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arXiv:2403.17842 · Physical Review X

Experimental Realization of Discrete Time Quasicrystals

G. He, Bingtian Ye, Ruotian Gong, Changyu Yao, Zhongyuan Liu, Kater W. Murch, Norman Y. Yao, Chong Zu

Published Mar 12, 2025• 29 citations
arXivHTMLPDF

Abstract

Floquet (periodically driven) systems can give rise to unique nonequilibrium phases of matter without equilibrium analogs. The most prominent example is the realization of discrete time crystals. An intriguing question emerges: What other novel phases can manifest when the constraint of time periodicity is relaxed? In this study, we explore quantum systems subjected to a quasiperiodic drive. Leveraging a strongly interacting spin ensemble in diamond, we identify the emergence of long-lived discrete time quasicrystals. Unlike conventional time crystals, time quasicrystals exhibit robust subharmonic responses at multiple incommensurate frequencies. Furthermore, we show that the multifrequency nature of the quasiperiodic drive allows for the formation of diverse patterns associated with different discrete time quasicrystalline phases. Our findings demonstrate the existence of nonequilibrium phases in quasi-Floquet settings, significantly broadening the catalog of novel phenomena in driven many-body quantum systems.

DOI
10.1103/physrevx.15.011055

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Periodically driven quantum many-body systems can spontaneously reorganize their motion and start moving with a period different than the driving period. These are ``discrete time crystals'' and they have been realized already in the laboratory. It turns out that systems from the same class can spontaneously reveal quasicrystalline structures in time. The interaction between the particles forces them into a quasicrystal pattern in the time domain, in spite of the fact that the driving is periodic.

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Floquet (periodically driven) systems can give rise to unique nonequilibrium phases of matter without equilibrium analogs. The most prominent example is the realization of discrete time crystals. An intriguing question emerges: What other novel phases can manifest when the constraint of time periodicity is relaxed? In this study, we explore quantum systems subjected to a quasiperiodic drive. Leveraging a strongly interacting spin ensemble in diamond, we identify the emergence of long-lived discrete time quasicrystals. Unlike conventional time crystals, time quasicrystals exhibit robust subharmonic responses at multiple incommensurate frequencies. Furthermore, we show that the multifrequency nature of the quasiperiodic drive allows for the formation of diverse patterns associated with different discrete time quasicrystalline phases. Our findings demonstrate the existence of nonequilibrium phases in quasi-Floquet settings, significantly broadening the catalog of novel phenomena in driven many-body quantum systems.
Discrete time quasicrystals (DTQC) constitute a class of non-equilibrium matter characterized by temporal order without strict periodicity, in contrast to conventional time crystals. Investigating these phenomena is essential for expanding our fundamental understanding of far-from-equilibrium quantum matter and spontaneous symmetry breaking beyond periodic regimes. Here, we experimentally observe a DTQC in a driven-dissipative ensemble of strongly interacting Rydberg atoms, displaying non-equilibrium dynamical response with a different finite Abelian group symmetry Zm×Zn{{\mathbb{Z}}}_{m}\times {{\mathbb{Z}}}_{n}Zm​×Zn​. By applying a quasiperiodic drive using a dual-frequency drive with incommensurate frequencies, we demonstrate that the system exhibits a robust subharmonic response at multiple incommensurate frequencies, signifying the emergence of a DTQC phase. We map the full phase diagram of the system, which includes the DTQC phase, and demonstrate its rigidity against perturbations in both RF field intensity and laser detuning. Moreover, we observe a cyclic group symmetry effect that constrains the construction of Z2×Z3{{\mathbb{Z}}}_{2}\times {{\mathbb{Z}}}_{3}Z2​×Z3​-symmetric DTQC. This work establishes a versatile platform for studying non-equilibrium phases of matter and provides insights into the dynamics of time-translation symmetry breaking in quantum many-body systems. Time-crystal phases have raised both theoretical and experimental interest across various platforms. Here, the authors report the observation of a discrete time-quasicrystal in a driven-dissipative ensemble of interacting Rydberg atoms, advancing the understanding of symmetry breaking in these systems.
Floquet (periodic) driving has recently emerged as a powerful technique for engineering quantum systems and realizing nonequilibrium phases of matter. A central challenge to stabilizing quantum phenomena in such systems is the need to prevent energy absorption from the driving field. Fortunately, when the frequency of the drive is significantly larger than the local energy scales of the many-body system, energy absorption is suppressed. The existence of this so-called prethermal regime depends sensitively on the range of interactions and the presence of multiple driving frequencies. Here, we report the observation of Floquet prethermalization in a strongly interacting dipolar spin ensemble in diamond, where the angular dependence of the dipolar coupling helps to mitigate the long-ranged nature of the interaction. Moreover, we extend our experimental observation to quasi-Floquet drives with multiple incommensurate frequencies. In contrast to a single-frequency drive, we find that the existence of prethermalization is extremely sensitive to the smoothness of the applied field. Our results open the door to stabilizing and characterizing nonequilibrium phenomena in quasiperiodically driven systems.
Time quasicrystals (TQCs) represent a compelling extension of the concept of time crystals (TCs). While TCs break discrete time-translation symmetry by exhibiting a periodic response at a subharmonic of the driving frequency, TQCs display a more complex temporal order. They respond at multiple incommensurate frequencies, values that are not integer multiples of the fundamental driving frequency, resulting in quasiperiodic dynamics. In this work, we investigate the emergence of a TQC in a disordered quantum Ising chain subjected to a quasiperiodic transverse field. Using exact diagonalization, we find that the transverse magnetization exhibits quasiperiodic oscillations which persist over extended prethermal timescales before eventual decay. This indicates that the TQC exists as a long-lived, prethermal dynamical phase rather than a true equilibrium state. We further assess the robustness of this prethermal TQC against interactions and driving imperfections, confirming its stability under realistic experimental conditions. Finite-size analysis reveals that the prethermal TQC lifetime exhibits minimal dependence on system size. Additionally, we explore the emergence of TQCs in the same chain under symmetric sampling of exchange couplings. Our results demonstrate that the TQC phase is highly sensitive to both the choice of coupling distribution and the values of the driving frequencies. These findings highlight promising experimental prospects for realizing TQCs in cold atomic systems and quantum simulators, providing valuable insights into their stability, dynamical properties, and potential for exploring novel non-equilibrium quantum phases.
A discrete time crystal (DTC) is a remarkable non-equilibrium phase of matter characterized by the persistent sub-harmonic oscillations of physical observables in periodically driven many-body systems. Motivated by the question of whether such a temporal periodic order can persist when the drive becomes aperiodic, we investigate the dynamics of a Lipkin-Meshkov-Glick model under quasi-periodic Thue-Morse (TM) driving. Intriguingly, this infinite-range-interacting spin system can host "quasi-discrete time crystal" (quasi-DTC) phases characterized by periodic oscillations of the magnetization. We demonstrate that our model can host the quasi-DTC analog of both period-doubling DTCs as well as higher-order DTCs. These quasi-DTCs are robust to various perturbations, and they originate from the interplay of "all-to-all" interactions and the recursive structure of the TM sequence. Our results suggest that quasi-periodic driving protocols can provide a promising route for realizing novel non-equilibrium phases of matter in long-range interacting systems.
The classification of phases of matter has been revolutionised by topological order and nonequilibrium phenomena such as time crystals. However, a unified framework connecting temporal order, topology, and dissipation remains elusive. Here we introduce the concept of "Time-Quasicrystals"-non-equilibrium topological phases that exhibit quasi-periodic temporal order protected by dissipative dynamics. These phases emerge in driven dissipative quantum systems through the interplay of Floquet engineering and non-local dissipation, leading to an effective non-Hermitian Floquet Hamiltonian with topological edge modes in the frequency domain. We demonstrate three hallmarks of Time-Quasicrystals: (1) fractal-like temporal correlations with multiple incommensurate frequencies, (2) a quantised topological invariant robust against disorder, and (3) algebraically decaying memory of phase perturbations. We provide explicit experimental realisations in Rydberg atom arrays and circuit quantum electrodynamics platforms. Our work establishes Time-Quasicrystals as a bridge between topological phases, time crystals, and quantum simulation, opening pathways to dissipativeprotected quantum memory and novel non-equilibrium quantum phenomena.
Periodically driven quantum many-body systems can spontaneously reorganize their motion and start moving with a period different than the driving period. These are ``discrete time crystals'' and they have been realized already in the laboratory. It turns out that systems from the same class can spontaneously reveal quasicrystalline structures in time. The interaction between the particles forces them into a quasicrystal pattern in the time domain, in spite of the fact that the driving is periodic.