This thesis presents studies performed on open quantum systems, that is, quantum systems interacting with their surrounding environment. Such systems are important not only in understanding the quantum-to-classical transition but also for the practical implementation of modern quantum technologies. In studies of open quantum systems performed to date, a very common assumption is that the system and the environment are in separated initial states to begin with. One primary objective of this thesis is to critically analyse this assumption. We follow two different approaches to investigate the dynamics. First, we solve an exactly solvable spin-spin model where a central spin system interacts with a collection of quantum spins. We analyse exactly the central spin dynamics, starting from both initially correlated and uncorrelated SE states, and look at the dynamical differences due to the different starting states. Second, we consider an arbitrary system interacting with an arbitrary environment and derive a master equation that describes the system dynamics and incorporates the effect of the initial SE correlations. This effect of initial correlations is captured by an extra term appearing in the master equation. The master equation is subsequently applied to the paradigmatic SE models such as the spin-boson model and the spin-spin model. We demonstrate that the role played by initial correlations can be noticeable even if the SE coupling strength is kept smaller. The next part of the thesis deals with estimating the parameters characterizing the environment of a quantum system where we show that the use of two two-level systems can greatly enhance the estimation of the environment parameters.
This thesis presents studies performed on open quantum systems, that is, quantum systems interacting with their surrounding environment. Such systems are important not only in understanding the quantum-to-classical transition but also for the practical implementation of modern quantum technologies. In studies of open quantum systems performed to date, a very common assumption is that the system and the environment are in separated initial states to begin with. One primary objective of this thesis is to critically analyse this assumption. We follow two different approaches to investigate the dynamics. First, we solve an exactly solvable spin-spin model where a central spin system interacts with a collection of quantum spins. We analyse exactly the central spin dynamics, starting from both initially correlated and uncorrelated SE states, and look at the dynamical differences due to the different starting states. Second, we consider an arbitrary system interacting with an arbitrary environment and derive a master equation that describes the system dynamics and incorporates the effect of the initial SE correlations. This effect of initial correlations is captured by an extra term appearing in the master equation. The master equation is subsequently applied to the paradigmatic SE models such as the spin-boson model and the spin-spin model. We demonstrate that the role played by initial correlations can be noticeable even if the SE coupling strength is kept smaller. The next part of the thesis deals with estimating the parameters characterizing the environment of a quantum system where we show that the use of two two-level systems can greatly enhance the estimation of the environment parameters.
Open quantum systems are a subject of immense interest as their understanding is crucial in the implementation of modern quantum technologies. In the study of their dynamics, the role of the initial system–environment correlations is commonly ignored. In this work, to gain insights into the role of these correlations, we solve an exactly solvable model of a single two-level system interacting with a spin environment, with the initial system state prepared by a suitable unitary operation. By solving the dynamics exactly for arbitrary system–environment coupling strength while taking into account the initial system–environment correlations, we show that the effect of the initial correlations is, in general, very significant and nontrivial. To further highlight the importance of the initial system–environment correlations, we also extend our study to investigate the dynamics of the entanglement between two two-level systems interacting with a common spin environment.
In order to achieve practical implementations of emerging quantum technologies, it is important to have a firm understanding of the dynamics of realistic quantum open systems. Master equations provide a widely used tool in this regard. In this work we first construct a master equation, valid for weak system-environment coupling, which explicitly takes into account the impact of preparing an initial system state from an equilibrium system-environment state that has system-environment correlations. We then investigate the role of initial system-environment correlations using this master equation for a system consisting of many two-level atoms interacting with a common environment. We show that, in general, due to the initial system-environment correlations before a state preparation, the quantum state of the system can evolve at a faster time scale. Moreover, we also consider different initial state preparations, and demonstrate that the influence of state preparations depends on the initial states prepared. Our results can be of interest to many topics based on quantum open systems where system-environment correlation effects have been neglected before.
A central aim of physics is to describe the dynamics of physical sys-tems. Schrödinger’s equation does this for isolated quantum systems. Describing the time evolution of a quantum system that interacts with its environment, in its most general form, has proved to be difficult because the dynamics is dependent on the state of the environment and the corre-lations with it. For discrete processes, such as quantum gates or chemical reactions, quantum process tomography provides the complete descrip-tion of the dynamics, provided that the initial states of the system and the environment are independent of each other. However, many physical systems are correlated with the environment at the beginning of the ex-periment. Here, we give a prescription of quantum process tomography that yields the complete description of the dynamics of the system even when the initial correlations are present. Surprisingly, our method also gives quantitative expressions for the initial correlation. There is a rich history to the studies of decoherence of quantum systems due to the interactions with the surrounding degrees of freedom. When the dynamics of the system (S) is Markovian it can be described by a master equation [1, 2, 3]. Nowadays many researchers are interested in systems that are non-Markovian, as there is mounting evidence that some natural systems of importance may be non-Markovian [4] and such features may allow to manipulate and control quantum systems in desired ways. There is also a great deal of interest in systems that are initially correlated with their environments (E) because non-Markovianity and initial system-environment (SE) correlations are intimately related [5, 6, 7]. 1 ar
Quantum mechanics has both deepened our understanding of the physical reality and allowed development of quantum technologies beating their classical counterparts in efficiency, security, and sensitivity. As a major downside, the quantum properties behind these technologies are very sensitive to the effects the system’s interaction with its environment. The theory of open quantum systems describes how such interaction influences the system, and as a consequence, how the quantum features are lost, controlled, and possibly returned by manipulating the environment. This thesis begins with a short description of the most relevant features and results of the open quantum system theory. We continue by presenting some commonly used measures to quantify the information encoded in quantum systems and the correlations between spatially or temporally separated parties. The literature review ends with discussion of non-Markovianity and memory effects which combine the fields of open quantum systems and quantum information in a natural way. The rest of the thesis presents the main results of Publications I – VII. We study the memory effects and physicality conditions of open system dynamics described by the vast family of phase-covariant master equations. We show how the open quantum system picture can be exploited to design probing protocols to extract information without knowing how the probe and system interact. Such protocols are considered also from the point-of view of efficiently obtaining the information required in the probing, both in theory and by experimental implementation. The experiment serves also as evidence for applicability of recently developed geometric tools to design informationally incomplete measurements for solving so-called membership problems. We present and experimentally realize a protocol where control over intial correlations between polarization and frequency gives full freedom to implement any dephasing dynamics in the open system polarization, thus dictating how its information content changes in time. We study the two-qubit memory effects of dephasing dynamics and compare them to the effect of such noise in the transmission efficiency in superdense coding. Optimal noise configurations in different situations are found. Finally, we characterize the families of initial states for which the decay of quantum correlations depends or does not depend on the noise location.
We present a general master equation, correct to second order in the system-environment coupling strength, that takes into account the initial system-environment correlations. We assume that the system and its environment are in a joint thermal equilibrium state, and thereafter, a unitary operation is performed to prepare the desired initial system state, with the system Hamiltonian possibly changing thereafter as well. We show that the effect of the initial correlations shows up in the second-order master equation as an additional term, similar in form to the usual second-order term describing relaxation and decoherence in quantum systems. We apply this master equation to a generalization of the paradigmatic spin-boson model, namely, a collection of two-level systems interacting with a common environment of harmonic oscillators, as well as a collection of two-level systems interacting with a common spin environment. We demonstrate that, in general, the initial system-environment correlations need to be accounted for in order to accurately obtain the system dynamics.
This thesis investigates two thematic lines of research, both underpinned by non-Markovian system-reservoir interactions in quantum optics. The overarching focus is on modelling the open system dynamics in a non-perturbative fashion, broadly on - though not restricted to - instances when the environment is structured. A theory is developed by means of enlarging the open system over environmental degrees of freedom to include memory effects in its dynamics. This is achieved using an established technique that involves mapping a bosonic environment onto a 1D chain of harmonic oscillators. Within this setting, we apply a Heisenberg equation-of-motion approach to derive an exact set coupled differential equations for the open system and a single auxiliary oscillator of the chain. The combined equations are shown to have their interpretation rooted in a quantum Markov stochastic process. Including the auxiliary chain oscillator as part of the original system then enables us to obtain an exact master equation for the enlarged system, avoiding any need for the Born-Markov approximations. Our method is valid for a dissipative two-state system, with cases of multiple excitations and added driving discussed. Separately, we apply the framework of quantum Darwinism to an atom-cavity system, and, subsequently, to a more general multiple-environment model. In both cases, the time-dependent spread of correlations between the open system and fractions of the environment is analysed during the course of the decoherence process. The degree to which information is redundant across different fractions is checked to infer the emergence of classicality. In the second case, we go further and present a decomposition of information in terms of its quantum and classical correlations. A quantitative measure of redundancy is also studied with regard to its ability to witness non-Markovian behaviour. Besides fundamental interest, our results have application to quantum information processing and quantum technologies, keeping in mind the potential beneficial use of non-Markovian effects in reservoir engineering.