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arXiv:2403.17838

Universal entropy transport far from equilibrium across the BCS-BEC crossover

Jeffrey Mohan, Philipp Fabritius, Mohsen Talebi, Simon Wili, Meng-Zi Huang, Tilman Esslinger

Published Mar 26, 2024• 0 citations
arXivHTMLPDF

Abstract

The transport properties of strongly interacting fermionic systems can reveal exotic states of matter, but experiments and theory have predominantly focused on bulk systems in the hydrodynamic limit describable with linear response coefficients such as electrical and thermal conductivity. In a ballistic channel connecting two superfluid reservoirs, recent experiments revealed a far-from-equilibrium regime beyond linear hydrodynamics where particle and entropy currents respond nonlinearly to biases of chemical potential and temperature, and their ratio is robust to the channel geometry. However, the origin of this robustness and its relation to the strong interparticle interactions remain unknown. Here, we study the coupled transport of particles and entropy tuning the interaction across the Bardeen-Cooper-Schrieffer to Bose-Einstein condensate (BCS-BEC) crossover, the reservoir degeneracy across the superfluid phase transition, as well as the local potentials and confinement of the channel. Surprisingly, the entropy advectively transported per particle depends only on the interactions and reservoir degeneracy and not on the details of the channel, suggesting that this property has its origin in the universal equilibrium properties of the reservoirs. In contrast, the magnitudes of the advective and diffusive entropy currents vary significantly with the channel details. The advective current increases monotonically towards the BEC side, which can be largely explained by the estimated superfluid gap in the channel. The Wiedemann-Franz law that links the advective and diffusive currents in Fermi liquids is most egregiously violated at unitarity, suggesting a change in the nature of the excitations responsible for entropy diffusion near unitarity. These observations pose fundamental questions regarding transport phenomena in strongly interacting Fermi systems far from equilibrium.

DOI
10.48550/arxiv.2403.17838

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The transport properties of strongly interacting fermionic systems can reveal exotic states of matter, but experiments and theory have predominantly focused on bulk systems in the hydrodynamic limit describable with linear response coefficients such as electrical and thermal conductivity. In a ballistic channel connecting two superfluid reservoirs, recent experiments revealed a far-from-equilibrium regime beyond linear hydrodynamics where particle and entropy currents respond nonlinearly to biases of chemical potential and temperature, and their ratio is robust to the channel geometry. However, the origin of this robustness and its relation to the strong interparticle interactions remain unknown. Here, we study the coupled transport of particles and entropy tuning the interaction across the Bardeen-Cooper-Schrieffer to Bose-Einstein condensate (BCS-BEC) crossover, the reservoir degeneracy across the superfluid phase transition, as well as the local potentials and confinement of the channel. Surprisingly, the entropy advectively transported per particle depends only on the interactions and reservoir degeneracy and not on the details of the channel, suggesting that this property has its origin in the universal equilibrium properties of the reservoirs. In contrast, the magnitudes of the advective and diffusive entropy currents vary significantly with the channel details. The advective current increases monotonically towards the BEC side, which can be largely explained by the estimated superfluid gap in the channel. The Wiedemann-Franz law that links the advective and diffusive currents in Fermi liquids is most egregiously violated at unitarity, suggesting a change in the nature of the excitations responsible for entropy diffusion near unitarity. These observations pose fundamental questions regarding transport phenomena in strongly interacting Fermi systems far from equilibrium.
The nature of particle and entropy flow between two superfluids is often understood in terms of reversible flow carried by an entropy-free, macroscopic wavefunction. While this wavefunction is responsible for many intriguing properties of superfluids and superconductors, its interplay with excitations in non-equilibrium situations is less understood. Here we observe large concurrent flows of both particles and entropy through a ballistic channel connecting two strongly interacting fermionic superfluids. Both currents respond nonlinearly to chemical potential and temperature biases. We find that the entropy transported per particle is much larger than the prediction of superfluid hydrodynamics in the linear regime and largely independent of changes in the channel's geometry. By contrast, the timescales of advective and diffusive entropy transport vary significantly with the channel geometry. In our setting, superfluidity counterintuitively increases the speed of entropy transport. Moreover, we develop a phenomenological model describing the nonlinear dynamics within the framework of generalized gradient dynamics. Our approach for measuring entropy currents may help elucidate mechanisms of heat transfer in superfluids and superconducting devices.
Abstract We present a theoretical review of the recent progress in non-equilibrium BCS (Bardeen-Cooper-Schrieffer)-BEC (Bose-Einstein condensation) crossover physics. As a paradigmatic example, we consider a strongly interacting driven-dissipative two-component Fermi gas where the non-equilibrium steady state is tuned by adjusting the chemical potential difference between two reservoirs that are coupled with the system. As a powerful theoretical tool to deal with this system, we employ the Schwinger-Keldysh Green’s function technique. We systematically evaluate the superfluid transition, as well as the single-particle properties, in the non-equilibrium BCS-BEC crossover region, by adjusting the chemical potential difference between the reservoirs and the strength of an s-wave pairing interaction associated with a Feshbach resonance. In the weak-coupling BCS side, the chemical potential difference is shown to imprint a two-step structure on the particle momentum distribution, leading to an anomalous enhancement of pseudogap, as well as the emergence of exotic Fulde-Ferrell-Larkin-Ovchinnikov-type superfluid instability. Since various non-equilibrium situations have recently been realized in ultracold Fermi gases, the theoretical understanding of non-equilibrium BCS-BEC crossover physics would become increasingly important in this research field.
The Bardeen–Cooper–Schrieffer (BCS) to Bose–Einstein condensate (BEC) crossover problem is solved for stationary gray solitons via the Boguliubov–de Gennes equations at zero temperature. These crossover solitons exhibit a localized notch in the gap and a characteristic phase difference across the notch for all interaction strengths, from BEC to BCS regimes. However, they do not follow the well-known Josephson-like sinusoidal relationship between velocity and phase difference except in the far BEC limit: at unitarity, the velocity has a nearly linear dependence on phase difference over an extended range. For a fixed phase difference, the soliton is of nearly constant depth from the BEC limit to unitarity and then grows progressively shallower into the BCS limit, and on the BCS side, Friedel oscillations are apparent in both gap amplitude and phase. The crossover soliton appears fundamentally in the gap; we show, however, that the density closely follows the gap, and the soliton is therefore observable. We develop an approximate power-law relationship to express this fact: the density of gray crossover solitons varies as the square of the gap amplitude in the BEC limit and as a power of about 1.5 at unitarity.
We study the emergence of dissipation in an atomic Josephson junction between weakly coupled superfluid Fermi gases. We find that vortex-induced phase slippage is the dominant microscopic source of dissipation across the Bose-Einstein condensate-Bardeen-Cooper-Schrieffer crossover. We explore different dynamical regimes by tuning the bias chemical potential between the two superfluid reservoirs. For small excitations, we observe dissipation and phase coherence to coexist, with a resistive current followed by well-defined Josephson oscillations. We link the junction transport properties to the phase-slippage mechanism, finding that vortex nucleation is primarily responsible for the observed trends of conductance and critical current. For large excitations, we observe the irreversible loss of coherence between the two superfluids, and transport cannot be described only within an uncorrelated phase-slip picture. Our findings open new directions for investigating the interplay between dissipative and superfluid transport in strongly correlated Fermi systems, and general concepts in out-of-equilibrium quantum systems.
Abstract Second sound is an entropy wave which propagates in the superfluid component of a quantum liquid. Because it is an entropy wave, it probes the thermodynamic properties of the quantum liquid. Here, we study second sound propagation for a large range of interaction strengths within the crossover between a Bose-Einstein condensate (BEC) and the Bardeen-Cooper-Schrieffer (BCS) superfluid, extending previous work at unitarity. In particular, we investigate the strongly-interacting regime where currently theoretical predictions only exist in terms of an interpolation in the crossover. Working with a quantum gas of ultracold fermionic 6Li atoms with tunable interactions, we show that the second sound speed varies only slightly in the crossover regime. By varying the excitation procedure, we gain deeper insight on sound propagation. We compare our measurement results with classical-field simulations, which help with the interpretation of our experiments.
Second sound is an entropy wave which propagates in the superfluid component of a quantum liquid. Because it is an entropy wave, it probes the thermodynamic properties of the quantum liquid which are determined, e.g., by the interaction strength between the particles of the quantum liquid and their temperature. Here, we study second sound propagation for a large range of interaction strengths within the crossover between a Bose-Einstein condensate (BEC) and the Bardeen-Cooper-Schrieffer (BCS) superfluid. In particular, we investigate the strongly-interacting regime where currently theoretical predictions only exist in terms of an interpolation between the BEC, BCS and unitary regimes. Working with a quantum gas of ultracold fermionic 6^66Li atoms with tunable interactions, we show that the second sound speed varies only slightly in the crossover regime. We gain deeper insights into sound propagation and excitation of second sound by varying the excitation procedure which ranges from a sudden force pulse to a gentle heating pulse at the cloud center. These measurements are accompanied by classical-field simulations which help with the interpretation of the experimental data. Furthermore, we determine the spatial extension of the superfluid phase and estimate the superfluid density. In the future, this may be used to construct the so far unknown equation of state throughout the crossover.