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arXiv:2404.00740 · Physical Review Letters

Quantum Walks and Correlated Dynamics in an Interacting Synthetic Rydberg Lattice

Tao Chen, Chenxi Huang, Bryce Gadway, Jacob P. Covey

Published Sep 18, 2024• 12 citations
arXivHTMLPDF

Abstract

Coherent dynamics of interacting quantum particles plays a central role in the study of strongly correlated quantum matter and the pursuit of quantum information processors. Here, we present the state space of interacting Rydberg atoms as a synthetic landscape on which to control and observe coherent and correlated dynamics. With full control of the coupling strengths and energy offsets between the pairs of sites in a nine-site synthetic lattice, we realize quantum walks, Bloch oscillations, and dynamics in an Escher-type "continuous staircase." In the interacting regime, we observe correlated quantum walks, Bloch oscillations, and confinement of particle pairs. Additionally, we simultaneously tilt our lattice both up and down to achieve coherent pair oscillations. When combined with a few straightforward upgrades, this work establishes synthetic Rydberg lattices of interacting atom arrays as a promising platform for programmable quantum many-body dynamics with access to features that are difficult to realize in real-space lattices.

DOI
10.1103/physrevlett.133.120604

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Coherent dynamics of interacting quantum particles plays a central role in the study of strongly correlated quantum matter and the pursuit of quantum information processors. Here, we present the state space of interacting Rydberg atoms as a synthetic landscape on which to control and observe coherent and correlated dynamics. With full control of the coupling strengths and energy offsets between the pairs of sites in a nine-site synthetic lattice, we realize quantum walks, Bloch oscillations, and dynamics in an Escher-type "continuous staircase." In the interacting regime, we observe correlated quantum walks, Bloch oscillations, and confinement of particle pairs. Additionally, we simultaneously tilt our lattice both up and down to achieve coherent pair oscillations. When combined with a few straightforward upgrades, this work establishes synthetic Rydberg lattices of interacting atom arrays as a promising platform for programmable quantum many-body dynamics with access to features that are difficult to realize in real-space lattices.
Full control over the dynamics of interacting, indistinguishable quantum particles is an important prerequisite for the experimental study of strongly correlated quantum matter and the implementation of high-fidelity quantum information processing. We demonstrate such control over the quantum walk-the quantum mechanical analog of the classical random walk-in the regime where dynamics are dominated by interparticle interactions. Using interacting bosonic atoms in an optical lattice, we directly observed fundamental effects such as the emergence of correlations in two-particle quantum walks, as well as strongly correlated Bloch oscillations in tilted optical lattices. Our approach can be scaled to larger systems, greatly extending the class of problems accessible via quantum walks.
Synthetic dimensions, wherein dynamics occurs in a set of internal states, have found great success in recent years in exploring topological effects in cold atoms and photonics. However, the phenomena thus far explored have largely been restricted to the non-interacting or weakly interacting regimes. Here, we extend the synthetic dimensions playbook to strongly interacting systems of Rydberg atoms prepared in optical tweezer arrays. We use precise control over driving microwave fields to introduce a tunable U(1) flux in a four-site lattice of coupled Rydberg levels. We find highly coherent dynamics, in good agreement with theory. Single atoms show oscillatory dynamics controllable by the gauge field. Small arrays of interacting atoms exhibit behavior suggestive of the emergence of ergodic and arrested dynamics in the regimes of intermediate and strong interactions, respectively. These demonstrations pave the way for future explorations of strongly interacting dynamics and many-body phases in Rydberg synthetic lattices.
The creation and coherent control of systems of many strongly-interacting quantum particles represents one of the most important challenges in quantum science and technology. Devices capable of performing such a task have applications ranging from sensing and simulation, to communications and computation. The past few decades have seen remarkable progress in the development of different platforms to address the challenges of isolating and controlling individual quantum objects and increasing the number of interacting elements. This thesis presents a novel platform using arrays of individually controlled neutral atoms in optical tweezers which enables high-fidelity control of large systems of strongly interacting particles. Using real-time imaging and feedback, we initialize the positions of hundreds of atoms in arbitrary one- and two-dimensional geometries. By coupling the internal state of the atoms to highly excited Rydberg states, we are able to introduce spatially-dependent interactions to the system. Combining the remarkable coherence properties of isolated neutral atoms with strong Rydberg interactions, we study complex spin Hamiltonians in regimes beyond classical simulability. In the context of quantum simulation, we use this platform to study the phase diagram of regular arrays, including the critical properties of some of the associated quantum phase transitions. Additionally, we report on the discovery of special slowly-thermalizing states known as quantum many-body scars, which are then used as a starting point to stabilize many-body dynamics across the Hilbert space. Through the addition of specialized local controls, we demonstrate the ability to generate large N-partite entangled states with up to 20 atoms, as well as the ability to implement quantum logic gates. We combine quantum simulation with quantum information processing by preparing states with signatures of quantum spin liquids, which may be developed as topologically protected qubits. Lastly, we explore the potential applications of this platform to classical combinatorial optimization problems by approximating the Maximum Independent Set of different graphs.
Synthetic dimensions are powerful tools for quantum simulation and computation. They are realized by harnessing internal or external degrees of freedom of an atom or molecule, which can mimic the motion of an electron in a real-space lattice potential. Such degrees of freedom are highly tunable and can be engineered to create configurations difficult to access or realize in real space. Some of the exciting possibilities include realizing higher dimensions systems[1, 2, 3], nontrivial real space[4, 5] and band structure[6, 7] topologies and artificial gauge fields[8, 9]. Experiments have utilized various degrees of freedom to create synthetic dimensions, such as motional[10, 11], spin[8, 12, 13, 14] and rotational[15] levels of atoms and molecules, and frequency modes, spatial modes, and arrival times in photonic systems[16]. Atomic synthetic dimensions have demonstrated artificial gauge fields, spin-orbit coupling, chiral edge states using Raman-coupled ground magnetic sublevels[8, 12, 17] of atoms, and phenomena such as Anderson localization using two-photon Bragg transitions by coupling free-particle momentum states[18]. Here, we harness the Rydberg levels of 84Sr to realize a synthetic lattice for studying quantum matter. Resonant millimeter-wave (mm-wave) radiation coupling Rydberg levels |i⟩ and |j⟩ with amplitude Ωij (Rabi frequency) are described by the same Hamiltonian as a particle tunneling between lattice sites |i⟩ and |j⟩ with tunneling amplitude Jij = Ωij /2. The mathematical equivalence to particles moving in a real-space lattice enables Rydberg levels to function as a synthetic spatial dimension. Rydberg-atom synthetic dimensions offer control over connectivity, tunneling rates and on-site potentials, which allows for the creation of a broad range of synthetic dimensional system. The capabilities of such a system are demonstrated by realizing the famous Su-Schrieffer-Heeger (SSH) model[19] and studying its topologically protected edge states(TPS).
"The many weird properties of quantum mechanics at the very small scale have led to surprising and useful discoveries that manifest at the macroscopic level, like the quantum Hall effect and high temperature superconductivity. Yet trying to understand the origin of correlated behavior from interacting quantum systems via classical simulation requires an infeasible level of computing power. Instead, we can use an easily tunable, clean quantum system as a quantum simulation of a more unwieldy system, building the same model to study the same physics, but in a more controlled environment. Our field of cold neutral atoms in optical lattices has seen success over many years as a platform for quantum simulation of various lattice models from condensed matter physics. The recent (2015) implementation of lattices not in position, but in a synthetic dimension by coupling individual quantum states with lasers has led to a more bottom-up approach to engineering lattice models. In this thesis, we present our ""momentum-space lattice"" technique in which we use individual laser frequencies to couple the momentum states of a rubidium-87 Bose-Einstein condensate, in order to create lattices with site-by-site and link-by-link precision. This technique is simple to implement experimentally, requiring just two additional common optical components (acousto-optic modulators) compared to a real-space lattice, yet is incredibly versatile. Using momentum-space lattices, we have studied the physics of artificial magnetic fields, disorder and pseudodisorder-induced localization, and atomic interactions across eight works described in this thesis. More interesting are the not-so-well-known effects that arise in the interplay among these three components of topology, disorder, and interactions, and we have made headway towards studying physics in this regime. To be more specific, in our studies we have generated an artificial magnetic field for neutral atoms, and directly observed the resulting chiral currents in both a square ladder and zigzag lattice geometry. We have further monitored the quantum walk behavior of atoms under disordered and pseudodisordered lattices, observing a transition to localization under a quasiperiodic potential. We have been able to introduce a tunable energy dependence to this localization transition (single-particle mobility edge) in two ways: with the addition of more tunneling pathways, and by modifying the form of the potential. Finally, we have studied the effects of nonlinear inter-atomic interactions in the momentum-space lattice, observing self-trapping in a double well system as well as on a full lattice, showing a skewed current-phase relationship in an analog to Josephson junction arrays, and investigating an interaction-induced shift in localization behavior under pseudodisorder. In constructing the momentum-space lattice apparatus, Eric, Bryce, and I have created a promising new platform for Hamiltonian engineering. The studies described here not only show off the capabilities of the technique, but also realize new models, reveal new physics, and provide a new perspective complementary to both real-space lattice techniques and real materials. We have observed topological edge states more directly than previous works and engineered precise lattice parameter variations unavailable to other techniques, and yet the best is still to come. With our ongoing experimental upgrades comes access to the regime of strong inter-particle interactions, which promises more challenging yet more rewarding experiments."
Topological pumping is a paradigmatic realization of quantized transport in band systems, yet its fate in strongly correlated regimes, especially with long-range interactions, remains largely unexplored. Here we report the experimental observation of interaction-enabled topological pumping of correlated Rydberg electrons in a synthetic lattice. We show that dipolar exchange interactions induce a controllable shift of the underlying topological singularity in parameter space, such that a fixed pumping trajectory can be driven through successive topological transitions by tuning the interaction strength alone. This leads to the emergence and breakdown of quantized transport. The observations are consistent with an effective Rice-Mele description with interaction-renormalized onsite potentials and are supported by characterizing the adiabaticity and robustness to control trajectory imperfections. Our results establish a platform for exploring interaction-controlled topological transport beyond perturbative regimes and open a route toward engineering correlated topological matter in synthetic quantum systems.