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arXiv:2401.11830 · Physical Review Research

Non-Hermitian pseudomodes for strongly coupled open quantum systems: Unravelings, correlations, and thermodynamics

Paul Menczel, Ken Funo, Mauro Cirio, Neill Lambert, Franco Nori

Published Sep 3, 2024• 38 citations
arXivHTMLPDF

Abstract

The pseudomode framework provides an exact description of the dynamics of an open quantum system coupled to a non-Markovian environment. Using this framework, the influence of the environment on the system is studied in an equivalent model, where the open system is coupled to a finite number of unphysical pseudomodes that follow a time-local master equation. Building on the insight that this master equation does not need to conserve the hermiticity of the pseudomode state, we here ask for the most general conditions on the master equation that guarantee the correct reproduction of the system's original dynamics. We demonstrate that our generalized approach decreases the number of pseudomodes that are required to model, for example, underdamped environments at finite temperature. We also provide an unraveling of the master equation into quantum jump trajectories of non-Hermitian states, which further facilitates the utilization of the pseudomode technique for numerical calculations by enabling the use of easily parallelizable Monte Carlo simulations. Finally, we show that pseudomodes, despite their unphysical nature, provide a natural picture in which physical processes, such as the creation of system-bath correlations or the exchange of heat, can be studied. Hence, our results pave the way for future investigations of the system-environment interaction leading to a better understanding of open quantum systems far from the Markovian weak-coupling limit. Published by the American Physical Society 2024

DOI
10.1103/physrevresearch.6.033237

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The pseudomode framework provides an exact description of the dynamics of an open quantum system coupled to a non-Markovian environment. Using this framework, the influence of the environment on the system is studied in an equivalent model, where the open system is coupled to a finite number of unphysical pseudomodes that follow a time-local master equation. Building on the insight that this master equation does not need to conserve the hermiticity of the pseudomode state, we here ask for the most general conditions on the master equation that guarantee the correct reproduction of the system's original dynamics. We demonstrate that our generalized approach decreases the number of pseudomodes that are required to model, for example, underdamped environments at finite temperature. We also provide an unraveling of the master equation into quantum jump trajectories of non-Hermitian states, which further facilitates the utilization of the pseudomode technique for numerical calculations by enabling the use of easily parallelizable Monte Carlo simulations. Finally, we show that pseudomodes, despite their unphysical nature, provide a natural picture in which physical processes, such as the creation of system-bath correlations or the exchange of heat, can be studied. Hence, our results pave the way for future investigations of the system-environment interaction leading to a better understanding of open quantum systems far from the Markovian weak-coupling limit. Published by the American Physical Society 2024
The influence of a Gaussian environment on a quantum system can be described by effectively replacing the continuum with a discrete set of ancillary quantum and classical degrees of freedom. This defines a pseudomode model which can be used to classically simulate the reduced system dynamics. Here we consider an alternative point of view and analyze the potential benefits of an analog or digital quantum simulation of the pseudomode model itself. Superficially, such a direct experimental implementation is, in general, impossible due to the unphysical properties of the effective degrees of freedom involved. However, we show that the effects of the unphysical pseudomode model can still be reproduced using measurement results over an ensemble of physical systems involving ancillary harmonic modes and an optional stochastic driving field. This is done by introducing an extrapolation technique whose efficiency is limited by stability against imprecision in the measurement data. We examine how such a simulation would allow us to (i) perform a quantum simulation of the effects of complex nonperturbative and non-Markovian environments in regimes that are challenging for classical simulation; (ii) conversely, mitigate potential unwanted non-Markovian noise present in quantum devices; and (iii) restructure some of the properties of a given physical bath, such as its temperature. Published by the American Physical Society 2024
We outline a non-perturbative approach for simulating the behavior of open quantum systems interacting with a bosonic environment defined by a generalized spectral density function. The method is based on replacing the environment by a set of damped harmonic oscillators - the pseudomodes - thereby forming an enlarged open system whose dynamics is governed by a Markovian master equation. Each pseudomode is connected to one of the poles of the spectral density when analytically continued to the lower-half complex frequency plane. Here, we extend previous results to a completely generic class of open system models, and discuss how our framework can be used as a powerful and versatile tool for analyzing non-Markovian open system dynamics. The effectiveness of the method is demonstrated on the spin-boson model by accurately benchmarking its predictions against numerically exact results.
Pseudomode approaches allow for an exact and unapproximated description of a quantum system interacting arbitrarily strongly with a bath. In general, a system coupled to pseudomodes will not thermalize to the system's Gibbs state: This is to be expected when the system-bath coupling is non-perturbative, but conflicts with common thermodynamic intuition when the system-bath coupling is asymptotically weak. We explore under which circumstances pseudomode models satisfy detailed balance (and subsequently thermalize to the system Gibbs state) and how specific choices of parameters can force "weak" detailed balance that is restricted to a limited frequency range. A combination of Hermitian and non-Hermitian pseudomodes that yields a flat effective-temperature profile is also considered. The results and criteria established here are relevant for the construction of pseudomode models in contexts where thermodynamic consistency is required.
Recent advances in quantum technologies and related experiments have created a need for highly accurate, versatile, and computationally efficient simulation techniques for the dynamics of open quantum systems. Long-lived correlation effects (non-Markovianity), system-environment hybridization, and the necessity for accuracy beyond the Born-Markov approximation form particular challenges. Approaches to meet these challenges have been introduced, originating from different fields, such as hierarchical equations of motion, Lindblad-pseudomode formulas, chain-mapping approaches, quantum Brownian motion master equations, stochastic unravelings, and refined quantum master equations. This diversity, while indicative of the field's relevance, has inadvertently led to a fragmentation that hinders cohesive advances and their effective cross-community application to current problems for complex systems. How are different approaches related to each other? What are their strengths and limitations? Here we give a systematic overview and concise discussion addressing these questions. We make use of a unified framework which very conveniently allows to link different schemes and, this way, may also catalyze further progress. In line with the state of the art, this framework is formulated not in a fully reduced space of the system but in an extended state space which in a minimal fashion includes effective reservoir modes. This in turn offers a comprehensive understanding of existing methods, elucidating their physical interpretations, interconnections, and applicability.
We develop an exact framework for describing the non-Markovian dynamics of an open quantum system interacting with an environment modeled by a generalized spectral density function.The approach relies on mapping the initial system onto an auxiliary configuration, comprising the original open system coupled to a small number of discrete modes, which in turn are each coupled to an independent Markovian reservoir.Based on the connection between the discrete modes and the poles of the spectral density function, we show how expanding the system using the discrete modes allows for the full inclusion non-Markovian effects within an enlarged open system whose dynamics is governed by an exact Lindblad master equation.Initially we apply this result to obtain a generalization of the pseudomode method [B.M. Garraway, Phys. Rev. A. 55, 2290 (1997)] in cases where the spectral density function has a Lorentzian structure.For many other types of spectral density function, we extend our proof to show that an open system dynamics may be modeled physically using discrete modes which admit a non-Hermitian coupling to the system and for such cases determine the equivalent master equation to no longer be of Lindblad form.For applications involving two discrete modes, we demonstrate how to convert between pathological and Lindblad forms of the master equation using the techniques of the pseudomode method.
Stochastic unravelings provide a useful way to represent open quantum system dynamics in terms of pure state realizations, and have been widely studied both from a fundamental and from a computational point of view. They were initially formulated for Markovian dynamics described by the Gorini-Kossakowski-Sudarshan-Lindblad master equation. However, due to recent technological and experimental development, most physical relevant dynamics present temporal correlations beyond the Markov approximation. Such correlations cause decay rates to turn temporarily negative, thus requiring the generalization of stochastic unravelings from Markovian to non-Markovian scenarios. Indeed, many unraveling techniques have been introduced in this regime, and a comprehensive review of the different jump methods is currently missing. In this work, we provide an overview of widely used quantum jump unraveling techniques for non-Markovian systems and also discuss them in terms of their numerical efficiency, divisibility requirements, Hilbert space extension, and measurement interpretation.