Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2403.04611 · npj Quantum Information

Cavity-assisted resonance fluorescence from a nitrogen-vacancy center in diamond

Viktoria Yurgens, Yannik Fontana, Andrea Corazza, Brendan Shields, Patrick Maletinsky, Richard John Warburton

Published Nov 7, 2024• 24 citations
arXivHTMLPDF

Abstract

The nitrogen-vacancy center in diamond is an attractive resource for the generation of remote entangled states owing to its optically addressable and long-lived electronic spin. However, its low native fraction of coherent photon emission, ~3%, undermines the achievable spin-photon entanglement rates. Here, we couple a nitrogen-vacancy center with a narrow extrinsically-broadened linewidth (159 MHz), hosted in a micron-thin membrane, to an open microcavity. The resulting Purcell factor of ~1.8 increases the zero-phonon line fraction to over 44%. Operation in the Purcell regime, together with an efficient collection of the zero-phonon-line photons, allows resonance fluorescence to be detected for the first time without any temporal filtering. We achieve a >10 signal-to-laser background ratio. This selective enhancement of the center's zero-phonon transitions could increase spin-spin entanglement success probabilities beyond an order of magnitude compared to state-of-the-art implementations, and enable powerful quantum optics techniques such as wave-packet shaping or all-optical spin manipulation.

DOI
10.1038/s41534-024-00915-9

Related papers

Enhanced zero phonon line emission from a nitrogen-vacancy centre in diamond coupled to an optical microcavity

Sam Johnson, Philip R. Dolan, Aurelien A. P. Trichet +1 more

The realisation of an efficient spin-photon interface using the negatively charged nitrogen-vacancy centre (NV-) in diamond requires the resonant coupling of the zero phonon line (ZPL) of the centre to an optical microcavity [1]. The cavity serves to encourage emission into the ZPL in preference to the phonon sidebands, and potentially also to increase the homogeneous linewidth via a reduction of the lifetime (the Purcell effect) thus assisting in the generation of indistinguishable photons. Cavity coupling thus has potential to improve by orders of magnitude the speed with which entanglement can be created between spatially remote NV- centres [2], and to enable other mechanisms for realising spin-photon interfaces via non-demolition measurements [3].

European Quantum Electronics Conference (EQEC)•Jun 21, 2015•0 citations

Tunable open-cavity coupling to the zero phonon line of a nitrogen-vacancy defect in diamond (Conference Presentation)

Sam Johnson, Laiyi Weng, Philip R. Dolan +10 more

Recent demonstrations of entanglement between two remote Nitrogen-Vacancy centers, have opened the way for their use in distributed quantum networks. An efficient spin-photon interface will now be required to help realize this system as a technology. Here we demonstrate the tunable enhancement of the zero phonon line of a single nitrogen-vacancy colour centre in nanodiamond at cryogenic temperatures. A plano-hemispherical open cavity, fabricated using focused ion beam milling provides mode volumes as small as 1.25 cubic microns and quality factor Q ~ 3000. It will be shown how the open geometry and independently adjustable mirrors allows for precise placement of the emitter in the centre of the cavity mode, and crucially enables in-situ tuning of the cavity resonances. At optimal coupling, the signal from individual zero phonon line transitions is enhanced by a factor of 6.25 through the Purcell effect and the overall emission rate of the NV- centre is increased by 40% compared with that measured from the same centre in the absence of cavity field confinement. This Purcell enhancement is mapped out as a function of cavity mode volume. These results represent a proof of principle for a tunable cryogenic spin-photon interface. However by far the best NV optical and spin coherences are to be found in bulk material and efforts towards the production of diamond membranes are currently being made, with dimensions suitable for open-cavity coupling. Efforts towards this and preliminary results will also be discussed.

•Apr 28, 2017•0 citations

Resonance fluorescence from a diamond nitrogen-vacancy center in a cavity

Yannik Fontana, Viktoria Yurgens, Andrea Corazza +3 more

Efficiently coupling a narrow-linewidth nitrogen-vacancy center (NV) in diamond to an open optical microcavity, we observe for the first time NV resonance fluorescence without requiring any time-filtering, marking a breakthrough toward high-efficiency spin-photon entanglement sources.

Quantum 2.0 Conference and Exhibition•Jan 1, 2024•0 citations

Deterministic enhancement of coherent photon generation from a nitrogen-vacancy center in ultrapure diamond (Conference Presentation)

Daniel Riedel, Immo Söllner, Brendan Shields +5 more

A key requirement for many applications in solid-state quantum sciences is a high fluence of indistinguishable photons. The spontaneous emission of these photons is governed by the coupling of an excited quantum system to electromagnetic vacuum fluctuations. In our experiment, we enhance this coupling by engineering a tunable Fabry-Perot microcavity. The quantum system we study is the nitrogen-vacancy (NV) center in diamond, a workhorse for quantum science and engineering, due to its optical transitions and the coherent electron spin system it hosts. Our device consists of a high-quality, nano-fabricated, single-crystalline diamond membrane bonded to a planar mirror; the cavity is completed by a second, concave mirror. Using piezo positioners, we achieve full spectral and spatial tunability and freedom in selecting NVs with favorable emission properties in our low-temperature (4 Kelvin) experiments. Upon tuning of the cavity into resonance, we find significant enhancement of the 637 nm zero phonon line for several individual NVs which is accompanied by a strong reduction of the overall photoluminescence (PL) lifetime. We infer a 30-fold enhancement of the zero-phonon transition rate at best. The fraction of the PL emission associated to this resonant transition is thereby increased from 3% to 46%. Our results constitute a significant leap on the route towards the implementation of fast long-distance quantum networks, which are currently limited by the photon emission rate in their nodes. Furthermore, our versatile design is readily applicable to other solid-state quantum emitters like color centers in silicon carbide.

Quantum Photonic Devices•Sep 19, 2017•4 citations

Superfluorescence and Collective Purcell-Enhancement of Nitrogen Vacancy Centers in diamond membranes

Maximilian Pallmann, Kerim Köster, Julia Heupel +2 more

We observe cavity-enhanced ensemble fluorescence of nitrogen-vacancy centers in diamond, showing Purcell-enhancement of the Zero Phonon Line (ZPL). The emission features temporal bunching of ZPL photons, indicating collective emission that can be attributed to superfluorescence.

Frontiers in Optics•Jan 1, 2022•0 citations

Engineering of the photonic environment of single nitrogen-vacancy centers in diamond

Daniel Riedel

The nitrogen-vacancy (NV) center in diamond has an optically addressable, highly coherent spin. However, an NV center even in high quality single-crystalline material is a very poor source of single photons: extraction out of the high-index diamond is inefficient, the emission of coherent photons represents just a few per cent of the total emission, and the decay time is large. In principle, all three problems can be addressed with a resonant microcavity, which significantly boosts the emission rate of coherent photons into the cavity mode based on the Purcell effect. In practice though, it has proved difficult to implement this concept: photonic engineering hinges on nano-fabrication yet it is notoriously difficult to process diamond without degrading the NV centers. \nIn this thesis, we present a microcavity scheme which employs minimally processed diamond membranes, thereby preserving the high quality of the starting material. The miniaturized plano-concave Fabry-Perot microcavity platform features full in situ spatial and spectral tunability. We demonstrate a clear change in the lifetime for multiple individual NV centers on tuning both the cavity frequency and anti-node position. The overall Purcell factor for the zero-phonon line (ZPL) of ~30 translates to an increase in the ZPL emission probability from ~3% to ~46%. \nFurthermore, we report the creation of a low-loss, broadband optical antenna giving highly directed output from a coherent single spin in the solid state. The device, the first crystalline solid-state realization of a dielectric antenna, is engineered for individual NV electronic spins in diamond. The photonic structure preserves the high spin coherence of single-crystalline diamond (T2 ~100µs). We demonstrate a directionality of close to 10 and single photon count rates approaching one MHz. The analysis of the angular emission pattern of our device suggests that 95% of the broadband NV fluorescence is channeled into a solid angle corresponding to a numerical aperture of 0.8. \nThe abovementioned approaches feature complementary benefits. The narrowband enhancement of the ZPL emission rate provided by the microcavity benefits applications in quantum information processing relying on coherent photons. With the prospect of integrating lifetime-limited emitters and achieving a high ZPL collection efficiency our results pave the way for much enhanced spin-photon and spin-spin entanglement rates. On the other hand, by channeling the major fraction of the broadband NV fluorescence into a narrow solid angle the dielectric optical antenna facilitates efficient spin readout. Our approach enables a near-unity collection efficiency which, upon mitigation of the known photon losses, renders it a potential key technology for quantum sensing applications. \n

•Jan 1, 2017•2 citations
The nitrogen-vacancy center in diamond is an attractive resource for the generation of remote entangled states owing to its optically addressable and long-lived electronic spin. However, its low native fraction of coherent photon emission, ~3%, undermines the achievable spin-photon entanglement rates. Here, we couple a nitrogen-vacancy center with a narrow extrinsically-broadened linewidth (159 MHz), hosted in a micron-thin membrane, to an open microcavity. The resulting Purcell factor of ~1.8 increases the zero-phonon line fraction to over 44%. Operation in the Purcell regime, together with an efficient collection of the zero-phonon-line photons, allows resonance fluorescence to be detected for the first time without any temporal filtering. We achieve a >10 signal-to-laser background ratio. This selective enhancement of the center's zero-phonon transitions could increase spin-spin entanglement success probabilities beyond an order of magnitude compared to state-of-the-art implementations, and enable powerful quantum optics techniques such as wave-packet shaping or all-optical spin manipulation.
The realisation of an efficient spin-photon interface using the negatively charged nitrogen-vacancy centre (NV-) in diamond requires the resonant coupling of the zero phonon line (ZPL) of the centre to an optical microcavity [1]. The cavity serves to encourage emission into the ZPL in preference to the phonon sidebands, and potentially also to increase the homogeneous linewidth via a reduction of the lifetime (the Purcell effect) thus assisting in the generation of indistinguishable photons. Cavity coupling thus has potential to improve by orders of magnitude the speed with which entanglement can be created between spatially remote NV- centres [2], and to enable other mechanisms for realising spin-photon interfaces via non-demolition measurements [3].
Recent demonstrations of entanglement between two remote Nitrogen-Vacancy centers, have opened the way for their use in distributed quantum networks. An efficient spin-photon interface will now be required to help realize this system as a technology. Here we demonstrate the tunable enhancement of the zero phonon line of a single nitrogen-vacancy colour centre in nanodiamond at cryogenic temperatures. A plano-hemispherical open cavity, fabricated using focused ion beam milling provides mode volumes as small as 1.25 cubic microns and quality factor Q ~ 3000. It will be shown how the open geometry and independently adjustable mirrors allows for precise placement of the emitter in the centre of the cavity mode, and crucially enables in-situ tuning of the cavity resonances. At optimal coupling, the signal from individual zero phonon line transitions is enhanced by a factor of 6.25 through the Purcell effect and the overall emission rate of the NV- centre is increased by 40% compared with that measured from the same centre in the absence of cavity field confinement. This Purcell enhancement is mapped out as a function of cavity mode volume. These results represent a proof of principle for a tunable cryogenic spin-photon interface. However by far the best NV optical and spin coherences are to be found in bulk material and efforts towards the production of diamond membranes are currently being made, with dimensions suitable for open-cavity coupling. Efforts towards this and preliminary results will also be discussed.
A key requirement for many applications in solid-state quantum sciences is a high fluence of indistinguishable photons. The spontaneous emission of these photons is governed by the coupling of an excited quantum system to electromagnetic vacuum fluctuations. In our experiment, we enhance this coupling by engineering a tunable Fabry-Perot microcavity. The quantum system we study is the nitrogen-vacancy (NV) center in diamond, a workhorse for quantum science and engineering, due to its optical transitions and the coherent electron spin system it hosts. Our device consists of a high-quality, nano-fabricated, single-crystalline diamond membrane bonded to a planar mirror; the cavity is completed by a second, concave mirror. Using piezo positioners, we achieve full spectral and spatial tunability and freedom in selecting NVs with favorable emission properties in our low-temperature (4 Kelvin) experiments. Upon tuning of the cavity into resonance, we find significant enhancement of the 637 nm zero phonon line for several individual NVs which is accompanied by a strong reduction of the overall photoluminescence (PL) lifetime. We infer a 30-fold enhancement of the zero-phonon transition rate at best. The fraction of the PL emission associated to this resonant transition is thereby increased from 3% to 46%. Our results constitute a significant leap on the route towards the implementation of fast long-distance quantum networks, which are currently limited by the photon emission rate in their nodes. Furthermore, our versatile design is readily applicable to other solid-state quantum emitters like color centers in silicon carbide.
The nitrogen-vacancy (NV) center in diamond has an optically addressable, highly coherent spin. However, an NV center even in high quality single-crystalline material is a very poor source of single photons: extraction out of the high-index diamond is inefficient, the emission of coherent photons represents just a few per cent of the total emission, and the decay time is large. In principle, all three problems can be addressed with a resonant microcavity, which significantly boosts the emission rate of coherent photons into the cavity mode based on the Purcell effect. In practice though, it has proved difficult to implement this concept: photonic engineering hinges on nano-fabrication yet it is notoriously difficult to process diamond without degrading the NV centers. \nIn this thesis, we present a microcavity scheme which employs minimally processed diamond membranes, thereby preserving the high quality of the starting material. The miniaturized plano-concave Fabry-Perot microcavity platform features full in situ spatial and spectral tunability. We demonstrate a clear change in the lifetime for multiple individual NV centers on tuning both the cavity frequency and anti-node position. The overall Purcell factor for the zero-phonon line (ZPL) of ~30 translates to an increase in the ZPL emission probability from ~3% to ~46%. \nFurthermore, we report the creation of a low-loss, broadband optical antenna giving highly directed output from a coherent single spin in the solid state. The device, the first crystalline solid-state realization of a dielectric antenna, is engineered for individual NV electronic spins in diamond. The photonic structure preserves the high spin coherence of single-crystalline diamond (T2 ~100µs). We demonstrate a directionality of close to 10 and single photon count rates approaching one MHz. The analysis of the angular emission pattern of our device suggests that 95% of the broadband NV fluorescence is channeled into a solid angle corresponding to a numerical aperture of 0.8. \nThe abovementioned approaches feature complementary benefits. The narrowband enhancement of the ZPL emission rate provided by the microcavity benefits applications in quantum information processing relying on coherent photons. With the prospect of integrating lifetime-limited emitters and achieving a high ZPL collection efficiency our results pave the way for much enhanced spin-photon and spin-spin entanglement rates. On the other hand, by channeling the major fraction of the broadband NV fluorescence into a narrow solid angle the dielectric optical antenna facilitates efficient spin readout. Our approach enables a near-unity collection efficiency which, upon mitigation of the known photon losses, renders it a potential key technology for quantum sensing applications. \n