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arXiv:2402.02839 · Nature Communications

Measuring topological invariants for higher-order exceptional points in quantum three-mode systems

Pei‐Rong Han, Wen Ning, Xin-Jie Huang, Ri‐Hua Zheng, Shou‐Bang Yang, Fan Wu, Zhen‐Biao Yang, Qi-Ping Su, Chui‐Ping Yang, Shi‐Biao Zheng

Published Nov 27, 2024• 16 citations
arXivHTMLPDF

Abstract

Owing to the presence of exceptional points (EPs), non-Hermitian (NH) systems can display intriguing topological phenomena without Hermitian analogs. However, experimental characterizations of exceptional topological invariants have been restricted to second-order EPs (EP2s) in classical or semiclassical systems. We here propose an NH multi-mode system with higher-order EPs, each of which is underlain by a multifold-degenerate multipartite entangled eigenstate. We implement the NH model by controllably coupling a Josephson-junction-based electronic mode to two microwave resonators. We experimentally quantify the topological invariant for an EP3, by mapping out the complex eigenspectra of the tripartite system along a loop surrounding this EP3 in the parameter space. The nonclassicality of the realized topology is manifested by the observed quantum correlations in the corresponding eigenstates. Our results extend research of exceptional topology to fully quantum-mechanical models with multipartite entangled eigenstates. Exceptional topology associated with higher-order exceptional points has not been completely characterised in quantum systems. Here, the authors fill this gap performing full quantum state tomography in a system composed of a superconducting qubit coupled to two cavities, one lossless and one lossy, featuring third-order exceptional points.

DOI
10.1038/s41467-024-54662-8

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Owing to the presence of exceptional points (EPs), non-Hermitian (NH) systems can display intriguing topological phenomena without Hermitian analogs. However, experimental characterizations of exceptional topological invariants have been restricted to second-order EPs (EP2s) in classical or semiclassical systems. We here propose an NH multi-mode system with higher-order EPs, each of which is underlain by a multifold-degenerate multipartite entangled eigenstate. We implement the NH model by controllably coupling a Josephson-junction-based electronic mode to two microwave resonators. We experimentally quantify the topological invariant for an EP3, by mapping out the complex eigenspectra of the tripartite system along a loop surrounding this EP3 in the parameter space. The nonclassicality of the realized topology is manifested by the observed quantum correlations in the corresponding eigenstates. Our results extend research of exceptional topology to fully quantum-mechanical models with multipartite entangled eigenstates. Exceptional topology associated with higher-order exceptional points has not been completely characterised in quantum systems. Here, the authors fill this gap performing full quantum state tomography in a system composed of a superconducting qubit coupled to two cavities, one lossless and one lossy, featuring third-order exceptional points.
Non-Hermitian systems exhibit a variety of unique features rooted in the presence of exceptional points (EPs). The distinct topological structure in the proximity of an EP gives rise to counterintuitive behaviors absent in Hermitian systems, which emerge after encircling the EP either quasistatically or dynamically. However, experimental exploration of EP encirclement in quantum systems, particularly those involving high-order EPs, remains challenging due to the difficulty of coherently controlling more degrees of freedom. In this work, we experimentally investigate the eigenvalue braiding and state transfer arising from the encirclement of EP in a three-dimensional non-Hermitian quantum system using superconducting circuits. We characterize the second- and third-order EPs through the coalescence of eigenvalues. Then we reveal the topological structure near the EP3 by quasistatically encircling it along various paths with three independent parameters, which yields the eigenvalue braiding described by the braid group B 3 . Additionally, we observe chiral state transfer between three eigenstates under a fast driving scheme when no EPs are enclosed, while time-symmetric behavior occurs when at least one EP is encircled. Our findings offer insights into understanding non-Hermitian topological structures and the manipulation of quantum states through dynamic operations.
The appearance of topological singularities, namely exceptional points (EPs) is an intriguing feature of parameter-dependent open quantum or wave systems. EPs are the special type of nonHermitian degeneracies where two (or more) eigenstates of the underlying system coalesce. In this paper, we present a three level non-Hermitian Hamiltonian which hosts three interacting eigenstates. The matrix elements are optimized in such a way that the intermediate eigenstate interacts with both the other states and the underlying system hosts at least two different second order EPs. The impact of quasi-static parameter variation along a cyclic contour around the embedded EPs on the dynamics of interacting eigenvalues is well investigated in the context of cascaded state conversion. Such dynamics of the eigenvalues shows a clear signature of the third order EP with a combined effect of both the second order EPs. Moreover, we examine the accumulation of phases around the identified EPs and study the hallmark of phase exchange during cascaded state conversions accompanied by the parametric encirclement of the third order EP.
The exploration of the effect of non-Hermitian (NH) in quantum systems is gaining renewed momentum as a result of the recent progress in experiments. It has been indicated that the ability to engineer the orders of exceptional points (EPs) can be fundamental to its applications in quantum control, such as accelerating entanglement generation; however, an initial survey of the interactions between different orders of EPs is still missing. In this work, we try to partially address this issue by employing a non-reciprocally coupled cavity system which can be experimentally realizable with a two-dimensional reconfigurable NH gauged laser array. With deliberate design, our systems display both second and third orders of EPs. The sign of a novel, purely quantum continuous entanglement phase transition is observed, which reveals how multi-EP interactions alter entanglement dynamics across different regimes while maintaining accelerated generation. Our findings reveil the genuinely quantum NH physics of higher-order EPs, which has opened up a new avenue for future investigations of the higher-order degeneracy application and the dynamic phase transitions of quantum systems.
Non-Hermitian (NH) systems can display exotic topological phenomena without Hermitian counterparts, enabled by exceptional points (EPs). So far, investigations of NH topology have been restricted to EPs of the NH Hamiltonian, which governs the system dynamics conditional upon no quantum jumps occurring. The Liouvillian superoperator, which combines the effects of quantum jumps with NH Hamiltonian dynamics, possesses EPs (LEPs) that are significantly different from those of the corresponding NH Hamiltonian. We here study the topological features of the LEPs in the system consisting of a qubit coupled to a non-Markovian reservoir. We find that two distinct winding numbers can be simultaneously produced by executing a single closed path encircling the twofold LEP2, formed by two coinciding LEP2s, each involving a pair of coalescing eigenvectors of the extended Liouvillian superoperator. We experimentally demonstrate this purely non-Markovian phenomenon with a circuit, where a superconducting qubit is coupled to a decaying resonator which acts as a reservoir with memory effects. The results push the exploration of exceptional topology from the Markovian to non-Markovian regime.
One of the most remarkable features that distinguish open systems from closed ones is the presence of exceptional points (EPs), where two or more eigenvectors of a non-Hermitian operator coalesce, accompanying the convergence of the corresponding eigenvalues. So far, EPs have been demonstrated on a number of platforms, ranging from classical optical systems to fully quantum-mechanical spin-boson models. In these demonstrations, the reservoir that induced the non-Hermiticity was treated as a Markovian one, without considering its memory effect. We here present the first experimental demonstration of non-Markovian quantum EPs, engineered by coupling a Josephson-junction-based qubit to a leaky electromagnetic resonator, which acts as a non-Markovian reservoir. We map out the spectrum of the extended Liouvillian superoperator by observing the quantum state evolution of the qubit and the pseudomode, in which the memory of the reservoir is encoded. We identify a twofold second-order EP and a third-order EP in the Liouvillian spectrum, which cannot be realized with a Markovian reservoir. Our results pave the way for experimental exploration of exotic phenomena associated with non-Markovian quantum EPs.
Exceptional points (EPs) are non-Hermitian spectral singularities exhibiting fractional-power responses, yet their implications for multipartite entanglement of interacting quantum many-body systems remain largely unexplored. Here we develop a general framework that links higher-order non-Hermitian degeneracies to the scaling behavior of genuine multipartite entanglement in interacting identical-qubit systems. Permutation symmetry of the identical qubits decomposes the exponentially large Hilbert space into independent irreducible-representation sectors, thereby constraining the maximal EP order of NNN qubits to N+1N+1N+1 rather than 2N2^N2N. Near an nnnth-order EP, genuine multipartite entanglement inherits the spectral response and generically exhibits a fractional-power scaling under weak perturbations. Explicit examples show that conventional two-body interactions support third- and fourth-order EPs with the corresponding entanglement responses, whereas higher-order EPs with genuine multipartite-entangled coalesced states require additional independent interaction channels, such as three-body interactions. Our results establish a fundamental connection among non-Hermitian degeneracies, multipartite entanglement, and symmetry, extending higher-order EP physics from spectral singularities to genuine many-body quantum correlations.