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arXiv:2401.02319

Maximizing Purity and Heralding Efficiency of Type-I Down-Converted Photons Using Beam Focal Parameters

Andrew Rockovich, Wang, Shu'an, Daniel J. Gauthier

Published Jan 4, 2024• 1 citation
arXivHTMLPDF

Abstract

We demonstrate theoretically that correlated bi-photons can be generated with high heralding efficiency and high spectral purity for non-collinear Type-I spontaneous parametric down-conversion. In Type-I down-conversion, the generated photons have the same linear polarization that is perpendicular to the linear pump polarization. Previously, it was thought that high efficiency and purity could not be obtained for this configuration. We show that the non-collinear geometry gives an additional degree-of-freedom that allows for simultaneous optimization of these source metrics. We predict near-unity ($\approx0.97$) heralding efficiency and single-photon spectral purity by adjusting the beam focal parameters, which can be obtained over a wide range of pump, signal, and idler wavelengths without requiring special crystal dispersion characteristics. As an example, we predict a heralding efficiency of 0.97, a single-photon purity of 0.97, and a pair production rate of 0.50 pairs/(s$~$mW$~$THz) using a 400-$μ$m-long $β$-barium borate crystal pumped by a 355-nm-wavelength pulsed laser with a bandwidth of 8-THz. Our work offers a simple and universal approach for producing high-quality quantum photonic states for a wide variety of quantum information science applications.

DOI
10.48550/arxiv.2401.02319

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We demonstrate theoretically that correlated bi-photons can be generated with high heralding efficiency and high spectral purity for non-collinear Type-I spontaneous parametric down-conversion. In Type-I down-conversion, the generated photons have the same linear polarization that is perpendicular to the linear pump polarization. Previously, it was thought that high efficiency and purity could not be obtained for this configuration. We show that the non-collinear geometry gives an additional degree-of-freedom that allows for simultaneous optimization of these source metrics. We predict near-unity (≈0.97\approx0.97≈0.97) heralding efficiency and single-photon spectral purity by adjusting the beam focal parameters, which can be obtained over a wide range of pump, signal, and idler wavelengths without requiring special crystal dispersion characteristics. As an example, we predict a heralding efficiency of 0.97, a single-photon purity of 0.97, and a pair production rate of 0.50 pairs/(s ~ mW ~ THz) using a 400-μμμm-long βββ-barium borate crystal pumped by a 355-nm-wavelength pulsed laser with a bandwidth of 8-THz. Our work offers a simple and universal approach for producing high-quality quantum photonic states for a wide variety of quantum information science applications.
Spontaneous parametric down-conversion (SPDC) is a reliable and robust source of photons for quantum information applications. For applications that involve operations such as entanglement swapping or single-photon heralding, two-photon states are required to be factorable (uncorrelated) in their spectral and spatial degrees of freedom. We report the design and experimental characterization of an SPDC source that has been optimized for high spectral and spatial purity. The source is pumped by the 776 nm output of a mode-locked Ti:Sapphire laser and consists of a periodically-poled Potassium Titanyl Phosphate (PPKTP) crystal phase-matched for collinear type-II SPDC. The dispersive properties of PPKTP at these wavelengths is such that it is possible to minimize the spectral entanglement by matching the widths of the pump to the spectral phase-matching function. The spatial entanglement is minimized through careful control of the pump focus, yielding nearly single-mode emission. An advantage of this approach is that the emission rate into the collection modes is very high, resulting in a very bright SPDC source. We also report a scheme that employs the output of collinear sources such as these to produce polarization-entangled photon pairs. The scheme, which requires only simple polarization elements, can be scaled to N-photon GHZ states.
The nonlinear optical process of spontaneous parametric down-conversion (SPDC) is widely studied for applications in quantum information science due to its ability to produce two photons that can be entangled in many degrees of freedom. For applications in quantum communication, two metrics of this process are particularly important: heralding efficiency and total joint rate. Here, we derive expressions for both quantities for a variety of different beam geometries and frequencies. We pay specific attention to the spectrum of both biphotons and individual photons. We reveal the underlying mechanisms responsible for the spectral shape and show they differ for different geometries and frequencies. We then use these spectra to calculate heralding efficiency and joint count rate and examine how each of these metrics changes with different geometries, frequencies, spectral filtering, and beam parameters. Interestingly, we find very high heralding efficiencies are achievable for collinear geometries without spectral filtering, while noncollinear geometries require spectral filtering to achieve the same values. We also find that the spectrum is narrower for nondegenerate SPDC than for degenerate SPDC, leading to lower joint count rates and higher heralding efficiency in the former. In addition to the theory, we verify selected predictions with experimental results.
There are several problems that must be solved in order to increase the distance of quantum communication protocols based on photons as an information carriers. One of them is the dispersion, whose effects can be minimized by engineering spectral properties of transmitted photons. In particular, it is expected that positively correlated photon pairs can be very useful. We present the full characterization of a source of single photon pairs at a telecom wavelength based on type II spontaneous parametric down conversion (SPDC) process in a beta-barium borate (BBO) crystal. In the type II process, a pump photon, which is polarized extraordinarily, splits in a nonlinear medium into signal and idler photons, which are polarized perpendicularly to each other. In order for the process to be efficient a phase matching condition must be fulfilled. These conditions originate from momentum and energy conservation rules and put severe restrictions on source parameters. Seemingly, these conditions force the photon pair to be negatively correlated in their spectral domain. However, it is possible to achieve positive correlation for pulsed pumping. The experimentally available degrees of freedom of a source are the width of the pumping beam, the collected modes’ widths, the length of the nonlinear crystal and the duration of the pumping pulse. In our numerical model we use the following figures of merit: the pair production rate, the efficiency of photon coupling into a single mode fiber, the spectral correlation of the coupled photon pair. The last one is defined as the Pearson correlation parameter for a joint spectral distribution. The aim here is to find the largest positive spectral correlation and the highest coupling efficiency. By resorting to the numerical model Ref. [1] we showed in Ref. [2], that by careful adjustment of the pump’s and the collected modes’ characteristics, one can optimize any of the source's parameters. Our numerical outcomes conform to the experimental results presented in Refs [3,4]. Here we investigate typical, experimentally available source parameters: the widths of the pump beam and collected modes ranging from 20μm to 500m, the crystal length ranging from 1mm to 7.5mm while the pulse duration is set to 50fs, 100fs or 150fs. We achieve the correlation coefficient value as high as approximately 0.8, or – for different values of parameters – coupling efficiency equal to 0.76.
The generation of high purity single photons and entangled photon pairs is a crucial first step in many quantum optics experiments, including those that require quantum teleportation [1], entanglement swapping [2], and the generation of multi-photon entanglement [3]. The most widely used and established approach for creating photon pairs is spontaneous parametric down conversion (SPDC) - where pump photons undergo a non-linear optical process to create a down-converted photon pair [4]. Traditionally, the generation of high-purity heralded single photons required severe spectral filtering, introducing additional loss. However, through careful engineering of spectral correlations of the down-converted photon pairs one can circumvent the need for filtering and avoid the accompanying reduction in heralding efficiency.
Both correlated-mode coupling efficiency and photon pair flux (brightness) of spontaneous parametric down-conversion (SPDC) coupled into single-mode fibers are key parameters for various quantum information science applications. We present an experimental investigation on the optimization of the correlated-mode coupling efficiency and the brightness of frequency-degenerated SPDC photon pairs into single-mode optical fibers. Using photon pairs generated from a type-I phase-matched bulk $\ensuremath{\beta}$-barium borate crystal pumped by a continuous-wave laser, we carefully evaluated both the correlated-mode coupling efficiency and the brightness of SPDC light coupled to a single-mode optical fiber, while continuously changing the focusing of the pump and collection modes, experimenting with Rayleigh lengths from 3 to 280 (for the pump) and 0.2 to 20 (for the collection) times the crystal length. The measured data suggest that the correlated-mode coupling efficiency can be close to unity for any pump focus, however, the optimal Rayleigh length of the collection mode depends on the pump focus parameter, and the brightness can be increased by tightening the pump focus, provided that the Rayleigh length of the collection mode is precisely adjusted. A maximal correlated-mode coupling efficiency of $99.0\ifmmode\pm\else\textpm\fi{}1.3%$ was experimentally achieved. These results will be useful for photonic quantum science and technology using SPDC sources with high heralding efficiencies.
Spontaneous parametric down-conversion (SPDC) is one of the most widely used sources of polarization-entangled photon pairs, and understanding the generated biphoton state is essential for realizing high-brightness and high-purity entangled-photon sources. In particular, Type-II SPDC produces a biphoton wavefunction with a complex coupling between the spatial and polarization degrees of freedom owing to birefringence. In this study, we calculate the real-space distribution of the two-photon polarization state from the biphoton wavefunction of Type-II SPDC generated in a \b{eta}-barium borate (BBO) crystal. By identifying the spatial correlation direction between polarization and real-space coordinates, we designed aperture shapes that restrict the collection along this correlation direction. Through both numerical simulations and experiments, we demonstrate that such correlation-aligned apertures simultaneously achieve higher entanglement purity and improved photon collection efficiency. These results establish a practical design principle for optimizing aperture geometries based on the real-space biphoton wavefunction, providing a new approach to realizing high-purity and high-brightness SPDC entangled-photon sources.