Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness 1.52⋅10 6 pairssmWGHz and large bandwidth (7.8 THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of Δ τ ≈ 120 fs while maintaining the narrow bandwidth Δ ω p ≪ 1 MHz of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.
Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness 1.52⋅10 6 pairssmWGHz and large bandwidth (7.8 THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of Δ τ ≈ 120 fs while maintaining the narrow bandwidth Δ ω p ≪ 1 MHz of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.
Abstract Broadband photon pairs are highly desirable for quantum metrology, quantum sensing, and quantum communication. Such sources are usually designed through type-0 phase-matching spontaneous parametric down-conversion (SPDC) that makes the photon pairs hard to separate in the frequency-degenerate case and thus limits their applications. In this paper, we design a broadband frequency-degenerate telecom-band photon pair source via the type-II SPDC in a dispersion-engineered thin-film lithium niobate waveguide, where the polarization modes of photon pairs are orthogonal and thus are easily separated deterministically. With a 5-mm-long waveguide, our design can achieve a bandwidth of 5.56 THz (44.8 nm), which is 8.6 times larger than that of the bulk lithium niobate, and the central wavelength can be flexibly adjusted. Our design is a promising approach towards high-quality integrated photon sources and may have wide applications in photonic quantum technologies.
Photon pairs from spontaneous parametric down-conversion (SPDC) are important for a wide range of quantum optics experiments with spectral properties such as their bandwidths often being a crucial concern. Here we show the generic existence of particular phase-matching conditions in quasi-phase-matched KTP, MgO:LN, and SLT crystals that lead to ultra-broadband, widely nondegenerate photon pairs. It is based on the existence of group-velocity-matched, far apart wavelength pairs and, for 2 mm long crystals, results in SPDC bandwidths between 15 and 25 THz for photon pairs with the idler photon in the technologically relevant mid-IR range of 3-5 μm and the signal photon in the near-IR below 1100 nm. We experimentally demonstrate this type of broadband phase matching in ppKTP crystals for photon pairs centered at 800 and 3800 nm and measure a bandwidth of 15 THz. This novel method of generating broadband photon pairs will be highly beneficial for SPDC-based imaging, spectroscopy, refractometry, and optical coherence tomography with undetected mid-IR photons.
We demonstrate a broadband entangled photon source based on a single-pass, type-0 phase-matched, non-collinear spontaneous parametric down-conversion (SPDC) process. By spatially multiplexing the intrinsically random transverse momentum states of biphotons emitted in an annular spatial distribution from a single-frequency-pumped, 2-mm-long periodically poled KTP crystal, we generate polarization-entangled pair photons with a spectral bandwidth of ∼130 nm centered at 810 nm. The negligible group-velocity mismatch of the co-polarized near-degenerate photons in single-pass and low birefringence of standard optical components preserves indistinguishability across the broadband emission without phase compensation, enabling high-quality polarization entanglement over the entire emission bandwidth. The source achieves a brightness of 0.57 Mpairs/s/mW and a two-photon coherence length of 6.97 μm, while exhibiting an interference visibility exceeding 95%, a Bell–CHSH parameter of 2.526 ± 0.005 that remains stable over 12 h of continuous operation and violates the Bell inequality by more than 100 standard deviations, and a state fidelity of 96.3%. The generic scheme providing the broadest bandwidth entangled biphotons at 810 nm, to our knowledge, can readily be used for other wavelengths as required for multiparty quantum networks and quantum sensing applications.
Quantum networks based on wavelength-multiplexed entanglement enable parallel distribution of quantum correlations, increasing channel capacity for secure communication and distributed quantum information processing. However, broadband integrated sources capable of generating multipartite entanglement beyond photon pairs remain scarce. Here we report on-chip generation of telecom-band four-photon entanglement in a periodically poled thin-film lithium niobate on insulator (LNOI) waveguide. Type-0 spontaneous parametric down-conversion provides a phase-matching bandwidth exceeding 200 nm, enabling spectrally separable generation of multi-photon entanglement across the telecom band. The generated photons are encoded in time bins for robust fiber compatibility, and a coherent interface enabling reversible conversion between time-bin and polarization degrees of freedom allows complete quantum state tomography. We measure two-photon entanglement with a brightness of 6.7 MHz/mW/nm and a fidelity of 0.874±0.002. At a pump power of 0.08 mW, the four-photon state exhibits a fourfold coincidence rate of 1 Hz and a fidelity of 0.74±0.01, representing a threefold improvement over previous integrated platforms. Our results establish LNOI as a scalable platform for broadband multi-photon entanglement and provide a practical route toward dense wavelength-multiplexed quantum networks.
Broadband nonlinear optical devices play a critical role in both classical and quantum optics. Here, we design and fabricate a 6.82-mm-long step-chirped periodically poled lithium niobate (CPPLN) waveguide on lithium niobate on insulator, which enables quasi-phase matching over a broad bandwidth for second-harmonic generation (SHG) and spontaneous parametric down-conversion (SPDC). The SHG achieves an average efficiency of 91%/W/cm 2 over the first-harmonic wavelength range of 1510 nm–1620 nm, paving the way for realizing SPDC across a wide range of pump wavelengths. For SPDC, by tuning the pump wavelength to 775 nm, 780 nm, and 785 nm, we achieve broadband photon-pair generation with a maximum full bandwidth and brightness up to 99 THz (846 nm) and 21 MHz/mW/nm, respectively. Our findings provide an efficient and experiment-friendly approach for generating broadband photon pairs, which holds significant promise for advancing applications in quantum metrology.
We demonstrate a broadband entangled photon source based on a single-pass, type-0 phase-matched, non-collinear spontaneous parametric down-conversion (SPDC) process. By spatially multiplexing the intrinsically random transverse momentum states of biphotons emitted in an annular spatial distribution from a single-frequency-pumped, 2-mm-long periodically poled KTP crystal, we generate polarization-entangled pair photons with a spectral bandwidth of ∼130 nm centered at 810 nm. The negligible group-velocity mismatch of the co-polarized near-degenerate photons in single-pass and low birefringence of standard optical components preserves indistinguishability across the broadband emission without phase compensation, enabling high-quality polarization entanglement over the entire emission bandwidth. The source achieves a brightness of 0.57 Mpairs/s/mW and a two-photon coherence length of 6.97 μm, while exhibiting an interference visibility exceeding 95%, a Bell–CHSH parameter of 2.526 ± 0.005 that remains stable over 12 h of continuous operation and violates the Bell inequality by more than 100 standard deviations, and a state fidelity of 96.3%. The generic scheme providing the broadest bandwidth entangled biphotons at 810 nm, to our knowledge, can readily be used for other wavelengths as required for multiparty quantum networks and quantum sensing applications.