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arXiv:2402.13873 · Physical Review Research

Time-reversal in a dipolar quantum many-body spin system

Sebastian Geier, Adrian Braemer, Eduard Braun, Maximilian Müllenbach, Titus Franz, Martin Gärttner, G. Zürn, Matthias Weidemüller

Published Aug 21, 2024• 11 citations
arXivHTMLPDF

Abstract

Time reversal in a macroscopic system contradicts daily experience. It is practically impossible to restore a shattered cup to its original state by just time reversing the microscopic dynamics that led to its breakage. Yet, with the precise control capabilities provided by modern quantum technology, the unitary evolution of a quantum system can be reversed in time. Here, we implement a time-reversal protocol in a dipolar interacting, isolated many-body spin system represented by Rydberg states in an atomic gas. By changing the states encoding the spin, we flip the sign of the interaction Hamiltonian, and demonstrate the reversal of the relaxation dynamics of the magnetization by letting a demagnetized many-body state evolve back in time into a magnetized state. We elucidate the role of atomic motion using the concept of a Loschmidt echo. Finally, by combining the approach with Floquet engineering, we demonstrate time reversal for a large family of spin models with different symmetries. Our method of state transfer is applicable across a wide range of quantum simulation platforms and has applications far beyond quantum many-body physics, reaching from quantum-enhanced sensing to quantum information scrambling. Published by the American Physical Society 2024

DOI
10.1103/physrevresearch.6.033197

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Time reversal in a macroscopic system contradicts daily experience. It is practically impossible to restore a shattered cup to its original state by just time reversing the microscopic dynamics that led to its breakage. Yet, with the precise control capabilities provided by modern quantum technology, the unitary evolution of a quantum system can be reversed in time. Here, we implement a time-reversal protocol in a dipolar interacting, isolated many-body spin system represented by Rydberg states in an atomic gas. By changing the states encoding the spin, we flip the sign of the interaction Hamiltonian, and demonstrate the reversal of the relaxation dynamics of the magnetization by letting a demagnetized many-body state evolve back in time into a magnetized state. We elucidate the role of atomic motion using the concept of a Loschmidt echo. Finally, by combining the approach with Floquet engineering, we demonstrate time reversal for a large family of spin models with different symmetries. Our method of state transfer is applicable across a wide range of quantum simulation platforms and has applications far beyond quantum many-body physics, reaching from quantum-enhanced sensing to quantum information scrambling. Published by the American Physical Society 2024
Quantum-enhanced metrology relies on entanglement to achieve sensitivities beyond the standard quantum limit. While remarkable progress has been made in generating highly entangled many-body states, extracting their metrological advantage remains a central challenge because the encoded information is often inaccessible to realistic measurements. A key development of the past decade has been the realization that many-body interactions can play a dual role: they can be used not only to generate entanglement, but also to decode it. This idea underlies interaction-based readout and time-reversal protocols, in which controlled non-linear dynamics transform weakly encoded signals into experimentally accessible observables. Cavity quantum electrodynamics (QED) provides a particularly powerful setting for these approaches because it combines collective enhancement, tunable interactions, and controllable reversibility within a single platform. In this review, we discuss the emergence of time-reversal protocols in cavity QED, from their conceptual roots in Loschmidt echoes to modern implementations of signal amplification through a time-reversed interaction (SATIN), scrambling-enhanced metrology, and more general interaction-based readout schemes. We examine the physical mechanisms that enable reversible many-body dynamics, review key experimental demonstrations, and discuss future directions involving complex entangled states, nonlinear decoding, and emerging quantum platforms. Together, these developments suggest that the ability to decode quantum information may become as important as the ability to generate it, establishing reversible many-body dynamics as a central resource for quantum-enhanced sensing.
In the long quest to identify and compensate the sources of decoherence in many-body systems far from the ground state, the varied family of Loschmidt echoes (LEs) became an invaluable tool in several experimental techniques. A LE involves a time-reversal procedure to assess the effect of perturbations in a quantum excitation dynamics. However, when addressing macroscopic systems one is repeatedly confronted with limitations that seem insurmountable. This led to the formulation of the central hypothesis of irreversibility stating that the timescale of decoherence, T3{T}_{3}T3​, is proportional to the timescale of the many-body interactions we reversed, T2{T}_{2}T2​. We test this by implementing two experimental schemes based on Floquet Hamiltonians where the effective strength of the dipolar spin-spin coupling, i.e., 1/T21/{T}_{2}1/T2​, is reduced by a variable scale factor kkk. This extends the perturbation timescale, ${T}_{\mathrm{\ensuremath{\Sigma}}}$, in relation to T2{T}_{2}T2​. Strikingly, we observe the superposition of the normalized Loschmidt echoes for the bigger values of kkk. This manifests the dominance of the intrinsic dynamics over the perturbation factors, even when the Loschmidt echo is devised to reverse that intrinsic dynamics. Thus, in the limit where the reversible interactions dominate over perturbations, the LE decays within a timescale, ${T}_{3}\ensuremath{\approx}{T}_{2}/R$ with $R=(0.15\ifmmode\pm\else\textpm\fi{}0.01)$, confirming the emergence of a perturbation independent regime. These results support the central hypothesis of irreversibility.
I discuss the time reversal of nonlinear many-body Hamiltonians and its application to the fields of quantum metrology and quantum information science. I present the experimental realization of such a protocol in an optically engineered many-body spin Hamiltonian. We used time-reversed Hamiltonian approach to achieve metrological gains well beyond the limit of the readout scheme. Moreover, with the same protocol, we experimentally elucidate the intimate relation between quantum information scrambling, out-of-time-order correlators, and metrological gain. In particular, I will highlight the robustness of time reversal protocols, and how these render many fast-scrambling and complex Hamiltonians useful for quantum-enhanced metrology.
If a magnetic polarization excess is locally injected in a crystal of interacting spins in thermal equilibrium, this 'excitation' would spread as consequence of spin-spin interactions. Such an apparently irreversible process is known as spin diffusion and it can lead the system back to 'equilibrium'. Even so, a unitary quantum dynamics would ensure a precise memory of the non-equilibrium initial condition. Then, if at a certain time, say , an experimental protocol reverses the many-body dynamics by changing the sign of the effective Hamiltonian, it would drive the system back to the initial non-equilibrium state at time t. As a matter of fact, the reversal is always perturbed by small experimental imperfections and/or uncontrolled internal or environmental degrees of freedom. This limits the amount of signal M(t) recovered locally at time t. The degradation of M(t) accounts for these perturbations, which can also be seen as the sources of decoherence. This general idea defines the Loschmidt echo (LE), which embodies the various time-reversal procedures implemented in nuclear magnetic resonance. Here, we present an invitation to the study of the LE following the pathway induced by the experiments. With such a purpose, we provide a historical and conceptual overview that briefly revisits selected phenomena that underlie the LE dynamics including chaos, decoherence, localization and equilibration. This guiding thread ultimately leads us to the discussion of decoherence and irreversibility as an emergent phenomenon. In addition, we introduce the LE formalism by means of spin-spin correlation functions in a manner suitable for presentation in a broad scope physics journal. Last, but not least, we present new results that could trigger new experiments and theoretical ideas. In particular, we propose to transform an initially localized excitation into a more complex initial state, enabling a dynamically prepared LE. This induces a global definition of the LE in terms of the raw overlap between many-body wave functions. Our results show that as the complexity of the prepared state increases, it becomes more fragile towards small perturbations.
Abstract If a magnetic polarization excess is locally injected in a crystal of interacting spins in thermal equilibrium, this ‘excitation’ would spread as consequence of spin–spin interactions. Such an apparently irreversible process is known as spin diffusion and it can lead the system back to ‘equilibrium’. Even so, a unitary quantum dynamics would ensure a precise memory of the non-equilibrium initial condition. Then, if at a certain time, say t / 2 , an experimental protocol reverses the many-body dynamics by changing the sign of the effective Hamiltonian, it would drive the system back to the initial non-equilibrium state at time t . As a matter of fact, the reversal is always perturbed by small experimental imperfections and/or uncontrolled internal or environmental degrees of freedom. This limits the amount of signal M ( t ) recovered locally at time t . The degradation of M ( t ) accounts for these perturbations, which can also be seen as the sources of decoherence. This general idea defines the Loschmidt echo (LE), which embodies the various time-reversal procedures implemented in nuclear magnetic resonance. Here, we present an invitation to the study of the LE following the pathway induced by the experiments. With such a purpose, we provide a historical and conceptual overview that briefly revisits selected phenomena that underlie the LE dynamics including chaos, decoherence, localization and equilibration. This guiding thread ultimately leads us to the discussion of decoherence and irreversibility as an emergent phenomenon. In addition, we introduce the LE formalism by means of spin–spin correlation functions in a manner suitable for presentation in a broad scope physics journal. Last, but not least, we present new results that could trigger new experiments and theoretical ideas. In particular, we propose to transform an initially localized excitation into a more complex initial state, enabling a dynamically prepared LE. This induces a global definition of the LE in terms of the raw overlap between many-body wave functions. Our results show that as the complexity of the prepared state increases, it becomes more fragile towards small perturbations.
Controlling interactions is the key element for the quantum engineering of many-body systems. Using time-periodic driving, a naturally given many-body Hamiltonian of a closed quantum system can be transformed into an effective target Hamiltonian that exhibits vastly different dynamics. We demonstrate such Floquet engineering with a system of spins represented by Rydberg states in an ultracold atomic gas. By applying a sequence of spin manipulations, we change the symmetry properties of the effective Heisenberg XYZ Hamiltonian. As a consequence, the relaxation behavior of the total spin is drastically modified. The observed dynamics can be qualitatively captured by a semiclassical simulation. Engineering a wide range of Hamiltonians opens vast opportunities for implementing quantum simulation of nonequilibrium dynamics in a single experimental setting.