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arXiv:2402.01308 · Progress in Nuclear Magnetic Resonance Spectroscopy

Controlling NMR spin systems for quantum computation

Jonathan A. Jones

Published Feb 9, 2024• 16 citations
arXivHTMLPDF

Abstract

Nuclear magnetic resonance is arguably both the best available quantum technology for implementing simple quantum computing experiments and the worst technology for building large scale quantum computers that has ever been seriously put forward. After a few years of rapid growth, leading to an implementation of Shor's quantum factoring algorithm in a seven-spin system, the field started to reach its natural limits and further progress became challenging. Rather than pursuing more complex algorithms on larger systems, interest has now largely moved into developing techniques for the precise and efficient manipulation of spin states with the aim of developing methods that can be applied in other more scalable technologies and within conventional NMR. However, the user friendliness of NMR implementations means that they remain popular for proof-of-principle demonstrations of simple quantum information protocols.

DOI
10.1016/j.pnmrs.2024.02.002

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Nuclear magnetic resonance is arguably both the best available quantum technology for implementing simple quantum computing experiments and the worst technology for building large scale quantum computers that has ever been seriously put forward. After a few years of rapid growth, leading to an implementation of Shor's quantum factoring algorithm in a seven-spin system, the field started to reach its natural limits and further progress became challenging. Rather than pursuing more complex algorithms on larger systems, interest has now largely moved into developing techniques for the precise and efficient manipulation of spin states with the aim of developing methods that can be applied in other more scalable technologies and within conventional NMR. However, the user friendliness of NMR implementations means that they remain popular for proof-of-principle demonstrations of simple quantum information protocols.
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Quantum information processing is the use of inherently quantum mechanical phenomena to perform information processing tasks that cannot be achieved using conventional classical information technologies. One famous example is quantum computing, which would permit calculations to be performed that are beyond the reach of any conceivable conventional computer. Initially it appeared that actually building a quantum computer would be extremely difficult, but in the last few years there has been an explosion of interest in the use of techniques adapted from conventional liquid state nuclear magnetic resonance (NMR) experiments to build small quantum computers. After a brief introduction to quantum computing I will review the current state of the art, describe some of the topics of current interest, and assess the long term contribution of NMR studies to the eventual implementation of practical quantum computers capable of solving real computational problems.
We have taken significant steps towards the realization of a practical quantum computer: using nuclear spins and magnetic resonance techniques at room temperature, we provided proof of principle of quantum computing in a series of experiments which culminated in the implementation of the simplest instance of Shor's quantum algorithm for prime factorization (15=3x5), using a seven-spin molecule. This algorithm achieves an exponential advantage over the best known classical factoring algorithms and its implementation represents a milestone in the experimental exploration of quantum computation. These remarkable successes have been made possible by the synthesis of suitable molecules and the development of many novel techniques for initialization, coherent control and readout of the state of multiple coupled nuclear spins. Furthermore, we devised and implemented a model to simulate both unitary and decoherence processes in these systems, in order to study and quantify the impact of various technological as well as fundamental sources of errors. In summary, this work has given us a much needed practical appreciation of what it takes to build a quantum computer. While liquid NMR quantum computing has well-understood scaling limitations, many of the techniques that originated from this research may find use in other, perhaps more scalable quantum computer implementations.
Nuclear Magnetic Resonance (NMR) forms a natural test-bed to perform quantum information processing (QIP) and has so far proven to be one of the most successful quantum information processors. The nuclear spins in a molecule treated as quantum bits or qubits which are the basic building blocks of a quantum computer. The development of NMR over half a century puts it in a platform where we can utilize its excellent control techniques over an ensemble of spin systems and perform quantum computation in a highly controlled way. Apart from a successful quantum information processor, NMR is also a highly powerful quantum platform where many of the potentially challenging quantum mechanical experiments can be performed.
Fifty years of developments in nuclear magnetic resonance (NMR) have resulted in an unrivaled degree of control of the dynamics of coupled two-level quantum systems. This coherent control of nuclear spin dynamics has recently been taken to a new level, motivated by the interest in quantum information processing. NMR has been the workhorse for the experimental implementation of quantum protocols, allowing exquisite control of systems up to seven qubits in size. This article surveys and summarizes a broad variety of pulse control and tomographic techniques which have been developed for, and used in, NMR quantum computation. Many of these will be useful in other quantum systems now being considered for the implementation of quantum information processing tasks.
Rapid developments in quantum information processing have been made, and remarkable achievements have been obtained in recent years, both in theory and experiments. Coherent control of nuclear spin dynamics is a powerful tool for the experimental implementation of quantum schemes in liquid and solid nuclear magnetic resonance (NMR) system, especially in liquid-state NMR. Compared with other quantum information processing systems, the NMR platform has the advantages such as the long coherence time, the precise manipulation, and well-developed quantum control techniques, which make it possible to accurately control a quantum system with up to 12-qubits. Extensive applications of liquid-state NMR spectroscopy in quantum information processing such as quantum communication, quantum computing, and quantum simulation have been thoroughly studied over half a century. This article introduces the general principles of NMR quantum information processing, and reviews the new-developed techniques. The review will also include the recent achievements of the experimental realization of quantum algorithms for machine learning, quantum simulations for high energy physics, and topological order in NMR. We also discuss the limitation and prospect of liquid-state NMR spectroscopy and the solid-state NMR systems as quantum computing in the article.