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arXiv:2402.16657 · Europhysics Letters (EPL)

Ultracold atomic spin mixtures in ultrastable magnetic field environments

Riccardo Cominotti, Chiara Rogora, Alessandro Zenesini, Giacomo Lamporesi, Gabriele Ferrari

Published May 1, 2024• 6 citations
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Abstract

Abstract Ultracold atomic spin mixtures develop rich and intriguing magnetic properties when external radiation coherently couples different spin states. In particular, the coupled mixture may acquire a critical behavior when the spin interactions equal the coupling energy. However, atomic mixtures generally feature a relatively high sensitivity to magnetic fields that can set a limitation to the observable phenomena. In this article, we present an overview of experimental studies of magnetism based on superfluid multicomponent gases in an ultrastable magnetic field environment, which recently became available.

DOI
10.1209/0295-5075/ad4b9a

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Abstract Ultracold atomic spin mixtures develop rich and intriguing magnetic properties when external radiation coherently couples different spin states. In particular, the coupled mixture may acquire a critical behavior when the spin interactions equal the coupling energy. However, atomic mixtures generally feature a relatively high sensitivity to magnetic fields that can set a limitation to the observable phenomena. In this article, we present an overview of experimental studies of magnetism based on superfluid multicomponent gases in an ultrastable magnetic field environment, which recently became available.
The high degree of control on ultracold gases allows us to precisely manipulate their internal state. When the gas is made of atoms in two different internal states, it can be considered as a two-component spin mixture. Below a critical temperature, the gas becomes a superfluid mixture, never realized before with any other platform, and therefore interesting to study per se, but it also constitutes a promising and versatile platform for applications in spintronic devices or to study phenomena belonging to very different fields, such as magnetism, high-energy physics or gravitation. Here, I will revisit ground-state properties and excitations of a binary bosonic superfluid, and then introduce a coherent coupling between the states and treat the global state of the atoms as a spin in the presence of a variable external field.
This article summarizes some of the relevant features exhibited by binary mixtures of Bose–Einstein condensates in the presence of coherent coupling at zero temperature. The coupling, which is experimentally produced by proper photon transitions, can involve either negligible momentum transfer from the electromagnetic radiation (Rabi coupling) or large momentum transfer (Raman coupling) associated with spin–orbit effects. The nature of the quantum phases exhibited by coherently coupled mixtures is discussed in detail, including their paramagnetic, ferromagnetic, and, in the case of spin–orbit coupling, supersolid phases. The behavior of the corresponding elementary excitations is discussed, with explicit emphasis on the novel features caused by the spin-like degree of freedom. Focus is further given to the topological excitations (solitons, vortices) as well as to the superfluid properties. This review also points out relevant open questions that deserve more systematic theoretical and experimental investigations.
The paper gives an overview of the recent developments in the field of ultracold fermionic quantum gases. In particular, results obtained on an ultracold spin-mixture of /sup 6/Li atoms in a series of experiments performed in Innsbruck is presented . Bose-Einstein condensation of strongly bound atom pairs (molecules) , the reversible crossover to a degenerate Fermi gas, measurements of collective excitation modes, and spectroscopic observation of pairing in a strongly interacting Fermi gas of atoms are also discussed. The experimental results provide strong evidence for superfluidity.
Since the achievement of quantum degeneracy in gases of chromium atoms in 2004, the experimental investigation of ultracold gases made of highly magnetic atoms has blossomed. The field has yielded the observation of many unprecedented phenomena, in particular those in which long-range and anisotropic dipole-dipole interactions (DDIs) play a crucial role. In this review, we aim to present the aspects of the magnetic quantum-gas platform that make it unique for exploring ultracold and quantum physics as well as to give a thorough overview of experimental achievements. Highly magnetic atoms distinguish themselves by the fact that their electronic ground-state configuration possesses a large electronic total angular momentum. This results in a large magnetic moment and a rich electronic transition spectrum. Such transitions are useful for cooling, trapping, and manipulating these atoms. The complex atomic structure and large dipolar moments of these atoms also lead to a dense spectrum of resonances in their two-body scattering behaviour. These resonances can be used to control the interatomic interactions and, in particular, the relative importance of contact over dipolar interactions. These features provide exquisite control knobs for exploring the few- and many-body physics of dipolar quantum gases. The study of dipolar effects in magnetic quantum gases has covered various few-body phenomena that are based on elastic and inelastic anisotropic scattering. Various many-body effects have also been demonstrated. These affect both the shape, stability, dynamics, and excitations of fully polarised repulsive Bose or Fermi gases. Beyond the mean-field instability, strong dipolar interactions competing with slightly weaker contact interactions between magnetic bosons yield new quantum-stabilised states, among which are self-bound droplets, droplet assemblies, and supersolids. Dipolar interactions also deeply affect the physics of atomic gases with an internal degree of freedom as these interactions intrinsically couple spin and atomic motion. Finally, long-range dipolar interactions can stabilise strongly correlated excited states of 1D gases and also impact the physics of lattice-confined systems, both at the spin-polarised level (Hubbard models with off-site interactions) and at the spinful level (XYZ models). In the present manuscript, we aim to provide an extensive overview of the various related experimental achievements up to the present.
Ultracold atom experiments offer the unique opportunity to study mixing of different types of superfluid states. Our interest is in superfluid mixtures comprising of particles with different statistics---Bose and Fermi. Such scenarios occur naturally, for example, in dense quantum chromodynamics (QCD) matter. Interestingly, cold atomic experiments are performed in traps with finite spatial extent, thus critically destabilizing the occurrence of various homogeneous phases. Critical to this analysis is the understanding that the trapped system can undergo phase separation, resulting in a unique situation where phase transition in either species (bosons or fermions) can overlap with the phase separation between possible phases. In the present work, we illustrate how this intriguing interplay manifests in an interacting two-species atomic mixture---one bosonic and another fermionic with two spin components---within a realistic trap configuration. We further show that such interplay of transitions can render the nature of the ground state to be highly sensitive to the experimental parameters and the dimensionality of the system.
Gaseous Bose-Einstein condensates with nonzero spin feature multicomponent order parameters that reflect the internal degrees of freedom. They exhibit a rich variety of superfluid and magnetic phenomena similar or complementary to those of superfluid helium-3. The unprecedented degree of manipulability of atomic gases makes spinor condensates a unique playground for exploring symmetry breaking, topological excitations, and the interplay between superfluidity and magnetism. An overview of these subjects is provided.