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arXiv:2312.16583 · Quantum Information Processing

Limitations on the maximal level of entanglement of two singlet–triplet qubits in GaAs quantum dots

Igor Bragar, Łukasz Cywiński

Published May 29, 2024• 0 citations
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Abstract

Abstract We analyze in detail a procedure of entangling of two singlet–triplet (S– $$T_{0}$$ T 0 ) qubits operated in a regime when energy associated with the magnetic field gradient, $$\Delta B_{z}$$ Δ B z , is an order of magnitude smaller than the exchange energy, J, between singlet and triplet states (Shulman et al. in Science 336:202, 2012). We have studied theoretically a single S– $$T_{0}$$ T 0 qubit in free induction decay and spin echo experiments. We have obtained analytical expressions for the time dependence of components of its Bloch vector for quasistatic fluctuations of $$\Delta B_{z}$$ Δ B z and quasistatic or dynamical $$1/f^{\beta }$$ 1 / f β -type fluctuations of J. We have then considered the impact of fluctuations of these parameters on the efficiency of the entangling procedure which uses an Ising-type coupling between two S– $$T_{0}$$ T 0 qubits. In particular, we have obtained an analytical expression for evolution of two qubits affected by $$1/f^{\beta }$$ 1 / f β -type fluctuations of J. This expression indicates the maximal level of entanglement that can be generated by performing the entangling procedure. Our results deliver also an evidence that in the above-mentioned experiment S– $$T_{0}$$ T 0 qubits were affected by uncorrelated $$1/f^{\beta }$$ 1 / f β charge noises.

DOI
10.1007/s11128-024-04407-9

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Abstract We analyze in detail a procedure of entangling of two singlet–triplet (S– T0T_{0}T0​ T 0 ) qubits operated in a regime when energy associated with the magnetic field gradient, ΔBz\Delta B_{z}ΔBz​ Δ B z , is an order of magnitude smaller than the exchange energy, J, between singlet and triplet states (Shulman et al. in Science 336:202, 2012). We have studied theoretically a single S– T0T_{0}T0​ T 0 qubit in free induction decay and spin echo experiments. We have obtained analytical expressions for the time dependence of components of its Bloch vector for quasistatic fluctuations of ΔBz\Delta B_{z}ΔBz​ Δ B z and quasistatic or dynamical 1/fβ1/f^{\beta }1/fβ 1 / f β -type fluctuations of J. We have then considered the impact of fluctuations of these parameters on the efficiency of the entangling procedure which uses an Ising-type coupling between two S– T0T_{0}T0​ T 0 qubits. In particular, we have obtained an analytical expression for evolution of two qubits affected by 1/fβ1/f^{\beta }1/fβ 1 / f β -type fluctuations of J. This expression indicates the maximal level of entanglement that can be generated by performing the entangling procedure. Our results deliver also an evidence that in the above-mentioned experiment S– T0T_{0}T0​ T 0 qubits were affected by uncorrelated 1/fβ1/f^{\beta }1/fβ 1 / f β charge noises.
We develop a theoretical model to describe the dissipative dynamics of singlet-triplet qubits in GaAs quantum dots. Using the concurrence experimentally obtained [Shulman et al., Science 336, 202 (2012)] as a guide, we assume that each logical qubit fluctuates under the action of a random telegraph noise (RTN) that simulates the $1/{f}^{\ensuremath{\alpha}}$ noise. We also study the dynamics of concurrence as a function of the amplitude of the RTN, the correlation time of the RTN, the preparation time of states, and the two-qubit coupling. Furthermore, we show that the two-qubit coupling together with the preparation time strongly affect the entanglement dissipative dynamics and both physical quantities can be employed to enhance the entanglement between singlet-triplet qubits.
Singlet-triplet qubits in lateral quantum dots in semiconductor heterostructures exhibit high-fidelity single-qubit gates via exchange interactions and magnetic field gradients. High-fidelity two-qubit entangling gates are challenging to generate since weak interqubit interactions result in slow gates that accumulate error in the presence of noise. However, the interqubit electrostatic interaction also produces a shift in the local double well detunings, effectively changing the dependence of exchange on the gate voltages. We consider an operating point where the effective exchange is first-order insensitive to charge fluctuations while maintaining nonzero interactions. This ``sweet spot'' exists only in the presence of interactions. We show that working at the interacting sweet spot can directly produce maximally entangling gates, and we simulate the gate evolution under realistic 1/f1/f1/f noise. We report theoretical two-qubit gate fidelities above 99% in GaAs and Si systems.
Electron spins confined in semiconductor quantum dots are emerging as a promising system to study quantum information science and to perform sensitive metrology. Their weak interaction with the environment leads to long coherence times and robust storage for quantum information, and the intrinsic tunability of semiconductors allows for controllable operations, initialization, and readout of their quantum state. These spin qubits are also promising candidates for the building block for a scalable quantum information processor due to their prospects for scalability and miniaturization. owever, several obstacles limit the performance of quantum information experiments in these systems. For example, the weak coupling to the environment makes inter-qubit operations challenging, and a fluctuating nuclear magnetic field limits the performance of single-qubit operations.\n\n\n\nThe focus of this thesis will be several experiments which address some of the outstanding problems in semiconductor spin qubits, in particular, singlet-triplet (S-T0) qubits. We use these qubits to probe both the electric field and magnetic field noise that limit the performance of these qubits. The magnetic noise bath is probed with high bandwidth and precision using novel techniques borrowed from the field of Hamiltonian learning, which are effective due to the rapid control and readout available in S-T0 qubits. These findings allow us to effectively undo the undesired effects of the fluctuating nuclear magnetic field by tracking them in real-time, and we demonstrate a 30-fold improvement in the coherence time T2*.\n\n\n\nWe probe the voltage noise environment of the qubit using coherent qubit oscillations, which is partially enabled by control of the nuclear magnetic field. We find that the voltage noise bath is frequency- dependent, even at frequencies as high as 1MHz, and it shows surprising and, as of yet, unexplained temperature dependence. We leverage this knowledge of the voltage noise environment, the nuclear magnetic field control, as well as new techniques for calibrated measurement of the density matrix in a singlet-triplet qubit to entangle two adjacent single-triplet qubits. We fully characterize the generated entangled states and prove that they are, indeed, entangled.\n\n\n\nThis work opens new opportunities to use qubits as sensors for improved metrological capabilities, as well as for improved quantum information processing. The singlet-triplet qubit is unique in that it can be used to probe two fundamentally different noise baths, which are important for a large variety of solid state qubits. More specifically, this work establishes the singlet-triplet qubit as a viable candidate for the building block of a scalable quantum information processor.
There is a huge, worldwide effort to build a quantum computer due to its potential to perform chemical and materials simulations and to break current cryptography schemes. While there has been incredible progress in recent years, each potential platform still faces meaningful obstacles. The singlet-triplet qubit in gallium arsenide, which is based on electric spin, boasts several advantages, including fast single-gate times and readout, long lifetimes, and a clear path to large-scale integration using current semiconductor manufacturing techniques. However, it also suffers from electric and magnetic field noise that limits coherence time and weak two-qubit interactions, which have prevented the construction of multi-qubit systems so far. In this thesis, I will discuss my research measuring and working to improve noise and entangling gates in singlet-triplet qubits and will examine the viability of the singlet-triplet qubit as the building block for a quantum computer. \nBy measuring the dynamics of the electric and magnetic field noise that the singlet-triplet experiences, we can develop an understanding of their origins and how to reduce their impact. The singlet-triplet can be operated rapidly enough to use it as a sensor and directly measure the fluctuating magnetic field arising from the nuclear spins in the semiconductor heterostructure surrounding it. We use Hamiltonian parameter estimation, a technique that maximizes the rate at which we learn information, given the strange properties of quantum measurement, to measure magnetic noise to within 15 μT at a rate of 2 kHz, and we use these measurements to provide real-time feedback to system controls, increasing the coherence time by a factor of 30. Charge noise has much larger high-frequency components than magnetic noise, and thus requires use of dynamical decoupling methods borrowed from NMR to measure it. We measure its power spectrum up to 1 MHz and find that it has a 1/f spectrum. We perform these measurements for several different devices and have begun to determine how our growth and fabrication processes affect dephasing. \nPlacing a high-impedance resonator between two singlet-triplet qubits to mediate their interaction shows promise as way to create long-distance entanglement and to increase the speed of the entangling gate. We analyze this gate theoretically, finding that we expect the fidelity to be over 95%, with a straightforward path to increasing it to above 99% with improved resonator parameters. However, because the singlet-triplet qubit is extremely sensitive to changes in its electrostatic environment, which can be affected both by the resonator’s fabrication process and the presence of the proximal resonator gate, implementing this gate experimentally is challenging. We have developed processes for fabricating narrow, thin, NbN resonators directly adjacent to the double quantum dots that compose singlet-triplet qubits. These processes yield quantum dots that can be tuned into low-noise, stable singlet-triplet qubits, and superconducting resonators with impedances over 1 kOhm.
We analyze a simple exchange-based two-qubit gate for singlet-triplet qubits in gate-defined semiconductor quantum dots that can be implemented in a single exchange pulse. Excitations from the logical subspace are suppressed by a magnetic field gradient that causes spin-flip transitions to be non-energy-conserving. We show that the use of adiabatic pulses greatly reduces leakage processes comapred to square pulses. We also characterize the effect of charge noise on the entanglement fidelity of the gate both analytically and in simulations; demonstrating high entanglement fidelities for physically realistic experimental parameters. Specifically we find that it is possible to achieve fidelities and gate times that are comparable to single-qubit states using realistic magnetic field gradients.
We investigate a method for entangling two singlet-triplet qubits in adjacent double quantum dots via capacitive interactions. In contrast to prior work, here we focus on a regime with strong interactions between the qubits. The interplay of the interaction energy and simultaneous large detunings for both double dots gives rise to the ``double charge resonant'' regime, in which the unpolarized (1111) and fully polarized (0202) four-electron states in the absence of interqubit tunneling are near degeneracy, while being energetically well separated from the partially polarized (0211 and 1102) states. A rapid controlled-phase gate may be realized by combining time evolution in this regime in the presence of intraqubit tunneling and the interqubit Coulomb interaction with refocusing $\ensuremath{\pi}$ pulses that swap the singly occupied singlet and triplet states of the two qubits via, e.g., magnetic gradients. We calculate the fidelity of this entangling gate, incorporating models for two types of noise---charge fluctuations in the single-qubit detunings and charge relaxation within the low-energy subspace via electron-phonon interaction---and identify parameter regimes that optimize the fidelity. The rates of phonon-induced decay for pairs of GaAs or Si double quantum dots vary with the sizes of the dipolar and quadrupolar contributions and are several orders of magnitude smaller for Si, leading to high theoretical gate fidelities for coupled singlet-triplet qubits in Si dots. We also consider the dependence of the capacitive coupling on the relative orientation of the double dots and find that a linear geometry provides the fastest potential gate.