovian master equation approaches, we introduce an effective master equation whose solution can be used to generate arbitrary moments of the heat statistics for any number of reservoirs. This theory applies equally to fermionic and bosonic systems, holds at arbitrarily strong coupling, and resolves out-of-equilibrium transient dynamics determined by the system's initial state. In the steady-state, weak-coupling limit, we recover results analogous to those of the well-known Landauer-Büttiker formalism. We conclude our discussion by demonstrating an application of the method to a prototypical fermionic system. Our results uncover a regime of transient negative heat conductance contingent upon the initial system preparation, providing a clear signature of non-trivial out-of-equilibrium dynamics.
Heat exchanged between an open quantum system and its environment exhibits fluctuations that carry crucial signatures of the underlying dynamics. Within the well-established two-point measurement scheme, we identify a “heat operator,” whose moments with respect to the vacuum state of a thermofield-doubled Hilbert space correspond to the stochastic moments of the heat exchanged with a bath. This recasts heat statistics as a unitary time evolution problem, which we solve by combining chain-mapped reservoirs with tensor-network propagation. In a multibath setup, all total and bath-resolved heat moments then follow from a single pure state evolution. We employ this approach to compute transient and steady-state heat fluctuations in Ohmic spin-boson models in and out of equilibrium, accessing the challenging low-temperature and long memory time regimes of the environment. In the nonequilibrium case, we show a crossover in the Fano factor from super-Poissonian to nearly Poissonian statistics under strong coupling asymmetry, corresponding to thermal rectification behavior. The method applies to noninteracting (bosonic or fermionic) nonequilibrium environments with arbitrary spectral densities, offering a powerful, nonperturbative framework for understanding heat transfer in open quantum systems.