We present a theoretical model of matter-wave diffraction through a material nanostructure. This model is based on the numerical solution of the time-dependent Schr{ö}dinger equation, which goes beyond the standard semi-classical approach. In particular, we consider the dispersion force interaction between the atoms and the material, which is responsible for high energy variations. The effect of such forces on the quantum model is investigated, along with a comparison with the semi-classical model. In particular, for atoms at low velocity and close to the material surface, the semi-classical approach fails, while the quantum model accurately describes the expected diffraction pattern. This description is thus relevant for slow and cold atom experiments where increased precision is required, e.g. for metrological applications.
We present a theoretical model of matter-wave diffraction through a material nanostructure. This model is based on the numerical solution of the time-dependent Schr{ö}dinger equation, which goes beyond the standard semi-classical approach. In particular, we consider the dispersion force interaction between the atoms and the material, which is responsible for high energy variations. The effect of such forces on the quantum model is investigated, along with a comparison with the semi-classical model. In particular, for atoms at low velocity and close to the material surface, the semi-classical approach fails, while the quantum model accurately describes the expected diffraction pattern. This description is thus relevant for slow and cold atom experiments where increased precision is required, e.g. for metrological applications.
We present a theoretical model of matter-wave diffraction through a material nanostructure. This model is based on the numerical solution of the time-dependent Schrödinger equation, which goes beyond the standard semiclassical approach. In particular, we consider the dispersion force interaction between the atoms and the material, which is responsible for high energy variations. The effect of such forces on the quantum model is investigated, along with a comparison with the semiclassical model. In particular, for atoms at low velocity and close to the material surface, the semiclassical approach fails, while the quantum model accurately describes the expected diffraction pattern. This description is thus relevant for slow and cold atom experiments where increased precision is required, e.g., for metrological applications. Published by the American Physical Society 2024
Abstract The diffraction of atoms and molecules through tiny, sub-nanometre holes in atomically thin membranes is a promising approach for advancing atom interferometry sensing and atomic holography. However, dispersion interactions, such as the Casimir-Polder force, pose a significant challenge by attracting diffracting particles to the membrane, limiting the minimum hole size. This paper presents a numerical simulation of helium matter-wave diffraction through sub-nanometre holes in hexagonal boron nitride by solving the time-dependent Schrödinger equation. Our results show that the transmission rates in the quantum approach are significantly higher than those predicted by the commonly used semi-classical approach. This suggests that significantly smaller holes can be used in the design of diffractive masks, provided that fabrication techniques can meet the atomic-level precision to realise such holes. Furthermore, we observe notable differences in diffraction patterns, even for atom velocities that are much greater than the expected convergence threshold between semi-classical and quantum computational models.
This work considers the semi-classical description of two applications involving cold atoms. This is, on one hand, the behavior of a BOSE-EINSTEIN condensate in hybrid systems, i.e. in contact with a microscopic object (carbon nanotubes, fullerenes, etc.). On the other, the evolution of phase space distributions in matter wave interferometers utilizing ray tracing methods was discussed. For describing condensates in hybrid systems, one can map the GROSS-PITAEVSKII equation, a differential equation in the complex-valued macroscopic wave function, onto a system of two differential equations in density and phase. Neglecting quantum dispersion, one obtains a semiclassical description which is easily modified to incorporate interactions between condensate and microscopical object. In our model, these interactions comprise attractive forces (CASIMIR-POLDER forces) and loss of condensed atoms due to inelastic collisions at the surface of the object. Our model exhibited the excitation of sound waves that are triggered by the object’s rapid immersion, and spread across the condensate thereafter. Moreover, local particle loss leads to a shrinking of the bulk condensate. We showed that the total number of condensed particles is decreasing potentially in the beginning (large condensate, strong mean field interaction), while it decays exponentially in the long-time limit (small condensate, mean field inetraction negligible). For representing the physics of matter wave interferometers in phase space, we utilized the WIGNER function. In semi-classical approximation, which again consists in ignoring the quantum dispersion, this representation is subject to the same equation of motion as classical phase space distributions, i.e. the LIOUVILLE equation. This implies that time evolution of theWIGNER function follows a phase space flow that consists of classical trajectories (classical transport). This means, for calculating a time-evolved distribution, one has know the initial distribution and one has to solve the classical equations of motion. Concerning the initial distribution, we have studied a stationary solution of the nonlinear LIOUVILLE equation, the LAMBERT density. We saw that it agrees very well with results from singleparticle quantum mechanics as well as the MAXWELL-BOLTZMANN distribution in the weakly interacting limit. Likewise, in the strongly interacting limit, familiar results of the THOMAS-FERMI approximation are recovered. A distribution that is first prepared in a trap and then released can be described quite conveniently in terms of WIGNER functions. However, propagation in optical potentials associated to the interferometer elements (beam splitter, Pi-half-pulse) do not satisfy the condition of the semiclassical approximation. Nevertheless, one finds discrete before-after mappings that describe the effect of these elements on incident distributions. This leads to several channels of phase space propagation which relate to the interferometer paths and interferences between them. The formalism for WIGNER functions in an interferometer can be translated straightforwardly into a ray tracing algorithm. As mentioned above, this algorithm solves the classical equations of motion and computes time-evolved distributions, using values of the initial distribution. This procedure, in contrast to most analytical solutions, does not require the HAMILTON function to be quadratic (e.g. free propagation, const. acceleration, harmonic oscillator). We compared simulation results to analytic expressions in case of freely propagating GAUSS distribution. They showed perfect agreement, especially for the functional dependence of wave length and contrast of interference fringes on the laser pulse timings.
Abstract Among the fundamental quantum effects, quantum reflection (QR) is one of the most notable phenomena. Approximating arbitrary potentials in the Schrödinger equation as multistep potentials allows us to determine the reflection coefficient by means of a Riccati equation. We introduce a measure for the wave function's characteristic reflection distance and derive an analytical expression for this reflection point in an arbitrary power-law potential. We study the associated QR rate in the context of Casimir-Polder atom surface interactions, revealing its strong dependence on critical parameters such as velocity and interaction duration. As an application, we demonstrate how the matter-wave diffraction of a low-velocity metastable argon beam impinging on a rotated grating facilitates high-precision potential analysis.
Quantum reflection occurs when ultra-cold atoms are incident on a material surface with sufficiently low velocity. The reflecting matter wave can interfere with the incident wave to form a detectable pattern, and this pattern contains information about atom-surface interactions at micrometer scales. We discuss how such an interferometer could be used to probe for anomalous short-range forces that are predicted by some beyond-standard model theories. We compare a simple analytical model for the anomalous phase to numerical solution of both the Schroedinger and Gross-Pitaevskii equations, finding good agreement. With interactions, the phase does depend on the atomic density, which can be a source of noise. We nonetheless predict that under realistic conditions, the reflection technique can reach sensitivities approaching those obtained with macroscopic objects, and significantly improve the limits on anomalous coupling to atoms.
Fabricating patterned nanostructures with matter waves can help to realise new nanophotonic devices. However, due to dispersion effects, designing patterns with nanoscale features is challenging. Here, we consider the propagation of a helium matter wave through different holes in hexagonal boron nitride (h-BN) as a case study for the weakest dispersion interaction and the matter wave's diffraction as it passes through the holes. We use a quantum-mechanical model to calculate the polarisability of edge atoms around the holes, where we observe polarisation ripples of enhanced and reduced polarisabilities around the holes. We use these values to calculate van der Waals dispersion coefficients for the scattered helium atoms. We find that the resulting diffraction patterns are affected by the shape and size of the holes, where the smallest holes have a radius of just 6 Å. These results can be used to predict the resolution limits of nano-hole patterns on nanophotonic materials.