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arXiv:2403.07188 · Physical Review A

Enhanced strong-interaction effect in synthetic spin-orbit coupling with mixed spin symmetry

Ayaka Usui, Abel Rojo-Francàs, James Schloss, Bruno Juliá-Díaz

Published Feb 4, 2025• 0 citations
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Abstract

Synthetic spin-orbit coupling in cold atoms couples the pseudospin and spatial degrees of freedom, and therefore, the inherent spin symmetry of the system plays an important role. In systems of two pseudospin degrees, two particles contain symmetric states and antisymmetric states, but the spin symmetry can be mixed for more particles. This mixed spin symmetry has been overlooked and has not been investigated thoroughly. We study the role of mixed spin symmetry in the presence of spin-orbit coupling and consider a system of three bosons with two hyperfine states trapped in a harmonic potential. We investigate the ground state and the energy spectrum by implementing exact diagonalization. Similar to that in two-particle systems, the interplay between spin-orbit coupling and repulsive interactions between antialigned pseudospins increases the population of the unaligned spin components in the ground state. Also, the emergence of mixed-spin symmetric states compensates for the rise of the interaction energy. In contrast to two-particle systems, the pair correlation of the ground state is analogous to the Tonks-Girardeau gas even for relatively small contact interactions, and this feature is enhanced by the spin-orbit coupling.

DOI
10.1103/physreva.111.023305

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Synthetic spin-orbit coupling in cold atoms couples the pseudospin and spatial degrees of freedom, and therefore, the inherent spin symmetry of the system plays an important role. In systems of two pseudospin degrees, two particles contain symmetric states and antisymmetric states, but the spin symmetry can be mixed for more particles. This mixed spin symmetry has been overlooked and has not been investigated thoroughly. We study the role of mixed spin symmetry in the presence of spin-orbit coupling and consider a system of three bosons with two hyperfine states trapped in a harmonic potential. We investigate the ground state and the energy spectrum by implementing exact diagonalization. Similar to that in two-particle systems, the interplay between spin-orbit coupling and repulsive interactions between antialigned pseudospins increases the population of the unaligned spin components in the ground state. Also, the emergence of mixed-spin symmetric states compensates for the rise of the interaction energy. In contrast to two-particle systems, the pair correlation of the ground state is analogous to the Tonks-Girardeau gas even for relatively small contact interactions, and this feature is enhanced by the spin-orbit coupling.
The coupling between the spin degrees of freedom and the orbital angular momentum has a profound effect on the properties of nuclei, atoms, and condensed-matter systems. Recently, synthetic gauge fields have been realized experimentally in neutral cold-atom systems, giving rise to a spin-orbit coupling term with ``strength'' kso{k}_{\text{so}}kso​. This paper investigates the interplay between the single-particle spin-orbit coupling term of Rashba type and the short-range two-body sss-wave interaction for cold atoms under external confinement. Specifically, we consider two different harmonically trapped two-atom systems. The first system consists of an atom with spin-orbit coupling that interacts with a structureless particle through a short-range two-body potential. The second system consists of two atoms that both feel the spin-orbit coupling term and that interact through a short-range two-body potential. Treating the spin-orbit term perturbatively, we determine the correction to the ground-state energy for various generic parameter combinations. Selected excited states are also treated. An important aspect of our study is that the perturbative treatment is not limited to small sss-wave scattering lengths but provides insights into the system behavior over a wide range of scattering lengths, including the strongly interacting unitary regime. We find that the interplay between the spin-orbit coupling term and the sss-wave interaction generically enters, depending on the exact parameter combinations of the sss-wave scattering lengths, at order kso2{k}_{\text{so}}^{2}kso2​ or kso4{k}_{\text{so}}^{4}kso4​ for the ground state and leads to a shift of the energy of either sign. While the absence of a term proportional to kso{k}_{\text{so}}kso​ follows straightforwardly from the functional form of the spin-orbit coupling term, the absence of a term proportional to kso2{k}_{\text{so}}^{2}kso2​ for certain parameter combinations is unexpected. The well-known fact that the spin-orbit coupling term couples the relative and center-of-mass degrees of freedom has interesting consequences for the trapped two-particle systems. For example, we find that, for certain parameter combinations, the spin-orbit coupling term turns sharp crossings into avoided crossings with an energy splitting proportional to kso{k}_{\text{so}}kso​. Our perturbative results are confirmed by numerical calculations that expand the eigenfunctions of the two-particle Hamiltonian in terms of basis functions that contain explicitly correlated Gaussians.
Abstract We explore the influence of contact interactions on a synthetically spin–orbit coupled system of two ultracold trapped atoms. Even though the system we consider is bosonic, we show that a regime exists in which the competition between the contact and spin–orbit interactions results in the emergence of a ground state that contains a significant contribution from the anti-symmetric spin state. This ground state is unique to few-particle systems and does not exist in the mean-field regime. The transition to this state is signalled by an inversion in the average momentum from being dominated by centre-of-mass momentum to relative momentum and also affects the global entanglement shared between the real- and pseudo-spin spaces. Indeed, competition between the interactions can also result in avoided crossings in the ground state which further enhances these correlations. However, we find that correlations shared between the pseudo-spin states are strongly depressed due to the spin–orbit coupling and therefore the system does not contain spin–spin entanglement.
The dissertation explores the effects of synthetic spin-orbit coupling on the behaviour of quantum gases in several different contexts. We first study realistic methods to create vortices in spin-orbit-coupled (SOC) Bose-Einstein condensates (BEC). We propose two different methods to induce thermodynamically stable static vortex configurations: (1) to rotate both the Raman lasers and the anisotropic trap; and (2) to impose a synthetic Abelian field on top of synthetic spin-orbit interactions. We solve the Gross-Pitaevskii equation for several experimentally relevant regimes and find new interesting effects such as spatial separation of left- and right-moving spin-orbit-coupled condensates, and the appearance of unusual vortex arrangements. Next we consider cold atoms in an optical lattice with synthetic SOC in the Mott-insulator regime. We calculate the parameters of the corresponding tight-binding model and derive the low-energy spin Hamiltonian which is a combination of Heisenberg model, quantum compass model and Dzyaloshinskii-Moriya interaction. We find that the Hamiltonian supports a rich classical phase diagram with collinear, spiral and vortex phases. Next we study the time evolution of the magnetization in a Rashba spin-orbit-coupled Fermi gas, starting from a fully-polarized initial state. We model the dynamics using a Boltzmann equation, which we solve in the Hartree-Fock approximation. The resulting non-linear system of equations gives rise to three distinct dynamical regimes controlled by the ratio of interaction and spin-orbit-coupling strength λ: for small λ, the magnetization decays to zero. For intermediate λ, it displays undamped oscillations about zero and for large λ, a partially magnetized state is dynamically stabilized. Motivated by an interesting stripe phase which appears in BEC with SOC [Li et al., Phys. Rev. Lett. 108, 225301 (2011)], we study the finite-temperature phase diagram of a pseudospin-1/2 Bose gas with contact interactions. We show that strong inter-spin interactions can lead to the appearance of magnetically ordered phases at temperatures above the superfluid transition. For the case of inter-spin attraction, we also discuss the possibility of a bosonic analogue of the Cooper-paired phase, however this state is not energetically favourable. We extend our calculations to a spin-orbit-coupled Bose gas to investigate the possibility of stripe ordering in the normal phase. However, within our approximations, we do not find an instability towards stripe formation. Finally, we consider a two-dimensional Bose gas at zero temperature with an underlying quartic single-particle dispersion in one spatial direction. This Hamiltonian can be realized using the NIST scheme of spin-orbit coupling [Y.-J. Lin, K. Jimenez-Garcia, and I. B. Spielman, Nature 471, 83 (2011)], or using the shaken lattice scheme of Parker et al. [C. V. Parker, L.-C. Ha and C. Chin, Nature Physics 9, 769 (2013)]. By numerically comparing energies of various trial wave-functions, we show that, at low densities, the ground state is strongly correlated, in contrast to a typical mean-field BEC. The trial wave-function with the lowest energy is of Jastrow-type and it describes a state with finite, but strongly reduced, condensate fraction.
This dissertation contains a collection of topics on the spin-orbit coupling of cold atoms and semiconductors. We first consider the effects of an optically induced spin-orbit interaction on a system of Bosonic atoms. The spin-orbit term couples the emergent pseudo-spin- 1/2 degree of freedom to momentum. The single particle energy spectrum has a low energy band with two minima at non-zero momentum. At low temperatures, a many-body system will condense into these minima. In the presence of vanishing interactions, the ground state wavefunction is found to be N00N state of "left" and "right"-moving state. An experimentally observable signature of the condensate is predicted that can be observed using time-of-flight imaging. We then predict a bulk manifestation of the spin-Hall effect in an inhomoge- neous spin-orbit-coupled system. The phenomena is predicted in the framework of the spin diffusion equations generalized to include arbitrary Rashba and linear and cubic Dresselhaus terms. This framework shows that a bulk spin-density wave with a wavevector oriented perpendicular to an applied electric field will induce a charge- density wave characterized by a π/2-phase shift and a non-monotonic time-varying amplitude. The optimal values of spin-orbit coupling for observation of the effect are determined. We propose a scheme for using atom interferometry to measure weak time- dependent accelerations. This proposal uses an ensemble of dilute trapped bosons with two pseudo-spin states coupled to a synthetic magnetic field, but with opposite effective charges. The synthetic field acts to couple spin to momentum continuously, which continuously imparts the acceleration on the phase of the internal states. We use time reversal pulses to reduce noise. The sensitivity of such a system is estimated to be S ∼ 10−7 m/s^2/√Hz Finally, we consider the semiclassical dynamics of a trapped spin-orbit coupled system. We find non-linear dynamics parameterized by the value of the initial displacement of the trap, and the anisotropy of the spin-orbit energy spectrum. We show that the dynamics can give a Berry's phase, and propose an experiment to measure this phase. We then propose a generalization of the 4-level scheme that allows for spin-orbit coupling described by a vector potential that is proportional to the angular momentum operator.
We present a variational study of pseudo-spin-1/21/21/2 Bose gases in a harmonic trap with weak three-dimensional (3D) spin-orbit coupling of $\mathbf{\ensuremath{\sigma}}\ifmmode\cdot\else\textperiodcentered\fi{}\mathbf{p}$ type. This spin-orbit coupling mixes states with different parities, which inspires us to approximate the single-particle state with the eigenstates of the total angular momentum, i.e., superposition of harmonic sss-wave and ppp-wave states. As the time-reversal symmetry is protected by two-body interaction, we set the variational order parameter as the combination of two mutually time-reversal symmetric eigenstates of the total angular momentum. The variational results essentially reproduce the 3D skyrmionlike ground state recently identified by Kawakami et al. [T. Kawakami, T. Mizushima, M. Nitta, and K. Machida, Phys. Rev. Lett. 109, 015301 (2012)]. We show that these skyrmionlike ground states emerging in this model are primarily caused by the ppp-wave spatial mode involved in the variational order parameter that drives two spin components spatially separated. We find the ground state of this system falls into two phases with different density distribution symmetries depending on the relative magnitude of intraspecies and interspecies interaction: phase I has parity symmetric and axisymmetric density distributions, while phase II is featured with special joint symmetries of discrete rotational and time-reversal symmetry. With the increasing interaction strength the transition occurs between two phases with distinct density distributions, while the topological 3D skyrmionlike spin texture is symmetry protected.
This review focuses on recent developments in synthetic spin-orbit (SO) coupling in ultracold atomic gases. Two types of SO coupling are discussed. One is Raman process induced coupling between spin and motion along one of the spatial directions and the other is Rashba SO coupling. We emphasize their common features in both single-particle and two-body physics and the consequences of both in many-body physics. For instance, single particle ground state degeneracy leads to novel features of superfluidity and a richer phase diagram; increased low-energy density-of-state enhances interaction effects; the absence of Galilean invariance and spin-momentum locking gives rise to intriguing behaviours of superfluid critical velocity and novel quantum dynamics; and the mixing of two-body singlet and triplet states yields a novel fermion pairing structure and topological superfluids. With these examples, we show that investigating SO coupling in cold atom systems can, enrich our understanding of basic phenomena such as superfluidity, provide a good platform for simulating condensed matter states such as topological superfluids and more importantly, result in novel quantum systems such as SO coupled unitary Fermi gas and high spin quantum gases. Finally we also point out major challenges and some possible future directions.